Abstract Carbon Capture and Storage at industrial processes (industrial CCS) is expected to play an important role in reducing industrial CO2 emissions in the short term. Industrial CCS involves capturing CO2 from industrial processes, such as steel and cement making, and storing the CO2 underground. This study examined the public opinion of industrial CCS through an informed opinion survey in the Netherlands (N = 987) and the United Kingdom (UK; N = 974). On average, respondents were neutral to slightly positive about the implementation of industrial CCS in their country. UK respondents were slightly more positive (M = 4.66 on a 7-point scale) than Dutch respondents (M = 4.38). Awareness and perceived knowledge levels were somewhat higher in the Netherlands than in the UK. In both countries, perceived outcomes of industrial CCS (e.g. for climate change; safety; employment) were strongly associated with industrial CCS opinion, when compared to socio-demographics, proximity to industry (actual and perceived), and psychological variables. Differences between countries in outcome perceptions occur. For example, the safety of CO2 transport is a larger concern in the Netherlands than in the UK, while cost-control is a larger concern in the UK than in the Netherlands. These findings suggest that the national context for CCS implementation matters. Our research suggests that public engagement strategies will benefit from focusing on the economic and climate impacts of industrial CCS, as well as from building trust in industry and addressing perceived safety concerns surrounding different aspects of industrial CCS.