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  • Energy Research

  • Effects of heat treatment atmosphere on the structure and activity of Pt3Sn nanoparticle electrocatalysts: a characterisation case study

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2018 United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | University of Bristol - E..., UKRI | The UK Catalysis Hub, UKRI | Catalytic Science in the ... +4 projects
    Authors: Vinod Kumar Puthiyapura; Vinod Kumar Puthiyapura; Dan J. L. Brett; Haoliang Huang; +6 Authors

    doi: 10.1039/c7fd00221a

    pmid: 29851419

    handle: 1983/e4e756a4-b0e8-45c7-923b-d4c646a58811

    In this work, a variation in heat treatment atmosphere approach is taken to provide a series of related PtSn catalysts with the same nominal composition of Pt3Sn, but with different surface compositions.

    downloadFull-Text
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ e-Prints Sotonarrow_drop_down
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    e-Prints Soton
    Article . 2018 . Peer-reviewed
    Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
    Data sources: e-Prints Soton
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    e-Prints Soton
    Article . 2018
    License: CC BY
    Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
    Data sources: Bielefeld Academic Search Engine (BASE)
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Faraday Discussions
    Article . 2018 . Peer-reviewed
    License: CC BY
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    Faraday Discussions
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    Faraday Discussions
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    Explore Bristol Research
    Article . 2018
    Data sources: Explore Bristol Research
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    The University of Manchester - Institutional Repository
    Article . 2018
    Data sources: The University of Manchester - Institutional Repository
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    University of Bristol: Bristol Research
    Article . 2018
    Data sources: Bielefeld Academic Search Engine (BASE)
    Faraday Discussions
    Article . 2019
    Data sources: Europe PubMed Central
    Faraday Discussions
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ e-Prints Sotonarrow_drop_down
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      e-Prints Soton
      Article . 2018 . Peer-reviewed
      Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
      Data sources: e-Prints Soton
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      e-Prints Soton
      Article . 2018
      License: CC BY
      Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
      Data sources: Bielefeld Academic Search Engine (BASE)
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Faraday Discussions
      Article . 2018 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Faraday Discussions
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      Faraday Discussions
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      Explore Bristol Research
      Article . 2018
      Data sources: Explore Bristol Research
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      The University of Manchester - Institutional Repository
      Article . 2018
      Data sources: The University of Manchester - Institutional Repository
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      University of Bristol: Bristol Research
      Article . 2018
      Data sources: Bielefeld Academic Search Engine (BASE)
      Faraday Discussions
      Article . 2019
      Data sources: Europe PubMed Central
      Faraday Discussions
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      Data sources: Microsoft Academic Graph
      Claim

      This Research product is the result of merged Research products in OpenAIRE.

      You have already added works in your ORCID record related to the merged Research product.

  • Effects of heat treatment atmosphere on the structure and activity of Pt3Sn nanoparticle electrocatalysts: a characterisation case study

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2018 United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | University of Bristol - E..., UKRI | The UK Catalysis Hub, UKRI | Catalytic Science in the ... +4 projects
    Authors: Vinod Kumar Puthiyapura; Vinod Kumar Puthiyapura; Dan J. L. Brett; Haoliang Huang; +6 Authors

    doi: 10.1039/c7fd00221a

    pmid: 29851419

    handle: 1983/e4e756a4-b0e8-45c7-923b-d4c646a58811

    In this work, a variation in heat treatment atmosphere approach is taken to provide a series of related PtSn catalysts with the same nominal composition of Pt3Sn, but with different surface compositions.

    downloadFull-Text
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ e-Prints Sotonarrow_drop_down
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    e-Prints Soton
    Article . 2018 . Peer-reviewed
    Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
    Data sources: e-Prints Soton
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    e-Prints Soton
    Article . 2018
    License: CC BY
    Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
    Data sources: Bielefeld Academic Search Engine (BASE)
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Faraday Discussions
    Article . 2018 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Faraday Discussions
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    License: CC BY
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    Faraday Discussions
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    Explore Bristol Research
    Article . 2018
    Data sources: Explore Bristol Research
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    The University of Manchester - Institutional Repository
    Article . 2018
    Data sources: The University of Manchester - Institutional Repository
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    University of Bristol: Bristol Research
    Article . 2018
    Data sources: Bielefeld Academic Search Engine (BASE)
    Faraday Discussions
    Article . 2019
    Data sources: Europe PubMed Central
    Faraday Discussions
    Journal
    Data sources: Microsoft Academic Graph
    Claim

    This Research product is the result of merged Research products in OpenAIRE.

    You have already added works in your ORCID record related to the merged Research product.
    Access Routes
    Green
    hybrid
    14
    citations14
    popularityTop 10%
    influenceAverage
    impulseTop 10%
    BIP!Powered by BIP!
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      downloadFull-Text
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ e-Prints Sotonarrow_drop_down
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      e-Prints Soton
      Article . 2018 . Peer-reviewed
      Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
      Data sources: e-Prints Soton
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      e-Prints Soton
      Article . 2018
      License: CC BY
      Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
      Data sources: Bielefeld Academic Search Engine (BASE)
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      Faraday Discussions
      Article . 2018 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
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      Faraday Discussions
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      Faraday Discussions
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      Explore Bristol Research
      Article . 2018
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      The University of Manchester - Institutional Repository
      Article . 2018
      Data sources: The University of Manchester - Institutional Repository
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      University of Bristol: Bristol Research
      Article . 2018
      Data sources: Bielefeld Academic Search Engine (BASE)
      Faraday Discussions
      Article . 2019
      Data sources: Europe PubMed Central
      Faraday Discussions
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      Data sources: Microsoft Academic Graph
      Claim

      This Research product is the result of merged Research products in OpenAIRE.

      You have already added works in your ORCID record related to the merged Research product.

  • Understanding the Competitive Gas Absorption of CO2 and SO2 in Superbase Ionic Liquids

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2018 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | A Coordinated, Comprehens..., UKRI | Utilisation of Solar Ener...
    Authors: Johan Jacquemin; Johan Jacquemin; Adam J. Greer; Matthew McClung; +4 Authors

    doi: 10.1021/acs.iecr.8b03623

    During this work, an original study of the CO2 and SO2 competitive gas absorption in three superbase ionic liquids (ILs), namely, trihexyltetradecylphosphonium 1,2,4-triazolide ([P66614][124Triz]), and trihexyltetradecylphoshonium benzimidazolide ([P66614][Benzim]), is reported for the first time. To initiate such a comprehensive study, the CO2 and SO2 mixed gas solubility in selected ILs was determined by using an original and accurate dynamic method coupled with mass spectrometry after several absorption and desorption cycles. This method has been validated by comparing the gravimetric uptake of CO2 with the mass spectrometry data using trihexyltetradecylphosphonium benzotriazolide, 1,2,4-triazolide, and benzimidazolide ILs and shown to be consistent within 10% in mole ratio units. Solubility results clearly show that the presence of SO2 in the gas stream decreases the CO2 capture capability of the investigated ILs. Furthermore, the viscosity, chemical analysis (water content and sulfur content), and sp...

