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  • Energy Research

  • Authors: Qizhi Tan; Yanji Wang; Hangyu Li; Shuyang Liu; +1 Authors

    Summary The simulation of the in-situ conversion process (ICP) is a challenging endeavor that involves complicated thermal-reactive-compositional coupling processes. The upscaling of ICP simulation has been investigated, but the developed methods have significant limitations, which hinder their use in complicated models. The most constraining limitation of previous ICP upscaling techniques is that they all require modifications of the simulation code, which make them difficult to use in closed-source commercial simulators. In this paper, we introduce a novel upscaling method for ICP simulation. In this new method, we introduce two correction factors (namely α and β in this paper) to adjust the coarse-scale reaction frequency factor and activation energy. The calculation of the two factors is based on the reactions on both coarse-scale and fine-scale models. The new upscaling method does not entail any additional modifications of the underlying simulation source code, and thus it is more feasible to implement. We demonstrate the accuracy and efficiency of our upscaling method with 2D and 3D models, respectively. Apart from model dimensions, the availability of the novel upscaling method for ICP simulations with different values of kinetic parameters is considered as well. It is shown that the novel upscaling method provides reasonably accurate results, and significant computational savings are also achieved.

    SPE Journalarrow_drop_down
    SPE Journal
    Article . 2023 . Peer-reviewed
    Data sources: Crossref
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      SPE Journalarrow_drop_down
      SPE Journal
      Article . 2023 . Peer-reviewed
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  • Authors: Qizhi Tan; Yanji Wang; Hangyu Li; Shuyang Liu; +1 Authors

    Summary The simulation of the in-situ conversion process (ICP) is a challenging endeavor that involves complicated thermal-reactive-compositional coupling processes. The upscaling of ICP simulation has been investigated, but the developed methods have significant limitations, which hinder their use in complicated models. The most constraining limitation of previous ICP upscaling techniques is that they all require modifications of the simulation code, which make them difficult to use in closed-source commercial simulators. In this paper, we introduce a novel upscaling method for ICP simulation. In this new method, we introduce two correction factors (namely α and β in this paper) to adjust the coarse-scale reaction frequency factor and activation energy. The calculation of the two factors is based on the reactions on both coarse-scale and fine-scale models. The new upscaling method does not entail any additional modifications of the underlying simulation source code, and thus it is more feasible to implement. We demonstrate the accuracy and efficiency of our upscaling method with 2D and 3D models, respectively. Apart from model dimensions, the availability of the novel upscaling method for ICP simulations with different values of kinetic parameters is considered as well. It is shown that the novel upscaling method provides reasonably accurate results, and significant computational savings are also achieved.

    SPE Journalarrow_drop_down
    SPE Journal
    Article . 2023 . Peer-reviewed
    Data sources: Crossref
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      SPE Journalarrow_drop_down
      SPE Journal
      Article . 2023 . Peer-reviewed
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Jianchun Xu; Ziwei Bu; Hangyu Li; Xiaopu Wang; +1 Authors

    Natural gas hydrates (NGHs) are regarded as a new energy resource with great potential and wide application prospects due to their tremendous reserves and low CO2 emission. Permeability, which governs the fluid flow and transport through hydrate-bearing sediments (HBSs), directly affects the fluid production from hydrate deposits. Therefore, permeability models play a significant role in the prediction and optimization of gas production from NGH reservoirs via numerical simulators. To quantitatively analyze and predict the long-term gas production performance of hydrate deposits under distinct hydrate phase behavior and saturation, it is essential to well-establish the permeability model, which can accurately capture the characteristics of permeability change during production. Recently, a wide variety of permeability models for single-phase fluid flowing sediment have been established. They typically consider the influences of hydrate saturation, hydrate pore habits, sediment pore structure, and other related factors on the hydraulic properties of hydrate sediments. However, the choice of permeability prediction models leads to substantially different predictions of gas production in numerical modeling. In this work, the most available and widely used permeability models proposed by researchers worldwide were firstly reviewed in detail. We divide them into four categories, namely the classical permeability models, reservoir simulator used models, modified permeability models, and novel permeability models, based on their theoretical basis and derivation method. In addition, the advantages and limitations of each model were discussed with suggestions provided. Finally, the challenges existing in the current research were discussed and the potential future investigation directions were proposed. This review can provide insightful guidance for understanding the modeling of fluid flow in HBSs and can be useful for developing more advanced models for accurately predicting the permeability change during hydrate resources exploitation.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energiesarrow_drop_down
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    Energies
    Article . 2022 . Peer-reviewed
    License: CC BY
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    Energies
    Article . 2022
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      Energies
      Article . 2022 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Energies
      Article . 2022
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Jianchun Xu; Ziwei Bu; Hangyu Li; Xiaopu Wang; +1 Authors

