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description Publicationkeyboard_double_arrow_right Article 2022 SpainPublisher:Elsevier BV Funded by:EC | BRISK II, EC | GTCLC-NEGEC| BRISK II ,EC| GTCLC-NEGHaodi Tan; Minjiao Yang; Yingquan Chen; Xu Chen; Francesco Fantozzi; Pietro Bartocci; Roman Tschentscher; Federica Barontini; Haiping Yang; Hanping Chen;handle: 10261/306654
9 figures, 1 table.-- Supplementary information available.-- © 2023. This manuscript version is made available under the CC-BY-NC-ND 4.0 license https://creativecommons.org/licenses/by-nc-nd/4.0/ Catalytic pyrolysis of digestate to produce aromatic hydrocarbons can be combined with anaerobic fermentation to effectively transform and utilize all biomass components, which can achieve the meaningful purpose of transforming waste into high-value products. This study explored whether catalytic pyrolysis of digestate is feasible to prepare aromatic hydrocarbons by analyzing the thermogravimetric characteristics, pyrolysis characteristics, and catalytic pyrolysis characteristics of digestate. For digestate pyrolysis, an increase in temperature was found to elevate the CO, CH4, and monocyclic aromatic hydrocarbon (benzene, toluene, and xylene; BTX) content, whereas it decreased the contents of phenols, acids, aldehydes, and other oxygenates. Furthermore, the catalytic pyrolysis process effectively inhibited the acids, phenols, and furans in the liquid, whereas the yield of BTX increased from 25.45% to 45.99%, and the selectivity of xylene was also increased from 10.32% to 28.72% after adding ZSM-5. ZSM-5 also inhibited the production of nitrogenous compounds. This work was partially funded by the GTCLC-NEG project, which received funding from the European Union’s Horizon 2020 Research and Innovation Programme under the Marie Sklodowska-Curie Grant Agreement(101018756). The authors would like to thank the Brisk 2 European project (731101) for funding this project. The project acronym was B2PB-SIN2-1001, and the project title was “Optimization of catalytic pyrolysis of digestate and sewage sludge.” The authors would also like to acknowledge the COST Action CA17128 “Establishment of a Pan-European Network on the Sustainable Valorisation of Lignin (LignoCOST)” for useful discussions on lignin valorization. Peer reviewed
Recolector de Cienci... arrow_drop_down Recolector de Ciencia Abierta, RECOLECTAArticle . 2022 . Peer-reviewedData sources: Recolector de Ciencia Abierta, RECOLECTAChinese Journal of Chemical EngineeringArticle . 2023 . Peer-reviewedLicense: Elsevier TDMData sources: Crossrefadd ClaimPlease grant OpenAIRE to access and update your ORCID works.This Research product is the result of merged Research products in OpenAIRE.
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For further information contact us at helpdesk@openaire.eu5 citations 5 popularity Average influence Average impulse Top 10% Powered by BIP!
more_vert Recolector de Cienci... arrow_drop_down Recolector de Ciencia Abierta, RECOLECTAArticle . 2022 . Peer-reviewedData sources: Recolector de Ciencia Abierta, RECOLECTAChinese Journal of Chemical EngineeringArticle . 2023 . Peer-reviewedLicense: Elsevier TDMData sources: Crossrefadd ClaimPlease grant OpenAIRE to access and update your ORCID works.This Research product is the result of merged Research products in OpenAIRE.
You have already added works in your ORCID record related to the merged Research product.This Research product is the result of merged Research products in OpenAIRE.
