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Response of aquatic organisms to eutrophication have been well reported, while less studies are available for the recovery of eutrophic lakes following a reduction in the external loading, especially for systems where nitrogen is reduced but the phosphorus concentration is maintained high due to internal loading. Diatoms are nitrate (NO3-N) opportunists but can also use ammonium (NH4-N). They may, therefore, be more sensitive to nitrogen reduction than other algae that typically prefer NH4-N. We document the variations of nutrients and diatoms in subtropical, eutrophic Lake Taihu over 28 yr during which a reduction of the external loading resulted from lake management. According to the results of change point analysis, data on environmental variables were divided into two periods (P1: 1992-2006; P2: 2007-2019) with two different seasons (WS: Winter-Spring; SA: Summer-Autumn), respectively. Compared with P1-WS, the concentration of NH4-N decreased significantly whereas NO3-N showed no significant change in P2-WS. In contrast, NH4-N concentrations were low and showed no significant changes in P1-SA and P2-SA and NO3-N decreased significantly in the latter period. Accordingly, NO3-N: NH4-N mass ratios in P1-SA and P2-WS were all significantly higher than those in P2-SA and P1-WS, respectively. The biomass of WS diatom increased significantly and the timing of the peak biomass shifted from P1-SA to P2-WS since 2007. The SEM analysis showed that NO3-N was retained as a statistically significant predictor for diatom biomass in P1-SA and significant effects of windspeed, zooplankton and NH4-N on diatom biomass in P2-WS. Windspeed and zooplankton have further changed the biomass of diatoms in the case of declining inorganic nitrogen. We conclude that the magnitude of vernal suppression or stimulation of diatom assemblages has increased, concomitant with the variations of NH4-N and NO3-N: NH4-N mass ratios. Diatoms response to NH4-N or NO3-N is apparently changing in response to water temperature in this eutrophic shallow lake. Thus, parallel reductions in external nitrogen loading, along with variations in dominant inorganic nitrogen, will stimulate the growth of diatom and therefore increase the total biomass of phytoplankton in still high internal phosphorus loading, which is should be regarded as a good sign of restoration measures.

Robust mitigation options will play significant role in achieving the target of limiting global change to below 1.5 °C above pre-industrial levels by 2100. To support cooperation for mitigation development, we establish a real options-based model to evaluate the rational decisions of exercising the abandon option for carbon capture and storage-enhanced oil recovery (CCS-EOR) projects under oil market and geological uncertainties. Three possible cooperative mechanisms (fixed carbon dioxide (CO2) price, oil-indexed CO2 price, and joint venture contracts) among CO2-EOR stakeholders are evaluated. The results show that the conflicts in profit maximization targets for different stakeholders in cooperative mitigation are to a great extent unable to be avoided. A joint venture business model is preferred in cooperative mitigation as it can effectively weaken such conflicts. And it is more reasonable to provide incentives to the downstream of the CO2-EOR chain than compensating the adoption cost of carbon capture technologies in the upstream. From a global perspective, the inefficient cooperation can be a main barrier that hinders the development of deep-cutting options. Global mitigation strategies should not only focus on promoting technology progress but also the design of innovative business models to balance the benefits among stakeholders. A joint venture business model is recommended in both the developed and developing countries for seizing the early mitigation opportunities.

The influence of elemental sulfur (S(0)) amendment on methylmercury (MeHg) accumulation in rice and the chemical form of Hg in the rhizosphere were investigated under waterlogged conditions in Hg-contaminated soil (the majority of the Hg (˜70%) in forms similar to HgS). Different levels of S(0) addition increased the MeHg accumulation in rice. After a sequential extraction analysis of the chemical forms of Hg in the rhizosphere, the results showed that S(0) addition increased the organic bound Hg and decreased the residual Hg in the soils. An Hg LIII XANES further showed that S(0) addition increased the proportion of Hg in the form of RS-Hg-SR and decreased the proportion of Hg in the form of HgS, indicating that S(0) input may reactivate the non-bioavailable Hg in the rhizosphere and improve the net Hg methylation. These findings suggest that the application of S fertilizers to Hg-contaminated paddy soils may increase the MeHg concentration in the edible parts of crops, which may lead to more potential health problems in humans depending on the crop type. However, our study also suggests that S(0) addition could be an effective measure for mobilizing the insoluble Hg and accelerating the phytoremediation process in Hg-contaminated paddy soils.