    Natural gas hydrates (NGHs) are regarded as a new energy resource with great potential and wide application prospects due to their tremendous reserves and low CO2 emission. Permeability, which governs the fluid flow and transport through hydrate-bearing sediments (HBSs), directly affects the fluid production from hydrate deposits. Therefore, permeability models play a significant role in the prediction and optimization of gas production from NGH reservoirs via numerical simulators. To quantitatively analyze and predict the long-term gas production performance of hydrate deposits under distinct hydrate phase behavior and saturation, it is essential to well-establish the permeability model, which can accurately capture the characteristics of permeability change during production. Recently, a wide variety of permeability models for single-phase fluid flowing sediment have been established. They typically consider the influences of hydrate saturation, hydrate pore habits, sediment pore structure, and other related factors on the hydraulic properties of hydrate sediments. However, the choice of permeability prediction models leads to substantially different predictions of gas production in numerical modeling. In this work, the most available and widely used permeability models proposed by researchers worldwide were firstly reviewed in detail. We divide them into four categories, namely the classical permeability models, reservoir simulator used models, modified permeability models, and novel permeability models, based on their theoretical basis and derivation method. In addition, the advantages and limitations of each model were discussed with suggestions provided. Finally, the challenges existing in the current research were discussed and the potential future investigation directions were proposed. This review can provide insightful guidance for understanding the modeling of fluid flow in HBSs and can be useful for developing more advanced models for accurately predicting the permeability change during hydrate resources exploitation.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energiesarrow_drop_down
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    Energies
    Article . 2022 . Peer-reviewed
    License: CC BY
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    Energies
    Article . 2022
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energiesarrow_drop_down
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      Energies
      Article . 2022 . Peer-reviewed
      License: CC BY
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      Energies
      Article . 2022
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Shuyang Liu; Weiwei Jian; Yi Zhang; Wanli Xing; +5 Authors

    AbstractEnhanced Gas Recovery by injecting CO2 is one of the efficient scenarios to accelerate gas production if the excessive mixing can be avoided in the process of CO2-CH4 displacement. A laboratory investigation was presented to describe the detailed CO2-CH4 displacement and analyze CO2 dispersion into CH4 in the sand pack for pressure of 10-14MPa at 40°C with the CO2 injection rate of 0.2, 0.3 and 0.4ml/min. And the displacement process was scanned by an X-ray micro-CT scanner. The results of CT scan images were consistent with the breakthrough profile obtained from outlet gas composition analysis. The dispersion coefficient is in the range from 4.478×10-7 to 9.898×10−7mm2/s and it increase with interstitial velocity of CO2 and decrease with pressure. The dispersivity of BZ04 sand pack is calculated as 0.0054 m.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
    Article . 2014 . Peer-reviewed
    License: CC BY NC ND
    Data sources: Crossref
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    Energy Procedia
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    Energy Procedia
    Article . 2014
    License: CC BY NC ND
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    http://dx.doi.org/10.1016/j.eg...
    Article . Peer-reviewed
    Data sources: CORE
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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      Energy Procedia
      Article . 2014 . Peer-reviewed
      License: CC BY NC ND
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      Energy Procedia
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      Energy Procedia
      Article . 2014
      License: CC BY NC ND
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      http://dx.doi.org/10.1016/j.eg...
      Article . Peer-reviewed
      Data sources: CORE
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    Authors: Shuyang Liu; Weiwei Jian; Yi Zhang; Wanli Xing; +5 Authors

    AbstractEnhanced Gas Recovery by injecting CO2 is one of the efficient scenarios to accelerate gas production if the excessive mixing can be avoided in the process of CO2-CH4 displacement. A laboratory investigation was presented to describe the detailed CO2-CH4 displacement and analyze CO2 dispersion into CH4 in the sand pack for pressure of 10-14MPa at 40°C with the CO2 injection rate of 0.2, 0.3 and 0.4ml/min. And the displacement process was scanned by an X-ray micro-CT scanner. The results of CT scan images were consistent with the breakthrough profile obtained from outlet gas composition analysis. The dispersion coefficient is in the range from 4.478×10-7 to 9.898×10−7mm2/s and it increase with interstitial velocity of CO2 and decrease with pressure. The dispersivity of BZ04 sand pack is calculated as 0.0054 m.

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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
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    Energy Procedia
    Article . 2014
    License: CC BY NC ND
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    http://dx.doi.org/10.1016/j.eg...
    Article . Peer-reviewed
    Data sources: CORE
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      Energy Procedia
      Article . 2014 . Peer-reviewed
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      Energy Procedia
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      Energy Procedia
      Article . 2014
      License: CC BY NC ND
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      http://dx.doi.org/10.1016/j.eg...
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    Authors: Hangyu Li; Xianzhi Song; Shuyang Liu;

    Recent advances in computer and data sciences have made artificial intelligence techniques a useful tool in tackling the problems in petroleum exploration and production [...]

