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Imaging the Spatial Evolution of Degradation in Perovskite/Si Tandem Solar Cells After Exposure to Humid Air

handle: 10754/625772
Monolithically integrated two-terminal perovskite/Si tandem solar cells promise to achieve high power conversion efficiency. However, there is a concern that the stability of the perovskite top cell will limit the long-term performance of tandem devices. To investigate the impact of perovskite cell degradation on the photocurrent generation and collection in the individual subcells, we employed light beam induced current mapping to spatially resolve the photocurrent under controlled humidity conditions. The evolution of the device behavior is consistent with the formation of an optically transparent hydrated perovskite phase that allows the bottom Si cell to continue to generate photocurrent at the probing wavelength (532 nm). Additional measurements were performed on perovskite thin films on glass substrates to verify the interpretation.
- University System of Ohio United States
- King Abdullah University of Science and Technology Saudi Arabia
- University of Toledo United States
- Swiss Center for Electronics and Microtechnology (Switzerland) Switzerland
- University of Toledo United States
light beam induced current (LBIC), silicon, Degradation, tandem solar cells, perovskite
light beam induced current (LBIC), silicon, Degradation, tandem solar cells, perovskite
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