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Industrial & Enginee...arrow_drop_down
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    Industrial & Engineering Chemistry Research
    Article . 2018 . Peer-reviewed
    License: http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html
    Data sources: Crossref
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    Industrial & Engineering Chemistry Research
    Article
    License: CC BY
    Data sources: UnpayWall
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    The University of Manchester - Institutional Repository
    Article . 2018
    Data sources: The University of Manchester - Institutional Repository
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    Hyper Article en Ligne
    Article . 2018
    Data sources: Hyper Article en Ligne
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    Mémoires en Sciences de l'Information et de la Communication
    Article . 2018
    Data sources: Mémoires en Sciences de l'Information et de la Communication
    Industrial & Engineering Chemistry Research
    Journal
    Data sources: Microsoft Academic Graph
    Université François-Rabelais de Tours: HAL
    Article . 2018
    Data sources: Bielefeld Academic Search Engine (BASE)
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      Industrial & Engineering Chemistry Research
      Article . 2018 . Peer-reviewed
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      Industrial & Engineering Chemistry Research
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      The University of Manchester - Institutional Repository
      Article . 2018
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      Article . 2018
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      Mémoires en Sciences de l'Information et de la Communication
      Article . 2018
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      Industrial & Engineering Chemistry Research
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      Université François-Rabelais de Tours: HAL
      Article . 2018
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  • Understanding the Competitive Gas Absorption of CO2 and SO2 in Superbase Ionic Liquids

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2018 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | A Coordinated, Comprehens..., UKRI | Utilisation of Solar Ener...
    Authors: Johan Jacquemin; Johan Jacquemin; Adam J. Greer; Matthew McClung; +4 Authors

    doi: 10.1021/acs.iecr.8b03623

    During this work, an original study of the CO2 and SO2 competitive gas absorption in three superbase ionic liquids (ILs), namely, trihexyltetradecylphosphonium 1,2,4-triazolide ([P66614][124Triz]), and trihexyltetradecylphoshonium benzimidazolide ([P66614][Benzim]), is reported for the first time. To initiate such a comprehensive study, the CO2 and SO2 mixed gas solubility in selected ILs was determined by using an original and accurate dynamic method coupled with mass spectrometry after several absorption and desorption cycles. This method has been validated by comparing the gravimetric uptake of CO2 with the mass spectrometry data using trihexyltetradecylphosphonium benzotriazolide, 1,2,4-triazolide, and benzimidazolide ILs and shown to be consistent within 10% in mole ratio units. Solubility results clearly show that the presence of SO2 in the gas stream decreases the CO2 capture capability of the investigated ILs. Furthermore, the viscosity, chemical analysis (water content and sulfur content), and sp...

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    Industrial & Engineering Chemistry Research
    Article . 2018 . Peer-reviewed
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    Industrial & Engineering Chemistry Research
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    The University of Manchester - Institutional Repository
    Article . 2018
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    Article . 2018
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    Mémoires en Sciences de l'Information et de la Communication
    Article . 2018
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    Industrial & Engineering Chemistry Research
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    Université François-Rabelais de Tours: HAL
    Article . 2018
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      Industrial & Engineering Chemistry Research
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      The University of Manchester - Institutional Repository
      Article . 2018
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      Mémoires en Sciences de l'Information et de la Communication
      Article . 2018
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      Université François-Rabelais de Tours: HAL
      Article . 2018
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  • Factors affecting bubble size in ionic liquids

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    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2017 France, United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | Utilisation of Solar Ener..., UKRI | A Coordinated, Comprehens...
    Authors: William A. Zimmerman; Stuart A. Brittle; Sarah F. R. Taylor; Sarah F. R. Taylor; +5 Authors

    doi: 10.1039/c7cp01725a

    pmid: 28537605

    Bubble behaviour of 11 ionic liquids was studied and the relationship of bubble size, physical properties and structure was examined.

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    White Rose Research Online
    Article . 2017
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    Physical Chemistry Chemical Physics
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    Physical Chemistry Chemical Physics
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    Queen's University Research Portal
    Article . 2017
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    The University of Manchester - Institutional Repository
    Article . 2017
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    Article . 2017
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    Mémoires en Sciences de l'Information et de la Communication
    Article . 2017
    Data sources: Mémoires en Sciences de l'Information et de la Communication
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    Queen's University Belfast Research Portal
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    HAL Université de Tours
    Article . 2017
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    Physical Chemistry Chemical Physics
    Article . 2017 . Peer-reviewed
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    Physical Chemistry Chemical Physics
    Article . 2018
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    Physical Chemistry Chemical Physics
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    Université François-Rabelais de Tours: HAL
    Article . 2017
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      The University of Manchester - Institutional Repository
      Article . 2017
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      HAL Université de Tours
      Article . 2017
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      Physical Chemistry Chemical Physics
      Article . 2017 . Peer-reviewed
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      Physical Chemistry Chemical Physics
      Article . 2018
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      Article . 2017
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  • Factors affecting bubble size in ionic liquids

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2017 France, United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | Utilisation of Solar Ener..., UKRI | A Coordinated, Comprehens...
    Authors: William A. Zimmerman; Stuart A. Brittle; Sarah F. R. Taylor; Sarah F. R. Taylor; +5 Authors

    doi: 10.1039/c7cp01725a

    pmid: 28537605

    Bubble behaviour of 11 ionic liquids was studied and the relationship of bubble size, physical properties and structure was examined.

    downloadFull-Text
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    CORE
    Article . 2017
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    White Rose Research Online
    Article . 2017
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  • How to go beyond C1 products with electrochemical reduction of CO2

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    Authors: Jean-Marie Fontmorin; Jean-Marie Fontmorin; Hang Xiang; Liam Banerji; +14 Authors

    doi: 10.1039/d1se00861g

    This review summaries recent development across electro-, photoelectro- and bioelectro-catalyst developments for multi-carbon products from CO2. It also explores the role of device design and operating conditions in enabling C–C bond generation.

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  • How to go beyond C1 products with electrochemical reduction of CO2

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2021 France Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | Flexible Routes to Liquid..., UKRI | Liquid Fuel and bioEnergy..., UKRI | UKRI Interdisciplinary Ce... +2 projects
    Authors: Jean-Marie Fontmorin; Jean-Marie Fontmorin; Hang Xiang; Liam Banerji; +14 Authors

    doi: 10.1039/d1se00861g

    This review summaries recent development across electro-, photoelectro- and bioelectro-catalyst developments for multi-carbon products from CO2. It also explores the role of device design and operating conditions in enabling C–C bond generation.

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      Sustainable Energy & Fuels
      Article . 2021 . Peer-reviewed
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  • Using lake sediments to assess the long-term impacts of anthropogenic activity in tropical river deltas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Review 2023 United Kingdom, Netherlands, United Kingdom, United Kingdom Publisher:SAGE PublicationsFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Richard E. Walton; Heather Moorhouse; Lucy R. Roberts; Jorge Salgado; +9 Authors

    doi: 10.1177/20530196231204334 , 10.60692/h7teh-1b055 , 10.60692/hq28v-61t17

    pmid: 39156121

    pmc: PMC11324390

    handle: 20.500.11755/e7bb944e-73af-4112-a5e8-ff134b2ea612

    Tropical river deltas, and the social-ecological systems they sustain, are changing rapidly due to anthropogenic activity and climatic change. Baseline data to inform sustainable management options for resilient deltas is urgently needed and palaeolimnology (reconstructing past conditions from lake or wetland deposits) can provide crucial long-term perspectives needed to identify drivers and rates of change. We review how palaeolimnology can be a valuable tool for resource managers using three current issues facing tropical delta regions: hydrology and sediment supply, salinisation and nutrient pollution. The unique ability of palaeolimnological methods to untangle multiple stressors is also discussed. We demonstrate how palaeolimnology has been used to understand each of these issues, in other aquatic environments, to be incorporated into policy. Palaeolimnology is a key tool to understanding how anthropogenic influences interact with other environmental stressors, providing policymakers and resource managers with a ‘big picture’ view and possible holistic solutions that can be implemented.

