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Article . 2013 . Peer-reviewed
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Article . 2013
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Engineering Coherence Among Excited States in Synthetic Heterodimer Systems

Authors: Gregory S. Engel; Graham B. Griffin; Dugan Hayes;

Engineering Coherence Among Excited States in Synthetic Heterodimer Systems

Abstract

Coherence in Photosynthesis It is unclear how energy absorbed by pigments in antenna proteins is transferred to the central site of chemical catalysis during photosynthesis. Hildner et al. (p. 1448 ) observed coherence—prolonged persistence of a quantum mechanical phase relationship—at the single-molecule level in light-harvesting complexes from purple bacteria. The results bolster conclusions from past ensemble measurements that coherence plays a pivotal role in photosynthetic energy transfer. Hayes et al. (p. 1431 , published online 18 April) examined a series of small molecules comprised of bridged chromophores that also manifest prolonged coherence.

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Keywords

Fourier Analysis, Spectrum Analysis, Light-Harvesting Protein Complexes, Fluoresceins, Spectrometry, Fluorescence, Energy Transfer, Quantum Theory, Photosynthesis, Dimerization, Electromagnetic Phenomena

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    126
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Top 1%
    influence
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    impulse
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
126
Top 1%
Top 10%
Top 1%
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Energy Research