• Energy Research

Abstract The first detailed study on the performance of a ZnO-based cryogenic scintillating bolometer as a detector to search for rare processes in zinc isotopes was carried out. A 7.2 g ZnO low-temperature detector, containing more than 80% of zinc in its mass, exhibits good energy resolution of baseline noise 1.0–2.7 keV FWHM at various working temperatures resulting in a low-energy threshold for the experiment, 2.0–6.0 keV. The light yield for β/γ events was measured as 1.5(3) keV/MeV, while it varies for α particles in the range of 0.2–3.0 keV/MeV. The detector demonstrates an effective identification of β/γ events from α events using time-properties of only heat signals. The radiopurity of the ZnO crystal was evaluated using the Inductively Coupled Plasma Mass Spectrometry, an ultra-low-background High Purity Ge γ-spectrometer, and bolometric measurements. Only limits were set at the level of 𝒪(1–100) mBq/kg on activities of 40K, 137Cs and daughter nuclides from the U/Th natural decay chains. The total internal α-activity was measured as 22(2) mBq/kg, with a major contribution caused by 6(1) mBq/kg of 232Th and 12(2) mBq/kg of 234U. Limits on double beta decay (DBD) processes in ^64Zn and 70Zn isotopes were set on the level of 𝒪(1017–1018) yr for various decay modes, profiting from 271 h of acquired background data in the above-ground lab. This study shows a good potential for ZnO-based scintillating bolometers to search for DBD processes of Zn isotopes, especially in 64Zn, with the most prominent spectral features at ∼ 10–20 keV, like the two-neutrino double electron capture. A 10 kg-scale experiment can reach the experimental sensitivity at the level of 𝒪(1024) yr.

AbstractThe CUPID-Mo experiment to search for 0$$\nu \beta \beta $$ ν β β decay in $$^{100}$$ 100 Mo has been recently completed after about 1.5 years of operation at Laboratoire Souterrain de Modane (France). It served as a demonstrator for CUPID, a next generation 0$$\nu \beta \beta $$ ν β β decay experiment. CUPID-Mo was comprised of 20 enriched $$\hbox {Li}_{{2}}$$ Li 2 $$^{100}$$ 100 $$\hbox {MoO}_4$$ MoO 4 scintillating calorimeters, each with a mass of $$\sim 0.2$$ ∼ 0.2  kg, operated at $$\sim 20$$ ∼ 20  mK. We present here the final analysis with the full exposure of CUPID-Mo ($$^{100}$$ 100 Mo exposure of 1.47 $$\hbox {kg} \times \hbox {year}$$ kg × year ) used to search for lepton number violation via 0$$\nu \beta \beta $$ ν β β decay. We report on various analysis improvements since the previous result on a subset of data, reprocessing all data with these new techniques. We observe zero events in the region of interest and set a new limit on the $$^{100}$$ 100 Mo 0$$\nu \beta \beta $$ ν β β decay half-life of $$T_{1/2}^{0\nu }$$ T 1 / 2 0 ν $$> {1.8}\times 10^{24}$$ > 1.8 × 10 24  year (stat. + syst.) at 90% CI. Under the light Majorana neutrino exchange mechanism this corresponds to an effective Majorana neutrino mass of $$\left<m_{\beta \beta }\right>$$ m β β $$<~{(0.28{-}0.49)} $$ < ( 0.28 - 0.49 )  eV, dependent upon the nuclear matrix element utilized.

We present the first search for the Majoron-emitting modes of the neutrinoless double $β$ decay ($0νββχ_0$) using scintillating cryogenic calorimeters. We analysed the CUPID-0 Phase I data using a Bayesian approach to reconstruct the background sources activities, and evaluate the potential contribution of the $^{82}$Se $0νββχ_0$. We considered several possible theoretical models which predict the existence of a Majoron-like boson coupling to the neutrino. The energy spectra arising from the emission of such bosons in the neutrinoless double $β$ decay have spectral indices $n=$ 1, 2, 3 or 7. We found no evidence of any of these decay modes, setting a lower limit (90% of credibility interval) on the half-life of 1.2 $\times$ 10$^{23}$ yr in the case of $n=$ 1, 3.8 $\times$ 10$^{22}$ yr for $n=$ 2, 1.4 $\times$ 10$^{22}$ yr for $n=$ 3 and 2.2 $\times$ 10$^{21}$ yr for $n=$ 7. These are the best limits on the $0νββχ_0$ half-life of the $^{82}$Se, and demonstrate the potentiality of the CUPID-0 technology in this field.