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    Review . 2023 . Peer-reviewed
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    Newcastle University Library ePrints Service
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    Full-Text: https://eprints.ncl.ac.uk/294122
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    Review . 2023
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    The Anthropocene Review
    Article . 2023 . Peer-reviewed
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    PubMed Central
    Other literature type . 2023
    License: http://creativecommons.org/licenses/by/4.0/This article is distributed under the terms of the Creative Commons Attribution 4.0 License (http://creativecommons.org/licenses/by/4.0/) which permits any use, reproduction and distribution of the work without further permission provided the original work is attributed as specified on the SAGE and Open Access pages (http://us.sagepub.com/en-us/nam/open-access-at-sage).
    Data sources: PubMed Central
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    Article . 2023
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    PURE Aarhus University
    Article . 2024
    Data sources: PURE Aarhus University
    https://dx.doi.org/10.60692/h7...
    Other literature type . 2023
    Data sources: Datacite
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    Other literature type . 2023
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    The Anthropocene Review
    Article
    Data sources: Europe PubMed Central
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  • Using lake sediments to assess the long-term impacts of anthropogenic activity in tropical river deltas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Review 2023 United Kingdom, Netherlands, United Kingdom, United Kingdom Publisher:SAGE PublicationsFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Richard E. Walton; Heather Moorhouse; Lucy R. Roberts; Jorge Salgado; +9 Authors

    doi: 10.1177/20530196231204334 , 10.60692/h7teh-1b055 , 10.60692/hq28v-61t17

    pmid: 39156121

    pmc: PMC11324390

    handle: 20.500.11755/e7bb944e-73af-4112-a5e8-ff134b2ea612

    Tropical river deltas, and the social-ecological systems they sustain, are changing rapidly due to anthropogenic activity and climatic change. Baseline data to inform sustainable management options for resilient deltas is urgently needed and palaeolimnology (reconstructing past conditions from lake or wetland deposits) can provide crucial long-term perspectives needed to identify drivers and rates of change. We review how palaeolimnology can be a valuable tool for resource managers using three current issues facing tropical delta regions: hydrology and sediment supply, salinisation and nutrient pollution. The unique ability of palaeolimnological methods to untangle multiple stressors is also discussed. We demonstrate how palaeolimnology has been used to understand each of these issues, in other aquatic environments, to be incorporated into policy. Palaeolimnology is a key tool to understanding how anthropogenic influences interact with other environmental stressors, providing policymakers and resource managers with a ‘big picture’ view and possible holistic solutions that can be implemented.

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    Full-Text: https://eprints.ncl.ac.uk/294122
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    e-Prints Soton
    Review . 2023
    License: CC BY
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    The Anthropocene Review
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
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    PubMed Central
    Other literature type . 2023
    License: http://creativecommons.org/licenses/by/4.0/This article is distributed under the terms of the Creative Commons Attribution 4.0 License (http://creativecommons.org/licenses/by/4.0/) which permits any use, reproduction and distribution of the work without further permission provided the original work is attributed as specified on the SAGE and Open Access pages (http://us.sagepub.com/en-us/nam/open-access-at-sage).
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    UCL Discovery
    Article . 2023
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    PURE Aarhus University
    Article . 2024
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    https://dx.doi.org/10.60692/h7...
    Other literature type . 2023
    Data sources: Datacite
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    The Anthropocene Review
    Article
    Data sources: Europe PubMed Central
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  • Combined Experimental and Theoretical Study of the Competitive Absorption of CO2 and NO2 by a Superbase Ionic Liquid

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Journal 2021 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | The UK Catalysis Hub - 'S..., UKRI | Biocatalysis & Biotra..., UKRI | Utilisation of Solar Ener...
    Authors: C. Richard A. Catlow; Johan Jacquemin; Matthew G. Quesne; Matthew G. Quesne; +6 Authors

    doi: 10.1021/acssuschemeng.1c01451

    pmid: 34306836

    pmc: PMC8296676

    A superbase ionic liquid (IL), trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is investigated for the capture of CO2 in the presence of NO2 impurities. The effect of the waste gas stream contaminant on the ability of the IL to absorb simultaneously CO2 is demonstrated using novel measurement techniques, including a mass spectrometry breakthrough method and in situ infrared spectroscopy. The findings show that the presence of an industrially relevant concentration of NO2 in a combined feed with CO2 has the effect of reducing the capacity of the IL to absorb CO2 efficiently by ∼60% after 10 absorption-desorption cycles. This finding is supported by physical property analysis (viscosity, 1H and 13C NMR, and X-ray photoelectron spectroscopy) and spectroscopic infrared characterization, in addition to density functional theory (DFT) calculations, to determine the structure of the IL-NO2 complex. The results are presented in comparison with another flue gas component, NO, demonstrating that the absorption of NO2 is more favorable, thereby hindering the ability of the IL to absorb CO2. Significantly, this work aids understanding of the effects that individual components of flue gas have on CO2 capture sorbents, through studying a contaminant that has received limited interest previously.

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    ACS Sustainable Chemistry & Engineering
    Article . 2021 . Peer-reviewed
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    Other literature type . 2021
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    Article . 2021
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    Article . 2021
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    The University of Manchester - Institutional Repository
    Article . 2021
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    ACS Sustainable Chemistry & Engineering
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      ACS Sustainable Chemistry & Engineering
      Article . 2021 . Peer-reviewed
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  • Combined Experimental and Theoretical Study of the Competitive Absorption of CO2 and NO2 by a Superbase Ionic Liquid

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Journal 2021 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | The UK Catalysis Hub - 'S..., UKRI | Biocatalysis & Biotra..., UKRI | Utilisation of Solar Ener...
    Authors: C. Richard A. Catlow; Johan Jacquemin; Matthew G. Quesne; Matthew G. Quesne; +6 Authors

    doi: 10.1021/acssuschemeng.1c01451

    pmid: 34306836

    pmc: PMC8296676

    A superbase ionic liquid (IL), trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is investigated for the capture of CO2 in the presence of NO2 impurities. The effect of the waste gas stream contaminant on the ability of the IL to absorb simultaneously CO2 is demonstrated using novel measurement techniques, including a mass spectrometry breakthrough method and in situ infrared spectroscopy. The findings show that the presence of an industrially relevant concentration of NO2 in a combined feed with CO2 has the effect of reducing the capacity of the IL to absorb CO2 efficiently by ∼60% after 10 absorption-desorption cycles. This finding is supported by physical property analysis (viscosity, 1H and 13C NMR, and X-ray photoelectron spectroscopy) and spectroscopic infrared characterization, in addition to density functional theory (DFT) calculations, to determine the structure of the IL-NO2 complex. The results are presented in comparison with another flue gas component, NO, demonstrating that the absorption of NO2 is more favorable, thereby hindering the ability of the IL to absorb CO2. Significantly, this work aids understanding of the effects that individual components of flue gas have on CO2 capture sorbents, through studying a contaminant that has received limited interest previously.

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    The University of Manchester - Institutional Repository
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  • Arc Synthesis, Crystal Structure, and Photoelectrochemistry of Copper(I) Tungstate

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Journal 2021 Netherlands, United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener..., NWO | Earth-abundant materials ...
    Authors: Miguel T. Galante; S. F. Rebecca Taylor; Adam J. Greer; Aleksandar Živković; +11 Authors

    doi: 10.1021/acsami.1c03928

    pmid: 34251184

    pmc: PMC8311641

    A little-studied p-type ternary oxide semiconductor, copper(I) tungstate (Cu2WO4), was assessed by a combined theoretical/experimental approach. A detailed computational study was performed to solve the long-standing debate on the space group of Cu2WO4, which was determined to be triclinic P1. Cu2WO4 was synthesized by a time-efficient, arc-melting method, and the crystalline reddish particulate product showed broad-band absorption in the UV-visible spectral region, thermal stability up to ∼260 °C, and cathodic photoelectrochemical activity. Controlled thermal oxidation of copper from the Cu(I) to Cu(II) oxidation state showed that the crystal lattice could accommodate Cu2+ cations up to ∼260 °C, beyond which the compound was converted to CuO and CuWO4. This process was monitored by powder X-ray diffraction and X-ray photoelectron spectroscopy. The electronic band structure of Cu2WO4 was contrasted with that of the Cu(II) counterpart, CuWO4 using spin-polarized density functional theory (DFT). Finally, the compound Cu2WO4 was determined to have a high-lying (negative potential) conduction band edge underlining its promise for driving energetic photoredox reactions.