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Applied Sciencesarrow_drop_down
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    Applied Sciences
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    Applied Sciences
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      Applied Sciences
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    Authors: Hangyu Li; Xianzhi Song; Shuyang Liu;

    Recent advances in computer and data sciences have made artificial intelligence techniques a useful tool in tackling the problems in petroleum exploration and production [...]

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Applied Sciencesarrow_drop_down
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    Applied Sciences
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    Applied Sciences
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      Applied Sciences
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      Applied Sciences
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Shuyang Liu; Hangyu Li; Bin Wang; Baojiang Sun;

    Abstract Natural gas hydrate (NGH) will be one of the major future energy sources due to its properties of clean energy and large reserves. Depressurization is proposed as an effective method to extract natural gas from hydrate, however, the gas production from hydrate dissociation may be interrupted by ice generation and hydrate re-formation due to insufficient heat supply in the single depressurization process. To solve this issue, this work conducted simulation on accelerating gas production from the depressurization-induced methane hydrate by electrical heating. The continuous heating and intermittent heating modes were employed and then the electrical heating scheme was optimized for the comprehensive effect of high energy efficiency and high gas production rate. The results show that electrical heating is conducive to gas production from hydrate dissociation at a rapid rate. In the continuous heating, a high initial hydration saturation, low initial water saturation, low specific heat capacity, and high thermal conductivity result in the high gas generation rate and efficient electrical energy utilization (a large energy efficiency ratio). The intermittent heating has a higher efficient utilization of electrical energy than continuous heating. The optimal scheme is determined as the first-half heating type with the optimized electrical heating power of 25.6 W and the heating time of 12.5 min by the gradient descent method of AdaGrad. Compared to the baseline continuous heating case, the energy efficiency ratio (10.70) of the optimal scheme is enhanced by 24.7% with the average gas production rate (2.55 SmL/s) enhanced by 18.2%. It's hoped that the findings of this work can provide some insights into extracting natural gas from gas hydrate deposits.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Petroleum Science and Engineering
    Article . 2022 . Peer-reviewed
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Petroleum Science and Engineering
      Article . 2022 . Peer-reviewed
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Shuyang Liu; Hangyu Li; Bin Wang; Baojiang Sun;

    Abstract Natural gas hydrate (NGH) will be one of the major future energy sources due to its properties of clean energy and large reserves. Depressurization is proposed as an effective method to extract natural gas from hydrate, however, the gas production from hydrate dissociation may be interrupted by ice generation and hydrate re-formation due to insufficient heat supply in the single depressurization process. To solve this issue, this work conducted simulation on accelerating gas production from the depressurization-induced methane hydrate by electrical heating. The continuous heating and intermittent heating modes were employed and then the electrical heating scheme was optimized for the comprehensive effect of high energy efficiency and high gas production rate. The results show that electrical heating is conducive to gas production from hydrate dissociation at a rapid rate. In the continuous heating, a high initial hydration saturation, low initial water saturation, low specific heat capacity, and high thermal conductivity result in the high gas generation rate and efficient electrical energy utilization (a large energy efficiency ratio). The intermittent heating has a higher efficient utilization of electrical energy than continuous heating. The optimal scheme is determined as the first-half heating type with the optimized electrical heating power of 25.6 W and the heating time of 12.5 min by the gradient descent method of AdaGrad. Compared to the baseline continuous heating case, the energy efficiency ratio (10.70) of the optimal scheme is enhanced by 24.7% with the average gas production rate (2.55 SmL/s) enhanced by 18.2%. It's hoped that the findings of this work can provide some insights into extracting natural gas from gas hydrate deposits.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Petroleum Science and Engineering
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Petroleum Science and Engineering
      Article . 2022 . Peer-reviewed
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Guangming Fu; Bin Wang; Shuyang Liu; Jianchun Xu; +3 Authors

