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Oxygen Electrode Reaction in a LiCl–KCl Eutectic Melt

descriptionPublicationkeyboard_double_arrow_right Article , Journal 01 Jan 2009 Japan Publisher:The Electrochemical SocietyJournal:Journal of The Electrochemical Society, volume 156, page E167 (issn: 0013-4651,

Authors: Kado, Yuya; Goto, Takuya; Hagiwara, Rika;

doi: 10.1149/1.3212844

handle: 2433/255613

Oxygen Electrode Reaction in a LiCl–KCl Eutectic Melt

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Abstract

Oxygen electrode reaction was investigated on a boron-doped diamond electrode in a LiCl―KCl eutectic melt. The standard formal potential of O 2 /O 2― decreases with the elevation of temperature. The potential at 773 K is 2.424 ± 0.003 V vs Li + /Li. The standard formal free energy change increases with the temperature elevation, calculated to be ―456.4 ± 0.5 kJ mol ―1 at 773 K. The standard formal entropy and enthalpy changes are determined to be ―151 ± 3 J K ―1 mol ―1 and ―573.5 ± 0.1 kJ mol ―1 , respectively, at 773 K.

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