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  • Arc Synthesis, Crystal Structure, and Photoelectrochemistry of Copper(I) Tungstate

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Journal 2021 Netherlands, United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener..., NWO | Earth-abundant materials ...
    Authors: Miguel T. Galante; S. F. Rebecca Taylor; Adam J. Greer; Aleksandar Živković; +11 Authors

    doi: 10.1021/acsami.1c03928

    pmid: 34251184

    pmc: PMC8311641

    A little-studied p-type ternary oxide semiconductor, copper(I) tungstate (Cu2WO4), was assessed by a combined theoretical/experimental approach. A detailed computational study was performed to solve the long-standing debate on the space group of Cu2WO4, which was determined to be triclinic P1. Cu2WO4 was synthesized by a time-efficient, arc-melting method, and the crystalline reddish particulate product showed broad-band absorption in the UV-visible spectral region, thermal stability up to ∼260 °C, and cathodic photoelectrochemical activity. Controlled thermal oxidation of copper from the Cu(I) to Cu(II) oxidation state showed that the crystal lattice could accommodate Cu2+ cations up to ∼260 °C, beyond which the compound was converted to CuO and CuWO4. This process was monitored by powder X-ray diffraction and X-ray photoelectron spectroscopy. The electronic band structure of Cu2WO4 was contrasted with that of the Cu(II) counterpart, CuWO4 using spin-polarized density functional theory (DFT). Finally, the compound Cu2WO4 was determined to have a high-lying (negative potential) conduction band edge underlining its promise for driving energetic photoredox reactions.

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  • Investigating the Effect of NO on the Capture of CO2 Using Superbase Ionic Liquids for Flue Gas Applications

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2019 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Matthew Quesne; +3 Authors

    doi: 10.1021/acssuschemeng.8b05870

    The effect of acidic gases present in flue gas, specifically NO, on the capture of CO2 by the superbase ionic liquid, trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is reported. An online mass spectrometry technique was utilized to study the CO2 uptake of the ionic liquid during multiple absorption and desorption cycles of a gas feed containing NO and CO2 at realistic flue gas concentrations, and it was found that while NO alone could bind irreversibly, the CO2 capacity of the IL was largely unaffected by the presence of NO in a cofeed of the gases. In situ attenuated total reflection infrared was employed to probe the competitive absorption of CO2 and NO by [P66614][Benzim], in which carbamate and NONOate species were observed to cobind to different sites of the benzimidazolide anion. These effects were further characterized by analyzing changes in physical properties (viscosity and nitrogen content) and other spectroscopic changes (1H NMR, 13C NMR and XPS). Density functional theory c...

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  • Investigating the Effect of NO on the Capture of CO2 Using Superbase Ionic Liquids for Flue Gas Applications

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2019 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Matthew Quesne; +3 Authors

    doi: 10.1021/acssuschemeng.8b05870

    The effect of acidic gases present in flue gas, specifically NO, on the capture of CO2 by the superbase ionic liquid, trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is reported. An online mass spectrometry technique was utilized to study the CO2 uptake of the ionic liquid during multiple absorption and desorption cycles of a gas feed containing NO and CO2 at realistic flue gas concentrations, and it was found that while NO alone could bind irreversibly, the CO2 capacity of the IL was largely unaffected by the presence of NO in a cofeed of the gases. In situ attenuated total reflection infrared was employed to probe the competitive absorption of CO2 and NO by [P66614][Benzim], in which carbamate and NONOate species were observed to cobind to different sites of the benzimidazolide anion. These effects were further characterized by analyzing changes in physical properties (viscosity and nitrogen content) and other spectroscopic changes (1H NMR, 13C NMR and XPS). Density functional theory c...

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  • Combined Superbase Ionic Liquid Approach to Separate CO2 from Flue Gas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Johan Jacquemin; +1 Authors

    doi: 10.1021/acssuschemeng.2c01848

    pmid: 35910293

    pmc: PMC9326967

    Superbase ionic liquids (ILs) with a trihexyltetradecylphosphonium cation and a benzimidazolide ([P66614][Benzim]) or tetrazolide ([P66614][Tetz]) anion were investigated in a dual-IL system allowing the selective capture and separation of CO2 and SO2, respectively, under realistic gas concentrations. The results show that [P66614][Tetz] is capable of efficiently capturing SO2 in preference to CO2 and thus, in a stepwise separation process, protects [P66614][Benzim] from the negative effects of the highly acidic contaminant. This results in [P66614][Benzim] maintaining >53% of its original CO2 uptake capacity after 30 absorption/desorption cycles in comparison to the 89% decrease observed after 11 cycles when [P66614][Tetz] was not present. Characterization of the ILs post exposure revealed that small amounts of SO2 were irreversibly absorbed to the [Benzim]- anion responsible for the decrease in CO2 capacity. While optimization of this dual-IL system is required, this feasibility study demonstrates that [P66614][Tetz] is a suitable sorbent for reversibly capturing SO2 and significantly extending the lifetime of [P66614][Benzim] for CO2 uptake.

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  • Combined Superbase Ionic Liquid Approach to Separate CO2 from Flue Gas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Johan Jacquemin; +1 Authors

    doi: 10.1021/acssuschemeng.2c01848

    pmid: 35910293

    pmc: PMC9326967

    Superbase ionic liquids (ILs) with a trihexyltetradecylphosphonium cation and a benzimidazolide ([P66614][Benzim]) or tetrazolide ([P66614][Tetz]) anion were investigated in a dual-IL system allowing the selective capture and separation of CO2 and SO2, respectively, under realistic gas concentrations. The results show that [P66614][Tetz] is capable of efficiently capturing SO2 in preference to CO2 and thus, in a stepwise separation process, protects [P66614][Benzim] from the negative effects of the highly acidic contaminant. This results in [P66614][Benzim] maintaining >53% of its original CO2 uptake capacity after 30 absorption/desorption cycles in comparison to the 89% decrease observed after 11 cycles when [P66614][Tetz] was not present. Characterization of the ILs post exposure revealed that small amounts of SO2 were irreversibly absorbed to the [Benzim]- anion responsible for the decrease in CO2 capacity. While optimization of this dual-IL system is required, this feasibility study demonstrates that [P66614][Tetz] is a suitable sorbent for reversibly capturing SO2 and significantly extending the lifetime of [P66614][Benzim] for CO2 uptake.

