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Radiation Induced Sodium Metal Colloid Formation in Natural Rock Salt From Different Geological Localities

Authors: Loman, J. M.; Levy, P. W.; Swyler, K. J.;

Radiation Induced Sodium Metal Colloid Formation in Natural Rock Salt From Different Geological Localities

Abstract

ABSTRACTRadiation damage has been studied in natural rock salt from various localities, including potential repository sites. In the 100 to 300 C range the damage consists of point defects, primarily F-centers, and colloidal metal sodium particles. With increasing dose the F-centers grow to a saturation level, reached at 107 –108 rad, that decreases with increasing temperature to a negligible level at 300 C. Colloid concentration vs. irradiation-time curves follow nucleation and growth curves accurately described by C tn, or C(dose)n, relations at large irradiation times. For fourteen samples,n = 1.85± 0.18 but the values of C vary by a factor of more than 103. The constant C is related to the sample strain, the impurity and void content, dose rate, and possibly other factors. The currently available data indicate that rock salt adjacent to radioactive waste canisters, at a temperature of 150 C, will contain between 0.01 and 10 mole percent of sodium metal when the total dose reaches 1010 rad.

Country
United States
Keywords

Radiation Doses, Doses, Alkali Metals, Geologic Deposits, Radioactive Waste Disposal, Comparative Evaluations, 360605 -- Materials-- Radiation Effects, Salt Deposits, Medium Temperature, Colloids, 12 Management Of Radioactive And Non-Radioactive Wastes From Nuclear Facilities, Dispersions, Vacancies, Physical Radiation Effects, Point Defects, High Temperature, 36 Materials Science, Waste Disposal, Sodium, Elements, Crystal Defects, Waste Management 052002* -- Nuclear Fuels-- Waste Disposal & Storage, Management, Radiation Effects, Particles, Metals, F Centers, Crystal Structure, Color Centers

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
2
Average
Average
Average
bronze