    Abstract The aim of CO2 enhanced gas recovery (CO2-EGR) is to extract more natural gas from depleted gas reservoirs and simultaneously sequestrate large amount of CO2. To achieve these dual objectives, the optimization of CO2 injection strategy in CO2-EGR is proposed to achieve maximum benefit. Thus, the focus of this work is to study CO2-EGR by numerical simulation and optimization. For this purpose, a 3D reservoir model with ‘five-spot’ well pattern (an injection well and four production wells) is established for simulations using the multiphase simulator TOUGH2, and the main focus is on optimization of CO2 injection rate and well placements by coupling the genetic algorithm (GA) with TOUGH2. Simulations are performed to determine the optimal injection rate for both two types of injection wells placements, one vertical injection well with number of perforations at various depth and orthogonal horizontal wells on top of the reservoir. The results show that multipoint perforations in the vertical injection well and the horizontal injection wells with appropriate length show improvement in natural gas recovery and CO2 storage compared to the injection location at the reservoir bottom. More importantly, the optimized injection rate determined by GA-TOUGH2 can substantially improve the natural gas recovery factor for both vertical and horizontal well injection. After computing a number of optimized cases, it’s shown that the case employing the horizontal injection wells with optimized injection rate of 0.0778 kg/s achieves the maximum recovery of 67.21% and maximum CO2 storage efficiency of 69.54%, equal to 23.88 × 106 kg of natural gas exploited from the depleted reservoir and 74.52 × 106 kg of CO2 stored in pore volume of 1.81 × 106 m3 of the reservoir. This case also has minimum injection pressure jump of 0.08 MPa thereby reducing the risk of formation fracture and CO2 leakage. However, by conducting a simple cost/benefit analysis, it is determined that this optimally performing case is not the best economically because of higher drilling cost of horizontal well compared to a vertical well. It is found that a vertical well with two suitably placed perforations with optimized injection rate of 0.1025 kg/s is economically superior since the previously used production wells can be reused for CO2 injection, which can therefore reduce both the equipment and the drilling costs. It is hoped that the findings of this work should provide some insights into the optimization of CO2-EGR with maximum economic benefit for implementation in industrial practice.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Cleaner P...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Cleaner Production
    Article . 2021 . Peer-reviewed
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Cleaner Production
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Guangming Fu; Bin Wang; Shuyang Liu; Jianchun Xu; +3 Authors

    Abstract The aim of CO2 enhanced gas recovery (CO2-EGR) is to extract more natural gas from depleted gas reservoirs and simultaneously sequestrate large amount of CO2. To achieve these dual objectives, the optimization of CO2 injection strategy in CO2-EGR is proposed to achieve maximum benefit. Thus, the focus of this work is to study CO2-EGR by numerical simulation and optimization. For this purpose, a 3D reservoir model with ‘five-spot’ well pattern (an injection well and four production wells) is established for simulations using the multiphase simulator TOUGH2, and the main focus is on optimization of CO2 injection rate and well placements by coupling the genetic algorithm (GA) with TOUGH2. Simulations are performed to determine the optimal injection rate for both two types of injection wells placements, one vertical injection well with number of perforations at various depth and orthogonal horizontal wells on top of the reservoir. The results show that multipoint perforations in the vertical injection well and the horizontal injection wells with appropriate length show improvement in natural gas recovery and CO2 storage compared to the injection location at the reservoir bottom. More importantly, the optimized injection rate determined by GA-TOUGH2 can substantially improve the natural gas recovery factor for both vertical and horizontal well injection. After computing a number of optimized cases, it’s shown that the case employing the horizontal injection wells with optimized injection rate of 0.0778 kg/s achieves the maximum recovery of 67.21% and maximum CO2 storage efficiency of 69.54%, equal to 23.88 × 106 kg of natural gas exploited from the depleted reservoir and 74.52 × 106 kg of CO2 stored in pore volume of 1.81 × 106 m3 of the reservoir. This case also has minimum injection pressure jump of 0.08 MPa thereby reducing the risk of formation fracture and CO2 leakage. However, by conducting a simple cost/benefit analysis, it is determined that this optimally performing case is not the best economically because of higher drilling cost of horizontal well compared to a vertical well. It is found that a vertical well with two suitably placed perforations with optimized injection rate of 0.1025 kg/s is economically superior since the previously used production wells can be reused for CO2 injection, which can therefore reduce both the equipment and the drilling costs. It is hoped that the findings of this work should provide some insights into the optimization of CO2-EGR with maximum economic benefit for implementation in industrial practice.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Cleaner P...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Cleaner Production
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Cleaner P...arrow_drop_down
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Cleaner Production
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    Authors: Changzhong Zhao; Shezhan Liu; Lei Yuan; Qian Zhang; +5 Authors

    Abstract The CO2/CH4 adsorption property on shale from Huadian shale gas reservoir in Jilin province of China was investigated at 40 °C with a wide pressure range (CH4: 0-15 MPa; CO2: 0-5 MPa) using a High Pressure Volumetric Analyzer (HPVAII-200), employing the static volumetric method. As the pressure rises, the excess adsorbed amount of CH4 increases gradually, while with the increasing pressure, the excess adsorbed amount of CO2 increases and then reaches the peak at about 4 MPa, followed by a downward trend. Furthermore, when the pressure is less than 5 MPa, the adsorption capacity of CO2 is obviously higher than that of CH4, and compared with CH4, the shale sample will preferentially adsorb CO2, which is beneficial to the application of CO2 enhanced shale gas recovery (CO2-ESGR).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
    Article . 2019 . Peer-reviewed
    License: CC BY NC ND
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    Energy Procedia
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      Energy Procedia
      Article . 2019 . Peer-reviewed
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      Energy Procedia
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    Authors: Changzhong Zhao; Shezhan Liu; Lei Yuan; Qian Zhang; +5 Authors