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  • Urbanization and seasonality strengthens the CO2 capacity of the Red River Delta, Vietnam

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 Netherlands, United Kingdom, United Kingdom Publisher:IOP PublishingFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Jorge Salgado; Duc Anh Trinh; Do Thu Nga; Virginia N. Panizzo; +7 Authors

    doi: 10.1088/1748-9326/ac9705 , 10.60692/ncsm6-s8622 , 10.60692/ygbqs-epf58

    handle: 20.500.11755/2a2e7fb9-f9e9-40f0-bcd0-983dcb51cedb

    Abstract Tropical rivers are dynamic CO2 sources. Regional patterns in the partial pressure of CO2 (pCO2) and relationships with other a/biotic factors in densely populated and rapidly developing river delta regions of Southeast Asia are still poorly constrained. Over one year, at 21 sites across the river system in the Red River Delta (RRD), Vietnam, we calculated pCO2 levels from temperature, pH, and total alkalinity and inter-linkages between pCO2 and phytoplankton, water chemistry and seasonality were then assessed. The smaller, more urbanized, and polluted Day River had an annual median pCO2 of 5000 ± 3300 µatm and the larger Red River of 2675 ± 2271 µatm. pCO2 was 1.6 and 3.2 times higher during the dry season in the Day and Red rivers respectively than the rainy season. Elevated pCO2 levels in the Day River during the dry season were also 2.4-fold higher than the median value (2811 ± 3577 µatm) of calculated and direct pCO2 measurements in >20 sub/tropical rivers. By further categorizing the river data into Hanoi City vs. other less urban-populated provinces, we found significantly higher nutrients, organic matter content, and riverine cyanobacteria during the dry season in the Day River across Hanoi City. Forward selection also identified riverine cyanobacteria and river discharge as the main predictors explaining pCO2 variation in the RRD. After accounting for the shared effects (14%), river discharge alone significantly explained 12% of the pCO2 variation, cyanobacteria uniquely a further 21%, while 53% of the pCO2 variance was unexplained by either. We show that the urbanization of rivers deltas could result in increased sources of riverine pCO2, water pollution, and harmful cyanobacterial blooms. Such risks could be mitigated through water management to increase water flows in problem areas during the dry season.

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    NERC Open Research Archive
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    Environmental Research Letters
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    Article . 2022
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    Article . 2022
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    https://dx.doi.org/10.60692/nc...
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      NERC Open Research Archive
      2022 . Peer-reviewed
      Full-Text: https://nora.nerc.ac.uk/id/eprint/533366/1/Salgado_2022_Environ._Res._Lett._17_104052.pdf
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      Article . 2022
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      Article . 2022 . Peer-reviewed
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      UCL Discovery
      Article . 2022
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      https://dx.doi.org/10.60692/nc...
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  • Urbanization and seasonality strengthens the CO2 capacity of the Red River Delta, Vietnam

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 Netherlands, United Kingdom, United Kingdom Publisher:IOP PublishingFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Jorge Salgado; Duc Anh Trinh; Do Thu Nga; Virginia N. Panizzo; +7 Authors

    doi: 10.1088/1748-9326/ac9705 , 10.60692/ncsm6-s8622 , 10.60692/ygbqs-epf58

    handle: 20.500.11755/2a2e7fb9-f9e9-40f0-bcd0-983dcb51cedb

    Abstract Tropical rivers are dynamic CO2 sources. Regional patterns in the partial pressure of CO2 (pCO2) and relationships with other a/biotic factors in densely populated and rapidly developing river delta regions of Southeast Asia are still poorly constrained. Over one year, at 21 sites across the river system in the Red River Delta (RRD), Vietnam, we calculated pCO2 levels from temperature, pH, and total alkalinity and inter-linkages between pCO2 and phytoplankton, water chemistry and seasonality were then assessed. The smaller, more urbanized, and polluted Day River had an annual median pCO2 of 5000 ± 3300 µatm and the larger Red River of 2675 ± 2271 µatm. pCO2 was 1.6 and 3.2 times higher during the dry season in the Day and Red rivers respectively than the rainy season. Elevated pCO2 levels in the Day River during the dry season were also 2.4-fold higher than the median value (2811 ± 3577 µatm) of calculated and direct pCO2 measurements in >20 sub/tropical rivers. By further categorizing the river data into Hanoi City vs. other less urban-populated provinces, we found significantly higher nutrients, organic matter content, and riverine cyanobacteria during the dry season in the Day River across Hanoi City. Forward selection also identified riverine cyanobacteria and river discharge as the main predictors explaining pCO2 variation in the RRD. After accounting for the shared effects (14%), river discharge alone significantly explained 12% of the pCO2 variation, cyanobacteria uniquely a further 21%, while 53% of the pCO2 variance was unexplained by either. We show that the urbanization of rivers deltas could result in increased sources of riverine pCO2, water pollution, and harmful cyanobacterial blooms. Such risks could be mitigated through water management to increase water flows in problem areas during the dry season.

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    Environmental Research Letters
    Article . 2022 . Peer-reviewed
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    Environmental Research Letters
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  • Effects of heat treatment atmosphere on the structure and activity of Pt3Sn nanoparticle electrocatalysts: a characterisation case study

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    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2018 United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | University of Bristol - E..., UKRI | The UK Catalysis Hub, UKRI | Catalytic Science in the ... +4 projects
    Authors: Vinod Kumar Puthiyapura; Vinod Kumar Puthiyapura; Dan J. L. Brett; Haoliang Huang; +6 Authors

    doi: 10.1039/c7fd00221a

    pmid: 29851419

    handle: 1983/e4e756a4-b0e8-45c7-923b-d4c646a58811

    In this work, a variation in heat treatment atmosphere approach is taken to provide a series of related PtSn catalysts with the same nominal composition of Pt3Sn, but with different surface compositions.

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    e-Prints Soton
    Article . 2018 . Peer-reviewed
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    Article . 2018
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    Full-Text: https://eprints.soton.ac.uk/421733/1/Manuscript_NP_FD_with_template_26_10_2018.pdf
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    Faraday Discussions
    Article . 2018 . Peer-reviewed
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    Explore Bristol Research
    Article . 2018
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    The University of Manchester - Institutional Repository
    Article . 2018
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    University of Bristol: Bristol Research
    Article . 2018
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    Faraday Discussions
    Article . 2019
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      Article . 2018 . Peer-reviewed
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      Article . 2018
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      Faraday Discussions
      Article . 2018 . Peer-reviewed
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      The University of Manchester - Institutional Repository
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  • Effects of heat treatment atmosphere on the structure and activity of Pt3Sn nanoparticle electrocatalysts: a characterisation case study

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    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2018 United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | University of Bristol - E..., UKRI | The UK Catalysis Hub, UKRI | Catalytic Science in the ... +4 projects
    Authors: Vinod Kumar Puthiyapura; Vinod Kumar Puthiyapura; Dan J. L. Brett; Haoliang Huang; +6 Authors

    doi: 10.1039/c7fd00221a

    pmid: 29851419

    handle: 1983/e4e756a4-b0e8-45c7-923b-d4c646a58811

    In this work, a variation in heat treatment atmosphere approach is taken to provide a series of related PtSn catalysts with the same nominal composition of Pt3Sn, but with different surface compositions.

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    The University of Manchester - Institutional Repository
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      The University of Manchester - Institutional Repository
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  • Understanding the Competitive Gas Absorption of CO2 and SO2 in Superbase Ionic Liquids

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2018 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | A Coordinated, Comprehens..., UKRI | Utilisation of Solar Ener...
    Authors: Johan Jacquemin; Johan Jacquemin; Adam J. Greer; Matthew McClung; +4 Authors

    doi: 10.1021/acs.iecr.8b03623

    During this work, an original study of the CO2 and SO2 competitive gas absorption in three superbase ionic liquids (ILs), namely, trihexyltetradecylphosphonium 1,2,4-triazolide ([P66614][124Triz]), and trihexyltetradecylphoshonium benzimidazolide ([P66614][Benzim]), is reported for the first time. To initiate such a comprehensive study, the CO2 and SO2 mixed gas solubility in selected ILs was determined by using an original and accurate dynamic method coupled with mass spectrometry after several absorption and desorption cycles. This method has been validated by comparing the gravimetric uptake of CO2 with the mass spectrometry data using trihexyltetradecylphosphonium benzotriazolide, 1,2,4-triazolide, and benzimidazolide ILs and shown to be consistent within 10% in mole ratio units. Solubility results clearly show that the presence of SO2 in the gas stream decreases the CO2 capture capability of the investigated ILs. Furthermore, the viscosity, chemical analysis (water content and sulfur content), and sp...

