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Thieno-Pyrrole-Fused 4,4-Difluoro-4-bora-3a,4a-diaza-s-indacene–Fullerene Dyads: Utilization of Near-Infrared Sensitizers for Ultrafast Charge Separation in Donor–Acceptor Systems

descriptionPublicationkeyboard_double_arrow_right Article , Journal 15 May 2014Publisher:American Chemical Society (ACS)Journal:Journal of the American Chemical Society, volume 136, pages 7,571-7,574 (issn: 0002-7863, eissn: 1520-5126,

Authors: Francis D'Souza; Venugopal Bandi; Sushanta K. Das; Samuel G. Awuah; Youngjae You;

doi: 10.1021/ja503015f

pmid: 24820034

Thieno-Pyrrole-Fused 4,4-Difluoro-4-bora-3a,4a-diaza-s-indacene–Fullerene Dyads: Utilization of Near-Infrared Sensitizers for Ultrafast Charge Separation in Donor–Acceptor Systems

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Abstract

Donor-acceptor dyads featuring near-IR sensitizers derived from thieno-pyrrole-fused BODIPY (abbreviated as SBDPiR) and fullerene, C60 have been newly synthesized and characterized. Occurrence of ultrafast photoinduced electron transfer (PET) leading to the formation of charge-separated state in these dyads, capable of harvesting light energy from the near-IR region, is established from femtosecond transient absorption studies.

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Keywords

Models, Molecular, Light, Molecular Structure, Fullerenes, Photochemical Processes

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NSF| Nanocarbon based Supramolecular Assemblies for Electron Transfer Applicable to Solar Energy Harvesting