Lithium-ion batteries are ubiquitous in modern day applications ranging from portable electronics to electric vehicles. Irrespective of the application, reliable real-time estimation of battery state of health (SOH) by on-board computers is crucial to the safe operation of the battery, ultimately safeguarding asset integrity. In this paper, we design and evaluate a machine learning pipeline for estimation of battery capacity fade - a metric of battery health - on 179 cells cycled under various conditions. The pipeline estimates battery SOH with an associated confidence interval by using two parametric and two non-parametric algorithms. Using segments of charge voltage and current curves, the pipeline engineers 30 features, performs automatic feature selection and calibrates the algorithms. When deployed on cells operated under the fast-charging protocol, the best model achieves a root mean squared percent error of 0.45\%. This work provides insights into the design of scalable data-driven models for battery SOH estimation, emphasising the value of confidence bounds around the prediction. The pipeline methodology combines experimental data with machine learning modelling and can be generalized to other critical components that require real-time estimation of SOH.

Peer review, pre-print to be published in Nature Machine Intelligence - 32 pages and 24 figures (including supplementary material)