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    Article . 2018
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  • Understanding the Competitive Gas Absorption of CO2 and SO2 in Superbase Ionic Liquids

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2018 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | A Coordinated, Comprehens..., UKRI | Utilisation of Solar Ener...
    Authors: Johan Jacquemin; Johan Jacquemin; Adam J. Greer; Matthew McClung; +4 Authors

    doi: 10.1021/acs.iecr.8b03623

    During this work, an original study of the CO2 and SO2 competitive gas absorption in three superbase ionic liquids (ILs), namely, trihexyltetradecylphosphonium 1,2,4-triazolide ([P66614][124Triz]), and trihexyltetradecylphoshonium benzimidazolide ([P66614][Benzim]), is reported for the first time. To initiate such a comprehensive study, the CO2 and SO2 mixed gas solubility in selected ILs was determined by using an original and accurate dynamic method coupled with mass spectrometry after several absorption and desorption cycles. This method has been validated by comparing the gravimetric uptake of CO2 with the mass spectrometry data using trihexyltetradecylphosphonium benzotriazolide, 1,2,4-triazolide, and benzimidazolide ILs and shown to be consistent within 10% in mole ratio units. Solubility results clearly show that the presence of SO2 in the gas stream decreases the CO2 capture capability of the investigated ILs. Furthermore, the viscosity, chemical analysis (water content and sulfur content), and sp...

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    The University of Manchester - Institutional Repository
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      Industrial & Engineering Chemistry Research
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  • Factors affecting bubble size in ionic liquids

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    Authors: William A. Zimmerman; Stuart A. Brittle; Sarah F. R. Taylor; Sarah F. R. Taylor; +5 Authors

    doi: 10.1039/c7cp01725a

    pmid: 28537605

    Bubble behaviour of 11 ionic liquids was studied and the relationship of bubble size, physical properties and structure was examined.

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  • Factors affecting bubble size in ionic liquids

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    descriptionPublicationkeyboard_double_arrow_right Article , Conference object , Journal 2017 France, United Kingdom Publisher:Royal Society of Chemistry (RSC)Funded by:UKRI | Utilisation of Solar Ener..., UKRI | A Coordinated, Comprehens...
    Authors: William A. Zimmerman; Stuart A. Brittle; Sarah F. R. Taylor; Sarah F. R. Taylor; +5 Authors

    doi: 10.1039/c7cp01725a

    pmid: 28537605

    Bubble behaviour of 11 ionic liquids was studied and the relationship of bubble size, physical properties and structure was examined.

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  • How to go beyond C1 products with electrochemical reduction of CO2

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    Authors: Jean-Marie Fontmorin; Jean-Marie Fontmorin; Hang Xiang; Liam Banerji; +14 Authors

    doi: 10.1039/d1se00861g

    This review summaries recent development across electro-, photoelectro- and bioelectro-catalyst developments for multi-carbon products from CO2. It also explores the role of device design and operating conditions in enabling C–C bond generation.

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  • How to go beyond C1 products with electrochemical reduction of CO2

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    Authors: Jean-Marie Fontmorin; Jean-Marie Fontmorin; Hang Xiang; Liam Banerji; +14 Authors

    doi: 10.1039/d1se00861g

    This review summaries recent development across electro-, photoelectro- and bioelectro-catalyst developments for multi-carbon products from CO2. It also explores the role of device design and operating conditions in enabling C–C bond generation.

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  • Using lake sediments to assess the long-term impacts of anthropogenic activity in tropical river deltas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Review 2023 United Kingdom, Netherlands, United Kingdom, United Kingdom Publisher:SAGE PublicationsFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Richard E. Walton; Heather Moorhouse; Lucy R. Roberts; Jorge Salgado; +9 Authors

    doi: 10.1177/20530196231204334 , 10.60692/h7teh-1b055 , 10.60692/hq28v-61t17

    pmid: 39156121

    pmc: PMC11324390

    handle: 20.500.11755/e7bb944e-73af-4112-a5e8-ff134b2ea612

    Tropical river deltas, and the social-ecological systems they sustain, are changing rapidly due to anthropogenic activity and climatic change. Baseline data to inform sustainable management options for resilient deltas is urgently needed and palaeolimnology (reconstructing past conditions from lake or wetland deposits) can provide crucial long-term perspectives needed to identify drivers and rates of change. We review how palaeolimnology can be a valuable tool for resource managers using three current issues facing tropical delta regions: hydrology and sediment supply, salinisation and nutrient pollution. The unique ability of palaeolimnological methods to untangle multiple stressors is also discussed. We demonstrate how palaeolimnology has been used to understand each of these issues, in other aquatic environments, to be incorporated into policy. Palaeolimnology is a key tool to understanding how anthropogenic influences interact with other environmental stressors, providing policymakers and resource managers with a ‘big picture’ view and possible holistic solutions that can be implemented.

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    Full-Text: https://eprints.ncl.ac.uk/294122
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    Review . 2023
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    The Anthropocene Review
    Article . 2023 . Peer-reviewed
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    Other literature type . 2023
    License: http://creativecommons.org/licenses/by/4.0/This article is distributed under the terms of the Creative Commons Attribution 4.0 License (http://creativecommons.org/licenses/by/4.0/) which permits any use, reproduction and distribution of the work without further permission provided the original work is attributed as specified on the SAGE and Open Access pages (http://us.sagepub.com/en-us/nam/open-access-at-sage).
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    PURE Aarhus University
    Article . 2024
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  • Using lake sediments to assess the long-term impacts of anthropogenic activity in tropical river deltas

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Review 2023 United Kingdom, Netherlands, United Kingdom, United Kingdom Publisher:SAGE PublicationsFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Richard E. Walton; Heather Moorhouse; Lucy R. Roberts; Jorge Salgado; +9 Authors

    doi: 10.1177/20530196231204334 , 10.60692/h7teh-1b055 , 10.60692/hq28v-61t17

    pmid: 39156121

    pmc: PMC11324390

    handle: 20.500.11755/e7bb944e-73af-4112-a5e8-ff134b2ea612

    Tropical river deltas, and the social-ecological systems they sustain, are changing rapidly due to anthropogenic activity and climatic change. Baseline data to inform sustainable management options for resilient deltas is urgently needed and palaeolimnology (reconstructing past conditions from lake or wetland deposits) can provide crucial long-term perspectives needed to identify drivers and rates of change. We review how palaeolimnology can be a valuable tool for resource managers using three current issues facing tropical delta regions: hydrology and sediment supply, salinisation and nutrient pollution. The unique ability of palaeolimnological methods to untangle multiple stressors is also discussed. We demonstrate how palaeolimnology has been used to understand each of these issues, in other aquatic environments, to be incorporated into policy. Palaeolimnology is a key tool to understanding how anthropogenic influences interact with other environmental stressors, providing policymakers and resource managers with a ‘big picture’ view and possible holistic solutions that can be implemented.

