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Low Temperature Selective Catalytic Reduction Using Molding Catalysts Mn-Ce/FA and Mn-Ce/FA-30%TiO2

Authors: Xiang Gou; Yating Wang; Chunfei Wu; Shian Liu; Dong Zhao; Yamei Li; Saima Iram;

Low Temperature Selective Catalytic Reduction Using Molding Catalysts Mn-Ce/FA and Mn-Ce/FA-30%TiO2

Abstract

Mn-Ce/FA (M) and Mn-Ce/FA-TiO2 (M), using fly ash (FA) with and without TiO2 as the carriers, were prepared by an integral molding technique. With the increase of TiO2 content, the rates of NO conversion and denitration of Mn-Ce/FA-TiO2 (M) increased, and the NO2 and N2O formation rates decreased. It is found that TiO2 could effectively inhibit the excessive oxidation of NO and the generation of N2O. The effects of space velocity, oxygen concentration and ammonia nitrogen ratio on three types of nitrogen oxides (NO, NO2, N2O) and denitration rates of the Mn-Ce/FA (M) and Mn-Ce/FA-30%TiO2 (M) were further investigated. In addition, it is demonstrated that Mn-Ce/FA (M) and Mn-Ce/FA-30%TiO2 (M) were more suitable to be used in the environment of low sulfur and less water.

Country
United Kingdom
Related Organizations
Keywords

/dk/atira/pure/subjectarea/asjc/2100/2105, Technology, Control and Optimization, /dk/atira/pure/subjectarea/asjc/2600/2606; name=Control and Optimization, /dk/atira/pure/subjectarea/asjc/2600/2606, name=Energy Engineering and Power Technology, /dk/atira/pure/subjectarea/asjc/2200/2208, Catalyst molding, Energy Engineering and Power Technology, name=SDG 7 - Affordable and Clean Energy, catalyst molding; Mn-Ce/FA (M); Mn-Ce/FA-30%TiO<sub>2</sub> (M); NO<sub>2</sub>; N<sub>2</sub>O; NO, /dk/atira/pure/subjectarea/asjc/2100/2105; name=Renewable Energy, Sustainability and the Environment, NO2, name=Control and Optimization, NO, /dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energy; name=SDG 7 - Affordable and Clean Energy, name=Renewable Energy, name=Energy (miscellaneous), Renewable Energy, SDG 7 - Affordable and Clean Energy, Electrical and Electronic Engineering, /dk/atira/pure/subjectarea/asjc/2100/2101, /dk/atira/pure/subjectarea/asjc/2100/2102, Mn-Ce/FA (M), /dk/atira/pure/sustainabledevelopmentgoals/affordable_and_clean_energy, Sustainability and the Environment, catalyst molding, T, Mn-Ce/FA-30%TiO2 (M), N2O, name=Electrical and Electronic Engineering, 540, /dk/atira/pure/subjectarea/asjc/2100/2101; name=Energy (miscellaneous), /dk/atira/pure/subjectarea/asjc/2200/2208; name=Electrical and Electronic Engineering, Mn-Ce/FA-30%TiO (M), Energy (miscellaneous), /dk/atira/pure/subjectarea/asjc/2100/2102; name=Energy Engineering and Power Technology

  • BIP!
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    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    6
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    Average
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
6
Top 10%
Average
Average
Green
gold