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description Publicationkeyboard_double_arrow_right Article 2022 SpainPublisher:Elsevier BV Funded by:EC | BRISK II, EC | GTCLC-NEGEC| BRISK II ,EC| GTCLC-NEGHaodi Tan; Minjiao Yang; Yingquan Chen; Xu Chen; Francesco Fantozzi; Pietro Bartocci; Roman Tschentscher; Federica Barontini; Haiping Yang; Hanping Chen;handle: 10261/306654
9 figures, 1 table.-- Supplementary information available.-- © 2023. This manuscript version is made available under the CC-BY-NC-ND 4.0 license https://creativecommons.org/licenses/by-nc-nd/4.0/ Catalytic pyrolysis of digestate to produce aromatic hydrocarbons can be combined with anaerobic fermentation to effectively transform and utilize all biomass components, which can achieve the meaningful purpose of transforming waste into high-value products. This study explored whether catalytic pyrolysis of digestate is feasible to prepare aromatic hydrocarbons by analyzing the thermogravimetric characteristics, pyrolysis characteristics, and catalytic pyrolysis characteristics of digestate. For digestate pyrolysis, an increase in temperature was found to elevate the CO, CH4, and monocyclic aromatic hydrocarbon (benzene, toluene, and xylene; BTX) content, whereas it decreased the contents of phenols, acids, aldehydes, and other oxygenates. Furthermore, the catalytic pyrolysis process effectively inhibited the acids, phenols, and furans in the liquid, whereas the yield of BTX increased from 25.45% to 45.99%, and the selectivity of xylene was also increased from 10.32% to 28.72% after adding ZSM-5. ZSM-5 also inhibited the production of nitrogenous compounds. This work was partially funded by the GTCLC-NEG project, which received funding from the European Union’s Horizon 2020 Research and Innovation Programme under the Marie Sklodowska-Curie Grant Agreement(101018756). The authors would like to thank the Brisk 2 European project (731101) for funding this project. The project acronym was B2PB-SIN2-1001, and the project title was “Optimization of catalytic pyrolysis of digestate and sewage sludge.” The authors would also like to acknowledge the COST Action CA17128 “Establishment of a Pan-European Network on the Sustainable Valorisation of Lignin (LignoCOST)” for useful discussions on lignin valorization. Peer reviewed
Recolector de Cienci... arrow_drop_down Recolector de Ciencia Abierta, RECOLECTAArticle . 2022 . Peer-reviewedData sources: Recolector de Ciencia Abierta, RECOLECTAChinese Journal of Chemical EngineeringArticle . 2023 . Peer-reviewedLicense: Elsevier TDMData sources: Crossrefadd ClaimPlease grant OpenAIRE to access and update your ORCID works.This Research product is the result of merged Research products in OpenAIRE.
You have already added works in your ORCID record related to the merged Research product.This Research product is the result of merged Research products in OpenAIRE.
You have already added works in your ORCID record related to the merged Research product.All Research productsarrow_drop_down <script type="text/javascript"> <!-- document.write('<div id="oa_widget"></div>'); document.write('<script type="text/javascript" src="https://beta.openaire.eu/index.php?option=com_openaire&view=widget&format=raw&projectId=10.1016/j.cjche.2022.09.002&type=result"></script>'); --> </script>
For further information contact us at helpdesk@openaire.eu5 citations 5 popularity Average influence Average impulse Top 10% Powered by BIP!
more_vert Recolector de Cienci... arrow_drop_down Recolector de Ciencia Abierta, RECOLECTAArticle . 2022 . Peer-reviewedData sources: Recolector de Ciencia Abierta, RECOLECTAChinese Journal of Chemical EngineeringArticle . 2023 . Peer-reviewedLicense: Elsevier TDMData sources: Crossrefadd ClaimPlease grant OpenAIRE to access and update your ORCID works.This Research product is the result of merged Research products in OpenAIRE.
You have already added works in your ORCID record related to the merged Research product.This Research product is the result of merged Research products in OpenAIRE.
You have already added works in your ORCID record related to the merged Research product.All Research productsarrow_drop_down <script type="text/javascript"> <!-- document.write('<div id="oa_widget"></div>'); document.write('<script type="text/javascript" src="https://beta.openaire.eu/index.php?option=com_openaire&view=widget&format=raw&projectId=10.1016/j.cjche.2022.09.002&type=result"></script>'); --> </script>
For further information contact us at helpdesk@openaire.eu