Abstract Algae have been considered as a promising biodiesel feedstock. One of the major factors affecting large-scale algae technology application is poor wintering cultivation performance. In this study, an integrated approach is investigated combining freshwater microalgae Chlorella zofingiensis wintering cultivation in pilot-scale photobioreactors with artificial wastewater treatment. Mixotrophic culture with the addition of acetic acid (pH-regulation group) and autotrophic culture (control group) were designed, and the characteristics of algal growth, lipid and biodiesel production, and nitrogen and phosphate removal were examined. The results showed that, by using acetic acid three times per day to regulate pH at between 6.8 and 7.2, the total nitrogen (TN) and total phosphate (TP) removal could be increased from 45.2% to 73.5% and from 92.2% to 100%, respectively. Higher biomass productivity of 66.94 mg L−1 day−1 with specific growth rate of 0.260 day−1 was achieved in the pH-regulation group. The lipid content was much higher when using acetic acid to regulate pH, and the relative lipid productivity reached 37.48 mg L−1 day−1. The biodiesel yield in the pH-regulated group was 19.44% of dry weight, with 16–18 carbons as the most abundant composition for fatty acid methyl esters. The findings of the study prove that pH adjustment using acetic acid is efficient in cultivating C. zofingiensis in wastewater in winter for biodiesel production and nutrient reduction.

Low carbon transformation plays an important role in promoting the energy production and consumption revolution. Currently, the power sector of China still faces a series of challenges, such as the overcapacity of coal-fired power, the renewable energy consumption, the new constraints of carbon-emissions, and fragmented power planning. This study develops a multi-objective optimization model to predict the future trend of China power structure by 2035. The key factors such as network, power, load and storage are taken into account. Besides, the technical feasibility, economic rationality and social acceptable constraints are also fully considered. Through planning and optimization, the premise of low carbon transformation is to ensure the continuity of existing policies for removing inefficient assets, and the core is to develop and utilize non-fossil energy on a large scale. Specifically, the capacity of coal-fired power will be attained in the peak in 2025, and the factor will also transfer from main power supplier to main power and energy supplier. Before 2025, the clean replacement of incremental power installation will be completed. In 2035, 92% of new investment comes from non-fossil energy. The economy and competitiveness of wind power and PV (Photovoltaic) power generation are continuously increasing. By 2020, the coal-fired power and the wind power in eastern of China will be parity firstly. In 2025, the cost of PV and wind power will be the same. Furthermore, the evaluation dimension of modern power system with clean, low-carbon, safety and high efficiency are innovatively constructed, and the index system target of 2035 is quantitatively analyzed and prospected.

Carbonaceous aerosols (CAs) scatter and absorb incident solar radiation in the atmosphere, thereby influencing the regional climate and hydrological cycle, particularly in the Third Pole (TP). Here, we present the characteristics of CAs at 19 observation stations from the Atmospheric Pollution and Cryospheric Change network to obtain a deep understanding of pollutant status in the TP. The organic carbon (OC) and elemental carbon (EC) concentrations decreased noticeably inwards from outside to inland of the TP, consistent with their emission load and also affected by transport process and meteorological condition. Urban areas, such as Kathmandu, Karachi, and Mardan, exhibited extremely high OC and EC concentrations, with low and high values occurring in the monsoon and non-monsoon seasons, respectively. However, remote regions inland the TP (e.g., Nam Co and Ngari) demonstrated much lower OC and EC concentrations. Different seasonal variations were observed between the southern and northern parts of the TP, suggesting differences in the patterns of pollutant sources and in distance from the sources between the two regions. In addition to the influence of long-range transported pollutants from the Indo-Gangetic Plain (IGP), the TP was affected by local emissions (e.g., biomass burning). The OC/EC ratio also suggested that biomass burning was prevalent in the center TP, whereas the marginal sites (e.g., Jomsom, Dhunche, and Laohugou) were affected by fossil fuel combustion from the up-wind regions. The mass absorption cross-section of EC (MACEC) at 632 nm ranged from 6.56 to 14.7 m2 g-1, with an increasing trend from outside to inland of the TP. Urban areas had low MACEC values because such regions were mainly affected by local fresh emissions. In addition, large amount of brown carbon can decrease the MACEC values in cities of South Asia. Remote sites had high MACEC values because of the coating enhancement of aerosols. Influenced by emission, transport process, and weather condition, the CA concentrations and MACEC presented decreasing and increasing trends, respectively, from outside to inland of the TP.