    Abstract The CO2/CH4 adsorption property on shale from Huadian shale gas reservoir in Jilin province of China was investigated at 40 °C with a wide pressure range (CH4: 0-15 MPa; CO2: 0-5 MPa) using a High Pressure Volumetric Analyzer (HPVAII-200), employing the static volumetric method. As the pressure rises, the excess adsorbed amount of CH4 increases gradually, while with the increasing pressure, the excess adsorbed amount of CO2 increases and then reaches the peak at about 4 MPa, followed by a downward trend. Furthermore, when the pressure is less than 5 MPa, the adsorption capacity of CO2 is obviously higher than that of CH4, and compared with CH4, the shale sample will preferentially adsorb CO2, which is beneficial to the application of CO2 enhanced shale gas recovery (CO2-ESGR).

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    Energy Procedia
    Article . 2019 . Peer-reviewed
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      Energy Procedia
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    Authors: Zhaoyan Liu; Wanli Xing; Weiwei Jian; Shuyang Liu; +3 Authors

    AbstractInjecting carbon dioxide into oil/gas fields has been regarded as a feasible way to reduce the global warming, at the same time it could enhance oil recovery. The density of CO2+oil is a key parameter for carbon dioxide capture and storage. Dodecane has similar thermal physical properties with petroleum. The aim of the work is to reveal the relationship between the density and the pressure and the temperature for the carbon dioxide (x) and dodecane (1-x). It was measured by the magnetic suspension balance (MSB) with temperature from 313.15K to 353.15K and pressure from 8 to 18MPa at different CO2 mole fractions: x=0, 0.2497, 0.5094, 0.7576 and 0.8610. The experimental results show that the density of CO2+dodecane mixture increases with the increasing pressure and decreases with the increasing temperature. It is found that the density of the mixture increases with the increasing concentration of CO2 firstly and then decreases at high mole fractions. The variation trend is similar with that of CO2+decane/tridecane mixtures. BWRS equation of state was established based on the experimental data, which agrees well with the density of CO2+dodecane.

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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
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    Energy Procedia
    Article . 2014
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    http://dx.doi.org/10.1016/j.eg...
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      Energy Procedia
      Article . 2014 . Peer-reviewed
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      Energy Procedia
      Article . 2014
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      http://dx.doi.org/10.1016/j.eg...
      Article . Peer-reviewed
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    Authors: Zhaoyan Liu; Wanli Xing; Weiwei Jian; Shuyang Liu; +3 Authors

    AbstractInjecting carbon dioxide into oil/gas fields has been regarded as a feasible way to reduce the global warming, at the same time it could enhance oil recovery. The density of CO2+oil is a key parameter for carbon dioxide capture and storage. Dodecane has similar thermal physical properties with petroleum. The aim of the work is to reveal the relationship between the density and the pressure and the temperature for the carbon dioxide (x) and dodecane (1-x). It was measured by the magnetic suspension balance (MSB) with temperature from 313.15K to 353.15K and pressure from 8 to 18MPa at different CO2 mole fractions: x=0, 0.2497, 0.5094, 0.7576 and 0.8610. The experimental results show that the density of CO2+dodecane mixture increases with the increasing pressure and decreases with the increasing temperature. It is found that the density of the mixture increases with the increasing concentration of CO2 firstly and then decreases at high mole fractions. The variation trend is similar with that of CO2+decane/tridecane mixtures. BWRS equation of state was established based on the experimental data, which agrees well with the density of CO2+dodecane.

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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
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    Energy Procedia
    Article . 2014
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    http://dx.doi.org/10.1016/j.eg...
    Article . Peer-reviewed
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      Energy Procedia
      Article . 2014
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      http://dx.doi.org/10.1016/j.eg...
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    Authors: Hangyu Li; Ze Zhou; Tao Long; Yao Wei; +3 Authors

    The U.S. Environmental Protection Agency’s (EPA) Superfund—the Comprehensive Environmental Response, Compensation, and Liability Act (CERCLA) database—has collected and built an open-source database based on nearly 2000 US soil remediation cases since 1980, providing detailed information and references for researchers worldwide to carry out remediation work. However, the cases were relatively independent to each other, so the whole database lacks systematicness and instructiveness to some extent. In this study, the basic features of all 144 soil remediation projects in four major oil-producing states (California, Texas, Oklahoma and Alaska) were extracted from the CERCLA database and the correlations among the pollutant species, pollutant site characteristics and selection of remediation methods were analyzed using traditional and machine learning techniques. The Decision Tree Classifier was selected as the machine learning model. The results showed that the growth of new contaminated sites has slowed down in recent years; physical remediation was the most commonly used method, and the probability of its application is more than 80%. The presence of benzene, toluene, ethylbenzene and xylene (BTEX) substances and the geographical location of the site were the two most influential factors in the choice of remediation method for a specific site; the maximum weights of these two features reaches 0.304 and 0.288.

