Abstract An experiment using spent coffee grounds (SCGs) was performed with moisture (6.2, 22.5, 23.2, and 33.4% w.b.) and die height (42, 52, 62, 72, 82, and 92 mm) as influencing parameters at a stable temperature of 93 °C and speed of 100 mm min−1, and the monitoring curves of pressure-displacements were studied. Both pelletization factors were significant parameters for the maximum pressure and corresponding piston displacements, pellet movement, specific work, pellet density, and breaking strength. An interaction was found between these factors, but the moisture had a greater and nonlinear effect on the agglomeration parameters than the die height, which influenced linearly the change of these parameters. The agglomeration parameters values increased with decreasing moisture and increasing the die height. The results suggest that high-strength fuel pellets (>1.0 MPa) could be produced from SCG at a suitable moisture (