Abstract The transport sector has become an important source of urban greenhouse gas (GHG) and air pollutant emissions, with the continuous growth of transportation demand. The co-benefits of reducing GHG and air pollutant emissions in the transport sector are receiving more and more attention. Taking Guangzhou as the case study city, this study quantitatively analyzed the co-benefits of reducing CO2 and air pollutant emissions under the sustainable scenario in the transport sector by developing a quantitative analysis model based on the Long-range Energy Alternatives Planning (LEAP) framework. The co-benefits quantitative parameter and the co-benefits radar chart analysis method are used to identify and evaluate the generated co-benefits, and then the co-benefits generated by implementing the sustainable measures are discussed. The results show that adjusting transport modes and increasing the application of electricity are the two most effective measures for achieving the co-benefits of reducing CO2 and air pollutant emissions in the Guangzhou transport sector. Thus, these two measures are highly preferential for mitigating CO2 and air pollutant emissions. In addition, increasing the application of biofuel and hydrogen energy also has good co-benefits. However, increasing the application of Liquefied Natural Gas (LNG) has poor co-benefits. Promoting the utilization of LNG intercity buses, trucks, and cargo ships will lead to emission increases of CO and HC compared to the current policy scenario, and small emission reductions of CO2 and other air pollutants. Therefore, to promote the utilization of LNG vehicles and ships, it is necessary to cooperate with the use of air pollutant end removal devices and high-pressure direct injection (HPDI) gas engines.

Recycling the arsenic-rich biomass of Pteris vittata is a critical problem during phytoremediation primarily because of the low value and high risk of arsenic-rich biomass. Nevertheless, extracts of P. vittata have been found to have a variety of bio-activities (e.g., anti-oxidation, anti-cancer, and anti-bacterial) and abundant valuable bio-active compositions (e.g., flavonoids), which might present a new solution for the recycling of P. vittata harvests. This work demonstrated a pilot-scale experiment to extract and purify the phenolic compounds from 1 t of arsenic-rich P. vittata biomass. Result showed that 47.9 kg of phenolic-rich extract with a potential value of US$908.66-8345.14 was obtained. This extract showed no acute oral toxicities (LD50 > 10 g/kg), no skin irritation, and no chronic risks in the long-term skin contact exposure pathways. All of the wastes from production have been recycled and safely disposed with low cost (US$28.44), and the cost may be further reduced. The calculated benefits from this method showed a potential to provide 995-53,050 US$/hm2 per year to a phytoremediation project. Therefore, this strategy could address the issue of expensive phytoremediation.

Ecosystem water use efficiency (EWUE) is a popular issue in the comprehensive study of climate change, ecology, and hydrology. Currently, views on the response of EWUE to temperature, precipitation, and drought remain controversial. Based on ecosystem net primary productivity (NPP) and evapotranspiration (ET) datasets, both of which were retrieved from the Moderate Resolution Imaging Spectroradiometer (MODIS) using the Carnegie Ames Stanford approach (CASA) and surface energy balance algorithms for land (SEBAL) models, respectively, this study comprehensively examined the relationship between EWUE and temperature, precipitation, and drought in the Tianshan Mountains of Central Asia. The results showed that EWUE had an obvious temporal change trend in the Tianshan Mountains. The EWUEs of all vegetation types presented an increasing trend in spring and a decreasing trend in autumn. These results led to a phase shift in the annual cycle of EWUE over the years. Compared with 2000 to 2003, from 2012 to 2016, the annual EWUE cycle had advanced by 32 days. Precipitation generally had a negative effect on EWUE, while temperature had an obvious positive effect on EWUE. The EWUE responses to drought for the different vegetation types showed a variety of change trends. With the increase in drought stress, EWUE not only showed a simple upward or downward trend but also showed an upward trend followed by a downward trend or a downward trend followed by an upward trend. EWUE is more sensitive to changing environments than NPP or ET and is more suitable for analyzing ecosystem responses to global change.