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    Energies
    Article . 2022 . Peer-reviewed
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    Energies
    Article . 2022
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      Energies
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      Energies
      Article . 2022
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    Authors: Hangyu Li; Ze Zhou; Tao Long; Yao Wei; +3 Authors

    The U.S. Environmental Protection Agency’s (EPA) Superfund—the Comprehensive Environmental Response, Compensation, and Liability Act (CERCLA) database—has collected and built an open-source database based on nearly 2000 US soil remediation cases since 1980, providing detailed information and references for researchers worldwide to carry out remediation work. However, the cases were relatively independent to each other, so the whole database lacks systematicness and instructiveness to some extent. In this study, the basic features of all 144 soil remediation projects in four major oil-producing states (California, Texas, Oklahoma and Alaska) were extracted from the CERCLA database and the correlations among the pollutant species, pollutant site characteristics and selection of remediation methods were analyzed using traditional and machine learning techniques. The Decision Tree Classifier was selected as the machine learning model. The results showed that the growth of new contaminated sites has slowed down in recent years; physical remediation was the most commonly used method, and the probability of its application is more than 80%. The presence of benzene, toluene, ethylbenzene and xylene (BTEX) substances and the geographical location of the site were the two most influential factors in the choice of remediation method for a specific site; the maximum weights of these two features reaches 0.304 and 0.288.

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    Energies
    Article . 2022 . Peer-reviewed
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    Energies
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      Energies
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      Energies
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    Authors: Shuyang Liu; Yuan Chi; Yongchen Song; Wanli Xing; +1 Authors

    Abstract The adsorption/desorption of CH4/CO2/N2 mixture was investigated at 294 K, 311 K, 333 K, and 353 K with a wide pressure range (0∼70 Bar) on anthracite from China using a High Pressure Volumetric Analyzer (HPVAII-200). When the temperature is relatively low (293 K and 311 K), as the pressure rises, the excess adsorbed amount increases and peaks before experiencing a decrease. However, when the temperature is relatively high (353 K), the excess adsorbed amount increases and plateaus among the entire pressure range in this study. The pressure corresponding to the maximum adsorbed amount is lower in the process of desorption compared with adsorption, because there exists a hysteresis between adsorption and desorption. With the increasing temperature, the excess adsorbed amount is on the decline, which is the same as pure gas. While the pressure corresponding to the maximum adsorbed amount ascends as the temperature rises, even beyond the pressure range in this study. Moreover, the excess adsorbed amount have a good linear relationship with the temperature. Furthermore, the CO2 shows the best adsorption capacity and the adsorption capacity of CH4 is greater slightly than N2. In addition, with the increasing temperature, the competitive adsorption among CO2, CH4 and N2 is weaker.

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    Energy Procedia
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      Energy Procedia
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    Authors: Shuyang Liu; Yuan Chi; Yongchen Song; Wanli Xing; +1 Authors

    Abstract The adsorption/desorption of CH4/CO2/N2 mixture was investigated at 294 K, 311 K, 333 K, and 353 K with a wide pressure range (0∼70 Bar) on anthracite from China using a High Pressure Volumetric Analyzer (HPVAII-200). When the temperature is relatively low (293 K and 311 K), as the pressure rises, the excess adsorbed amount increases and peaks before experiencing a decrease. However, when the temperature is relatively high (353 K), the excess adsorbed amount increases and plateaus among the entire pressure range in this study. The pressure corresponding to the maximum adsorbed amount is lower in the process of desorption compared with adsorption, because there exists a hysteresis between adsorption and desorption. With the increasing temperature, the excess adsorbed amount is on the decline, which is the same as pure gas. While the pressure corresponding to the maximum adsorbed amount ascends as the temperature rises, even beyond the pressure range in this study. Moreover, the excess adsorbed amount have a good linear relationship with the temperature. Furthermore, the CO2 shows the best adsorption capacity and the adsorption capacity of CH4 is greater slightly than N2. In addition, with the increasing temperature, the competitive adsorption among CO2, CH4 and N2 is weaker.

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    Energy Procedia
    Article . 2017 . Peer-reviewed
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17 Research products
  • Authors: Qizhi Tan; Yanji Wang; Hangyu Li; Shuyang Liu; +1 Authors

    Summary The simulation of the in-situ conversion process (ICP) is a challenging endeavor that involves complicated thermal-reactive-compositional coupling processes. The upscaling of ICP simulation has been investigated, but the developed methods have significant limitations, which hinder their use in complicated models. The most constraining limitation of previous ICP upscaling techniques is that they all require modifications of the simulation code, which make them difficult to use in closed-source commercial simulators. In this paper, we introduce a novel upscaling method for ICP simulation. In this new method, we introduce two correction factors (namely α and β in this paper) to adjust the coarse-scale reaction frequency factor and activation energy. The calculation of the two factors is based on the reactions on both coarse-scale and fine-scale models. The new upscaling method does not entail any additional modifications of the underlying simulation source code, and thus it is more feasible to implement. We demonstrate the accuracy and efficiency of our upscaling method with 2D and 3D models, respectively. Apart from model dimensions, the availability of the novel upscaling method for ICP simulations with different values of kinetic parameters is considered as well. It is shown that the novel upscaling method provides reasonably accurate results, and significant computational savings are also achieved.

