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Recycling of lithium iron phosphate batteries: Status, technologies, challenges, and prospects

The limited fossil fuel supply toward carbon neutrality has driven tremendous efforts to replace fuel vehicles by electric ones. The recycling of retired power batteries, a core energy supply component of electric vehicles (EVs), is necessary for developing a sustainable EV industry. Here, we comprehensively review the current status and technical challenges of recycling lithium iron phosphate (LFP) batteries. The review focuses on: 1) environmental risks of LFP batteries, 2) cascade utilization, 3) separation of cathode material and aluminium foil, 4) lithium (Li) extraction technologies, and 5) regeneration and transformation of cathode materials. Detailed analyses are elaborated with case examples and technical challenges. Our critical analysis demonstrates that compared with retired lithium nickel cobalt manganese oxide (NCM) batteries, LFP batteries do not contain the high-value elements such as Co and Ni, so the economic drive for LFP recycling is compromised although future market prospects are substantial. It is of great practical significance to develop low-carbon and cost-effective Li extraction technologies and regeneration processes for cathode materials to ensure a sustainable and stable development of the LFP battery and EV industry.
- University of Alberta Canada
- Hong Kong Polytechnic University China (People's Republic of)
- Korea University Korea (Republic of)
- Korea University Korea (Republic of)
- Sejong University Korea (Republic of)
Lithium extraction, Resources circulation, Sustainable development goals, Retired power batteries, Clean energy, Waste battery recycling
Lithium extraction, Resources circulation, Sustainable development goals, Retired power batteries, Clean energy, Waste battery recycling
citations This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).137 popularity This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.Top 1% influence This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).Top 10% impulse This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.Top 0.1%