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  • Combined Experimental and Theoretical Study of the Competitive Absorption of CO2 and NO2 by a Superbase Ionic Liquid

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    Authors: C. Richard A. Catlow; Johan Jacquemin; Matthew G. Quesne; Matthew G. Quesne; +6 Authors

    doi: 10.1021/acssuschemeng.1c01451

    pmid: 34306836

    pmc: PMC8296676

    A superbase ionic liquid (IL), trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is investigated for the capture of CO2 in the presence of NO2 impurities. The effect of the waste gas stream contaminant on the ability of the IL to absorb simultaneously CO2 is demonstrated using novel measurement techniques, including a mass spectrometry breakthrough method and in situ infrared spectroscopy. The findings show that the presence of an industrially relevant concentration of NO2 in a combined feed with CO2 has the effect of reducing the capacity of the IL to absorb CO2 efficiently by ∼60% after 10 absorption-desorption cycles. This finding is supported by physical property analysis (viscosity, 1H and 13C NMR, and X-ray photoelectron spectroscopy) and spectroscopic infrared characterization, in addition to density functional theory (DFT) calculations, to determine the structure of the IL-NO2 complex. The results are presented in comparison with another flue gas component, NO, demonstrating that the absorption of NO2 is more favorable, thereby hindering the ability of the IL to absorb CO2. Significantly, this work aids understanding of the effects that individual components of flue gas have on CO2 capture sorbents, through studying a contaminant that has received limited interest previously.

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  • Combined Experimental and Theoretical Study of the Competitive Absorption of CO2 and NO2 by a Superbase Ionic Liquid

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Journal 2021 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | The UK Catalysis Hub - 'S..., UKRI | Biocatalysis & Biotra..., UKRI | Utilisation of Solar Ener...
    Authors: C. Richard A. Catlow; Johan Jacquemin; Matthew G. Quesne; Matthew G. Quesne; +6 Authors

    doi: 10.1021/acssuschemeng.1c01451

    pmid: 34306836

    pmc: PMC8296676

    A superbase ionic liquid (IL), trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is investigated for the capture of CO2 in the presence of NO2 impurities. The effect of the waste gas stream contaminant on the ability of the IL to absorb simultaneously CO2 is demonstrated using novel measurement techniques, including a mass spectrometry breakthrough method and in situ infrared spectroscopy. The findings show that the presence of an industrially relevant concentration of NO2 in a combined feed with CO2 has the effect of reducing the capacity of the IL to absorb CO2 efficiently by ∼60% after 10 absorption-desorption cycles. This finding is supported by physical property analysis (viscosity, 1H and 13C NMR, and X-ray photoelectron spectroscopy) and spectroscopic infrared characterization, in addition to density functional theory (DFT) calculations, to determine the structure of the IL-NO2 complex. The results are presented in comparison with another flue gas component, NO, demonstrating that the absorption of NO2 is more favorable, thereby hindering the ability of the IL to absorb CO2. Significantly, this work aids understanding of the effects that individual components of flue gas have on CO2 capture sorbents, through studying a contaminant that has received limited interest previously.

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  • Arc Synthesis, Crystal Structure, and Photoelectrochemistry of Copper(I) Tungstate

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    Authors: Miguel T. Galante; S. F. Rebecca Taylor; Adam J. Greer; Aleksandar Živković; +11 Authors

    doi: 10.1021/acsami.1c03928

    pmid: 34251184

    pmc: PMC8311641

    A little-studied p-type ternary oxide semiconductor, copper(I) tungstate (Cu2WO4), was assessed by a combined theoretical/experimental approach. A detailed computational study was performed to solve the long-standing debate on the space group of Cu2WO4, which was determined to be triclinic P1. Cu2WO4 was synthesized by a time-efficient, arc-melting method, and the crystalline reddish particulate product showed broad-band absorption in the UV-visible spectral region, thermal stability up to ∼260 °C, and cathodic photoelectrochemical activity. Controlled thermal oxidation of copper from the Cu(I) to Cu(II) oxidation state showed that the crystal lattice could accommodate Cu2+ cations up to ∼260 °C, beyond which the compound was converted to CuO and CuWO4. This process was monitored by powder X-ray diffraction and X-ray photoelectron spectroscopy. The electronic band structure of Cu2WO4 was contrasted with that of the Cu(II) counterpart, CuWO4 using spin-polarized density functional theory (DFT). Finally, the compound Cu2WO4 was determined to have a high-lying (negative potential) conduction band edge underlining its promise for driving energetic photoredox reactions.

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  • Arc Synthesis, Crystal Structure, and Photoelectrochemistry of Copper(I) Tungstate

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Journal 2021 Netherlands, United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener..., NWO | Earth-abundant materials ...
    Authors: Miguel T. Galante; S. F. Rebecca Taylor; Adam J. Greer; Aleksandar Živković; +11 Authors

    doi: 10.1021/acsami.1c03928

    pmid: 34251184

    pmc: PMC8311641

    A little-studied p-type ternary oxide semiconductor, copper(I) tungstate (Cu2WO4), was assessed by a combined theoretical/experimental approach. A detailed computational study was performed to solve the long-standing debate on the space group of Cu2WO4, which was determined to be triclinic P1. Cu2WO4 was synthesized by a time-efficient, arc-melting method, and the crystalline reddish particulate product showed broad-band absorption in the UV-visible spectral region, thermal stability up to ∼260 °C, and cathodic photoelectrochemical activity. Controlled thermal oxidation of copper from the Cu(I) to Cu(II) oxidation state showed that the crystal lattice could accommodate Cu2+ cations up to ∼260 °C, beyond which the compound was converted to CuO and CuWO4. This process was monitored by powder X-ray diffraction and X-ray photoelectron spectroscopy. The electronic band structure of Cu2WO4 was contrasted with that of the Cu(II) counterpart, CuWO4 using spin-polarized density functional theory (DFT). Finally, the compound Cu2WO4 was determined to have a high-lying (negative potential) conduction band edge underlining its promise for driving energetic photoredox reactions.

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  • Investigating the Effect of NO on the Capture of CO2 Using Superbase Ionic Liquids for Flue Gas Applications

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2019 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Matthew Quesne; +3 Authors

    doi: 10.1021/acssuschemeng.8b05870

    The effect of acidic gases present in flue gas, specifically NO, on the capture of CO2 by the superbase ionic liquid, trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is reported. An online mass spectrometry technique was utilized to study the CO2 uptake of the ionic liquid during multiple absorption and desorption cycles of a gas feed containing NO and CO2 at realistic flue gas concentrations, and it was found that while NO alone could bind irreversibly, the CO2 capacity of the IL was largely unaffected by the presence of NO in a cofeed of the gases. In situ attenuated total reflection infrared was employed to probe the competitive absorption of CO2 and NO by [P66614][Benzim], in which carbamate and NONOate species were observed to cobind to different sites of the benzimidazolide anion. These effects were further characterized by analyzing changes in physical properties (viscosity and nitrogen content) and other spectroscopic changes (1H NMR, 13C NMR and XPS). Density functional theory c...

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  • Investigating the Effect of NO on the Capture of CO2 Using Superbase Ionic Liquids for Flue Gas Applications

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    descriptionPublicationkeyboard_double_arrow_right Article , Journal 2019 United Kingdom, France Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Matthew Quesne; +3 Authors

    doi: 10.1021/acssuschemeng.8b05870

    The effect of acidic gases present in flue gas, specifically NO, on the capture of CO2 by the superbase ionic liquid, trihexyltetradecylphosphonium benzimidazolide ([P66614][Benzim]), is reported. An online mass spectrometry technique was utilized to study the CO2 uptake of the ionic liquid during multiple absorption and desorption cycles of a gas feed containing NO and CO2 at realistic flue gas concentrations, and it was found that while NO alone could bind irreversibly, the CO2 capacity of the IL was largely unaffected by the presence of NO in a cofeed of the gases. In situ attenuated total reflection infrared was employed to probe the competitive absorption of CO2 and NO by [P66614][Benzim], in which carbamate and NONOate species were observed to cobind to different sites of the benzimidazolide anion. These effects were further characterized by analyzing changes in physical properties (viscosity and nitrogen content) and other spectroscopic changes (1H NMR, 13C NMR and XPS). Density functional theory c...

