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Near-Infrared Plasmon-Induced Hot Electron Extraction Evidence in an Indium Tin Oxide Nanoparticle/Monolayer Molybdenum Disulfide Heterostructure

descriptionPublicationkeyboard_double_arrow_right Article , Other literature type , Preprint 18 Oct 2022Embargo end date: 01 Jan 2022 Switzerland, Italy Publisher:American Chemical Society (ACS)Journal:The Journal of Physical Chemistry Letters, volume 13, pages 9,903-9,909 (issn: 1948-7185, eissn: 1948-7185, Copyright policy )Funded by:EC | Light-DYNAMO, EC | LIGHT-CAP, EC | PAIDEIA
Authors: Michele Guizzardi; Michele Ghini; Andrea Villa; Luca Rebecchi; Qiuyang Li; Giorgio Mancini; Fabio Marangi; +4 Authors

doi: 10.1021/acs.jpclett.2c02358 , 10.48550/arxiv.2207.04195

pmid: 36256582

pmc: PMC9619877

arXiv: http://arxiv.org/abs/2207.04195 , 2207.04195

handle: 11583/2985586 , 11567/1146395 , 11311/1229808

Near-Infrared Plasmon-Induced Hot Electron Extraction Evidence in an Indium Tin Oxide Nanoparticle/Monolayer Molybdenum Disulfide Heterostructure

Abstract

In this work, we observe plasmon induced hot electron extraction in a heterojunction between indium tin oxide nanocrystals and monolayer molybdenum disulphide. We study the sample with ultrafast differential transmission exciting the sample at 1750 nm where the intense localized plasmon surface resonance of the indium tin oxide nanocrystals is and where the monolayer molybdenum disulphide does not absorb light. With the excitation at 1750 nm we observe the excitonic features of molybdenum disulphide in the visible range, close to the exciton of molybdenum disulphide. Such phenomenon can be ascribed to a charge transfer between indium tin oxide nanocrystals and monolayer molybdenum disulphide upon plasmon excitation. These results are a first step towards the implementation of near infrared plasmonic materials for photoconversion.

12 pages, 3 figures

Countries
Switzerland, Italy
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Keywords

spectroscopy, nanocrystals, Condensed Matter - Mesoscale and Nanoscale Physics, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), FOS: Physical sciences, size, Physics - Optics, Optics (physics.optics)

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
10
Top 10%
Average
Top 10%
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