AbstractObjectiveThe aim of the present article is to conduct an integrated assessment in order to explore whether CCS could be a viable technological option for significantly reducing future CO2 emissions in India.MethodsIn this paper, an integrated approach covering five assessment dimensions is chosen. However, each dimension is investigated using specific methods (graphical abstract).ResultsThe most crucial precondition that must be met is a reliable storage capacity assessment based on site-specific geological data since only rough figures concerning the theoretical capacity exist at present. Our projection of different trends of coal-based power plant capacities up to 2050 ranges between 13 and 111Gt of CO2 that may be captured from coal-fired power plants to be built by 2050. If very optimistic assumptions about the country’s CO2 storage potential are applied, 75Gt of CO2 could theoretically be stored as a result of matching these sources with suitable sinks. If a cautious approach is taken by considering the country’s effective storage potential, only a fraction may potentially be sequestered. In practice, this potential will decrease further with the impact of technical, legal, economic and social acceptance factors. Further constraints may be the delayed commercial availability of CCS in India, a significant barrier to achieving the economic viability of CCS, an expected net maximum reduction rate of the power plant’s greenhouse gas emissions of 71–74%, an increase of most other environmental and social impacts, and a lack of governmental, industrial or societal CCS advocates.Conclusion and practice implicationsSeveral preconditions need to be fulfilled if CCS is to play a future role in reducing CO2 emissions in India, the most crucial one being to determine reliable storage capacity figures. In order to overcome these barriers, the industrialised world would need to make a stronger commitment in terms of CCS technology demonstration, cooperation and transfer to emerging economies like India. The integrated assessment might also be extended by a comparison with other low-carbon technology options to draw fully valid conclusions on the most suitable solution for a sustainable future energy supply in India.