    SPE Journalarrow_drop_down
    SPE Journal
    Article . 2023 . Peer-reviewed
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      SPE Journal
      Article . 2023 . Peer-reviewed
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  • Authors: Qizhi Tan; Yanji Wang; Hangyu Li; Shuyang Liu; +1 Authors

    Summary The simulation of the in-situ conversion process (ICP) is a challenging endeavor that involves complicated thermal-reactive-compositional coupling processes. The upscaling of ICP simulation has been investigated, but the developed methods have significant limitations, which hinder their use in complicated models. The most constraining limitation of previous ICP upscaling techniques is that they all require modifications of the simulation code, which make them difficult to use in closed-source commercial simulators. In this paper, we introduce a novel upscaling method for ICP simulation. In this new method, we introduce two correction factors (namely α and β in this paper) to adjust the coarse-scale reaction frequency factor and activation energy. The calculation of the two factors is based on the reactions on both coarse-scale and fine-scale models. The new upscaling method does not entail any additional modifications of the underlying simulation source code, and thus it is more feasible to implement. We demonstrate the accuracy and efficiency of our upscaling method with 2D and 3D models, respectively. Apart from model dimensions, the availability of the novel upscaling method for ICP simulations with different values of kinetic parameters is considered as well. It is shown that the novel upscaling method provides reasonably accurate results, and significant computational savings are also achieved.

    SPE Journalarrow_drop_down
    SPE Journal
    Article . 2023 . Peer-reviewed
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      SPE Journal
      Article . 2023 . Peer-reviewed
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    Authors: Jianchun Xu; Ziwei Bu; Hangyu Li; Xiaopu Wang; +1 Authors

    Natural gas hydrates (NGHs) are regarded as a new energy resource with great potential and wide application prospects due to their tremendous reserves and low CO2 emission. Permeability, which governs the fluid flow and transport through hydrate-bearing sediments (HBSs), directly affects the fluid production from hydrate deposits. Therefore, permeability models play a significant role in the prediction and optimization of gas production from NGH reservoirs via numerical simulators. To quantitatively analyze and predict the long-term gas production performance of hydrate deposits under distinct hydrate phase behavior and saturation, it is essential to well-establish the permeability model, which can accurately capture the characteristics of permeability change during production. Recently, a wide variety of permeability models for single-phase fluid flowing sediment have been established. They typically consider the influences of hydrate saturation, hydrate pore habits, sediment pore structure, and other related factors on the hydraulic properties of hydrate sediments. However, the choice of permeability prediction models leads to substantially different predictions of gas production in numerical modeling. In this work, the most available and widely used permeability models proposed by researchers worldwide were firstly reviewed in detail. We divide them into four categories, namely the classical permeability models, reservoir simulator used models, modified permeability models, and novel permeability models, based on their theoretical basis and derivation method. In addition, the advantages and limitations of each model were discussed with suggestions provided. Finally, the challenges existing in the current research were discussed and the potential future investigation directions were proposed. This review can provide insightful guidance for understanding the modeling of fluid flow in HBSs and can be useful for developing more advanced models for accurately predicting the permeability change during hydrate resources exploitation.

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    Energies
    Article . 2022 . Peer-reviewed
    License: CC BY
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    Energies
    Article . 2022
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      Energies
      Article . 2022 . Peer-reviewed
      License: CC BY
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      Energies
      Article . 2022
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Jianchun Xu; Ziwei Bu; Hangyu Li; Xiaopu Wang; +1 Authors

    Natural gas hydrates (NGHs) are regarded as a new energy resource with great potential and wide application prospects due to their tremendous reserves and low CO2 emission. Permeability, which governs the fluid flow and transport through hydrate-bearing sediments (HBSs), directly affects the fluid production from hydrate deposits. Therefore, permeability models play a significant role in the prediction and optimization of gas production from NGH reservoirs via numerical simulators. To quantitatively analyze and predict the long-term gas production performance of hydrate deposits under distinct hydrate phase behavior and saturation, it is essential to well-establish the permeability model, which can accurately capture the characteristics of permeability change during production. Recently, a wide variety of permeability models for single-phase fluid flowing sediment have been established. They typically consider the influences of hydrate saturation, hydrate pore habits, sediment pore structure, and other related factors on the hydraulic properties of hydrate sediments. However, the choice of permeability prediction models leads to substantially different predictions of gas production in numerical modeling. In this work, the most available and widely used permeability models proposed by researchers worldwide were firstly reviewed in detail. We divide them into four categories, namely the classical permeability models, reservoir simulator used models, modified permeability models, and novel permeability models, based on their theoretical basis and derivation method. In addition, the advantages and limitations of each model were discussed with suggestions provided. Finally, the challenges existing in the current research were discussed and the potential future investigation directions were proposed. This review can provide insightful guidance for understanding the modeling of fluid flow in HBSs and can be useful for developing more advanced models for accurately predicting the permeability change during hydrate resources exploitation.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energiesarrow_drop_down
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    Energies
    Article . 2022 . Peer-reviewed
    License: CC BY
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      Energies
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      Energies
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    Authors: Shuyang Liu; Weiwei Jian; Yi Zhang; Wanli Xing; +5 Authors