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  • Combined Superbase Ionic Liquid Approach to Separate CO2 from Flue Gas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Johan Jacquemin; +1 Authors

    doi: 10.1021/acssuschemeng.2c01848

    pmid: 35910293

    pmc: PMC9326967

    Superbase ionic liquids (ILs) with a trihexyltetradecylphosphonium cation and a benzimidazolide ([P66614][Benzim]) or tetrazolide ([P66614][Tetz]) anion were investigated in a dual-IL system allowing the selective capture and separation of CO2 and SO2, respectively, under realistic gas concentrations. The results show that [P66614][Tetz] is capable of efficiently capturing SO2 in preference to CO2 and thus, in a stepwise separation process, protects [P66614][Benzim] from the negative effects of the highly acidic contaminant. This results in [P66614][Benzim] maintaining >53% of its original CO2 uptake capacity after 30 absorption/desorption cycles in comparison to the 89% decrease observed after 11 cycles when [P66614][Tetz] was not present. Characterization of the ILs post exposure revealed that small amounts of SO2 were irreversibly absorbed to the [Benzim]- anion responsible for the decrease in CO2 capacity. While optimization of this dual-IL system is required, this feasibility study demonstrates that [P66614][Tetz] is a suitable sorbent for reversibly capturing SO2 and significantly extending the lifetime of [P66614][Benzim] for CO2 uptake.

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  • Combined Superbase Ionic Liquid Approach to Separate CO2 from Flue Gas

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 United Kingdom Publisher:American Chemical Society (ACS)Funded by:UKRI | Utilisation of Solar Ener...
    Authors: Adam J. Greer; S. F. Rebecca Taylor; Helen Daly; Johan Jacquemin; +1 Authors

    doi: 10.1021/acssuschemeng.2c01848

    pmid: 35910293

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    Superbase ionic liquids (ILs) with a trihexyltetradecylphosphonium cation and a benzimidazolide ([P66614][Benzim]) or tetrazolide ([P66614][Tetz]) anion were investigated in a dual-IL system allowing the selective capture and separation of CO2 and SO2, respectively, under realistic gas concentrations. The results show that [P66614][Tetz] is capable of efficiently capturing SO2 in preference to CO2 and thus, in a stepwise separation process, protects [P66614][Benzim] from the negative effects of the highly acidic contaminant. This results in [P66614][Benzim] maintaining >53% of its original CO2 uptake capacity after 30 absorption/desorption cycles in comparison to the 89% decrease observed after 11 cycles when [P66614][Tetz] was not present. Characterization of the ILs post exposure revealed that small amounts of SO2 were irreversibly absorbed to the [Benzim]- anion responsible for the decrease in CO2 capacity. While optimization of this dual-IL system is required, this feasibility study demonstrates that [P66614][Tetz] is a suitable sorbent for reversibly capturing SO2 and significantly extending the lifetime of [P66614][Benzim] for CO2 uptake.

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  • Urbanization and seasonality strengthens the CO2 capacity of the Red River Delta, Vietnam

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 Netherlands, United Kingdom, United Kingdom Publisher:IOP PublishingFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Jorge Salgado; Duc Anh Trinh; Do Thu Nga; Virginia N. Panizzo; +7 Authors

    doi: 10.1088/1748-9326/ac9705 , 10.60692/ncsm6-s8622 , 10.60692/ygbqs-epf58

    handle: 20.500.11755/2a2e7fb9-f9e9-40f0-bcd0-983dcb51cedb

    Abstract Tropical rivers are dynamic CO2 sources. Regional patterns in the partial pressure of CO2 (pCO2) and relationships with other a/biotic factors in densely populated and rapidly developing river delta regions of Southeast Asia are still poorly constrained. Over one year, at 21 sites across the river system in the Red River Delta (RRD), Vietnam, we calculated pCO2 levels from temperature, pH, and total alkalinity and inter-linkages between pCO2 and phytoplankton, water chemistry and seasonality were then assessed. The smaller, more urbanized, and polluted Day River had an annual median pCO2 of 5000 ± 3300 µatm and the larger Red River of 2675 ± 2271 µatm. pCO2 was 1.6 and 3.2 times higher during the dry season in the Day and Red rivers respectively than the rainy season. Elevated pCO2 levels in the Day River during the dry season were also 2.4-fold higher than the median value (2811 ± 3577 µatm) of calculated and direct pCO2 measurements in >20 sub/tropical rivers. By further categorizing the river data into Hanoi City vs. other less urban-populated provinces, we found significantly higher nutrients, organic matter content, and riverine cyanobacteria during the dry season in the Day River across Hanoi City. Forward selection also identified riverine cyanobacteria and river discharge as the main predictors explaining pCO2 variation in the RRD. After accounting for the shared effects (14%), river discharge alone significantly explained 12% of the pCO2 variation, cyanobacteria uniquely a further 21%, while 53% of the pCO2 variance was unexplained by either. We show that the urbanization of rivers deltas could result in increased sources of riverine pCO2, water pollution, and harmful cyanobacterial blooms. Such risks could be mitigated through water management to increase water flows in problem areas during the dry season.

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  • Urbanization and seasonality strengthens the CO2 capacity of the Red River Delta, Vietnam

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    descriptionPublicationkeyboard_double_arrow_right Article , Other literature type 2022 Netherlands, United Kingdom, United Kingdom Publisher:IOP PublishingFunded by:UKRI | GCRF Living Deltas Hub
    Authors: Jorge Salgado; Duc Anh Trinh; Do Thu Nga; Virginia N. Panizzo; +7 Authors

    doi: 10.1088/1748-9326/ac9705 , 10.60692/ncsm6-s8622 , 10.60692/ygbqs-epf58

    handle: 20.500.11755/2a2e7fb9-f9e9-40f0-bcd0-983dcb51cedb

    Abstract Tropical rivers are dynamic CO2 sources. Regional patterns in the partial pressure of CO2 (pCO2) and relationships with other a/biotic factors in densely populated and rapidly developing river delta regions of Southeast Asia are still poorly constrained. Over one year, at 21 sites across the river system in the Red River Delta (RRD), Vietnam, we calculated pCO2 levels from temperature, pH, and total alkalinity and inter-linkages between pCO2 and phytoplankton, water chemistry and seasonality were then assessed. The smaller, more urbanized, and polluted Day River had an annual median pCO2 of 5000 ± 3300 µatm and the larger Red River of 2675 ± 2271 µatm. pCO2 was 1.6 and 3.2 times higher during the dry season in the Day and Red rivers respectively than the rainy season. Elevated pCO2 levels in the Day River during the dry season were also 2.4-fold higher than the median value (2811 ± 3577 µatm) of calculated and direct pCO2 measurements in >20 sub/tropical rivers. By further categorizing the river data into Hanoi City vs. other less urban-populated provinces, we found significantly higher nutrients, organic matter content, and riverine cyanobacteria during the dry season in the Day River across Hanoi City. Forward selection also identified riverine cyanobacteria and river discharge as the main predictors explaining pCO2 variation in the RRD. After accounting for the shared effects (14%), river discharge alone significantly explained 12% of the pCO2 variation, cyanobacteria uniquely a further 21%, while 53% of the pCO2 variance was unexplained by either. We show that the urbanization of rivers deltas could result in increased sources of riverine pCO2, water pollution, and harmful cyanobacterial blooms. Such risks could be mitigated through water management to increase water flows in problem areas during the dry season.

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