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Low Temperature Selective Catalytic Reduction Using Molding Catalysts Mn-Ce/FA and Mn-Ce/FA-30%TiO2

doi: 10.3390/en10122084
Low Temperature Selective Catalytic Reduction Using Molding Catalysts Mn-Ce/FA and Mn-Ce/FA-30%TiO2
Mn-Ce/FA (M) and Mn-Ce/FA-TiO2 (M), using fly ash (FA) with and without TiO2 as the carriers, were prepared by an integral molding technique. With the increase of TiO2 content, the rates of NO conversion and denitration of Mn-Ce/FA-TiO2 (M) increased, and the NO2 and N2O formation rates decreased. It is found that TiO2 could effectively inhibit the excessive oxidation of NO and the generation of N2O. The effects of space velocity, oxygen concentration and ammonia nitrogen ratio on three types of nitrogen oxides (NO, NO2, N2O) and denitration rates of the Mn-Ce/FA (M) and Mn-Ce/FA-30%TiO2 (M) were further investigated. In addition, it is demonstrated that Mn-Ce/FA (M) and Mn-Ce/FA-30%TiO2 (M) were more suitable to be used in the environment of low sulfur and less water.
- Hebei University of Technology China (People's Republic of)
- University of Hull United Kingdom
- Hebei University of Technology China (People's Republic of)
- University of Hull United Kingdom
- Queen's University Belfast United Kingdom
/dk/atira/pure/subjectarea/asjc/2100/2105, Technology, Control and Optimization, /dk/atira/pure/subjectarea/asjc/2600/2606; name=Control and Optimization, /dk/atira/pure/subjectarea/asjc/2600/2606, name=Energy Engineering and Power Technology, /dk/atira/pure/subjectarea/asjc/2200/2208, Catalyst molding, Energy Engineering and Power Technology, name=SDG 7 - Affordable and Clean Energy, catalyst molding; Mn-Ce/FA (M); Mn-Ce/FA-30%TiO<sub>2</sub> (M); NO<sub>2</sub>; N<sub>2</sub>O; NO, /dk/atira/pure/subjectarea/asjc/2100/2105; name=Renewable Energy, Sustainability and the Environment, NO2, name=Control and Optimization, NO, /dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energy; name=SDG 7 - Affordable and Clean Energy, name=Renewable Energy, name=Energy (miscellaneous), Renewable Energy, SDG 7 - Affordable and Clean Energy, Electrical and Electronic Engineering, /dk/atira/pure/subjectarea/asjc/2100/2101, /dk/atira/pure/subjectarea/asjc/2100/2102, Mn-Ce/FA (M), /dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energy, Sustainability and the Environment, catalyst molding, T, Mn-Ce/FA-30%TiO2 (M), N2O, name=Electrical and Electronic Engineering, 540, /dk/atira/pure/subjectarea/asjc/2100/2101; name=Energy (miscellaneous), /dk/atira/pure/subjectarea/asjc/2200/2208; name=Electrical and Electronic Engineering, Mn-Ce/FA-30%TiO (M), Energy (miscellaneous), /dk/atira/pure/subjectarea/asjc/2100/2102; name=Energy Engineering and Power Technology
/dk/atira/pure/subjectarea/asjc/2100/2105, Technology, Control and Optimization, /dk/atira/pure/subjectarea/asjc/2600/2606; name=Control and Optimization, /dk/atira/pure/subjectarea/asjc/2600/2606, name=Energy Engineering and Power Technology, /dk/atira/pure/subjectarea/asjc/2200/2208, Catalyst molding, Energy Engineering and Power Technology, name=SDG 7 - Affordable and Clean Energy, catalyst molding; Mn-Ce/FA (M); Mn-Ce/FA-30%TiO<sub>2</sub> (M); NO<sub>2</sub>; N<sub>2</sub>O; NO, /dk/atira/pure/subjectarea/asjc/2100/2105; name=Renewable Energy, Sustainability and the Environment, NO2, name=Control and Optimization, NO, /dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energy; name=SDG 7 - Affordable and Clean Energy, name=Renewable Energy, name=Energy (miscellaneous), Renewable Energy, SDG 7 - Affordable and Clean Energy, Electrical and Electronic Engineering, /dk/atira/pure/subjectarea/asjc/2100/2101, /dk/atira/pure/subjectarea/asjc/2100/2102, Mn-Ce/FA (M), /dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energy, Sustainability and the Environment, catalyst molding, T, Mn-Ce/FA-30%TiO2 (M), N2O, name=Electrical and Electronic Engineering, 540, /dk/atira/pure/subjectarea/asjc/2100/2101; name=Energy (miscellaneous), /dk/atira/pure/subjectarea/asjc/2200/2208; name=Electrical and Electronic Engineering, Mn-Ce/FA-30%TiO (M), Energy (miscellaneous), /dk/atira/pure/subjectarea/asjc/2100/2102; name=Energy Engineering and Power Technology
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