    AbstractEnhanced Gas Recovery by injecting CO2 is one of the efficient scenarios to accelerate gas production if the excessive mixing can be avoided in the process of CO2-CH4 displacement. A laboratory investigation was presented to describe the detailed CO2-CH4 displacement and analyze CO2 dispersion into CH4 in the sand pack for pressure of 10-14MPa at 40°C with the CO2 injection rate of 0.2, 0.3 and 0.4ml/min. And the displacement process was scanned by an X-ray micro-CT scanner. The results of CT scan images were consistent with the breakthrough profile obtained from outlet gas composition analysis. The dispersion coefficient is in the range from 4.478×10-7 to 9.898×10−7mm2/s and it increase with interstitial velocity of CO2 and decrease with pressure. The dispersivity of BZ04 sand pack is calculated as 0.0054 m.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
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    Energy Procedia
    Article . 2014
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    http://dx.doi.org/10.1016/j.eg...
    Article . Peer-reviewed
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      Energy Procedia
      Article . 2014 . Peer-reviewed
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      Energy Procedia
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      Energy Procedia
      Article . 2014
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      http://dx.doi.org/10.1016/j.eg...
      Article . Peer-reviewed
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    Authors: Shuyang Liu; Weiwei Jian; Yi Zhang; Wanli Xing; +5 Authors

    AbstractEnhanced Gas Recovery by injecting CO2 is one of the efficient scenarios to accelerate gas production if the excessive mixing can be avoided in the process of CO2-CH4 displacement. A laboratory investigation was presented to describe the detailed CO2-CH4 displacement and analyze CO2 dispersion into CH4 in the sand pack for pressure of 10-14MPa at 40°C with the CO2 injection rate of 0.2, 0.3 and 0.4ml/min. And the displacement process was scanned by an X-ray micro-CT scanner. The results of CT scan images were consistent with the breakthrough profile obtained from outlet gas composition analysis. The dispersion coefficient is in the range from 4.478×10-7 to 9.898×10−7mm2/s and it increase with interstitial velocity of CO2 and decrease with pressure. The dispersivity of BZ04 sand pack is calculated as 0.0054 m.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
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    Energy Procedia
    Article . 2014
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    http://dx.doi.org/10.1016/j.eg...
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      Energy Procedia
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      Energy Procedia
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      Energy Procedia
      Article . 2014
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      http://dx.doi.org/10.1016/j.eg...
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Authors: Hangyu Li; Xianzhi Song; Shuyang Liu;

    Recent advances in computer and data sciences have made artificial intelligence techniques a useful tool in tackling the problems in petroleum exploration and production [...]

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    Applied Sciences
    Article . 2023 . Peer-reviewed
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    Applied Sciences
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      Applied Sciences
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    Authors: Hangyu Li; Xianzhi Song; Shuyang Liu;

    Recent advances in computer and data sciences have made artificial intelligence techniques a useful tool in tackling the problems in petroleum exploration and production [...]

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    Applied Sciences
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    Applied Sciences
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      Applied Sciences
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Shuyang Liu; Hangyu Li; Bin Wang; Baojiang Sun;

    Abstract Natural gas hydrate (NGH) will be one of the major future energy sources due to its properties of clean energy and large reserves. Depressurization is proposed as an effective method to extract natural gas from hydrate, however, the gas production from hydrate dissociation may be interrupted by ice generation and hydrate re-formation due to insufficient heat supply in the single depressurization process. To solve this issue, this work conducted simulation on accelerating gas production from the depressurization-induced methane hydrate by electrical heating. The continuous heating and intermittent heating modes were employed and then the electrical heating scheme was optimized for the comprehensive effect of high energy efficiency and high gas production rate. The results show that electrical heating is conducive to gas production from hydrate dissociation at a rapid rate. In the continuous heating, a high initial hydration saturation, low initial water saturation, low specific heat capacity, and high thermal conductivity result in the high gas generation rate and efficient electrical energy utilization (a large energy efficiency ratio). The intermittent heating has a higher efficient utilization of electrical energy than continuous heating. The optimal scheme is determined as the first-half heating type with the optimized electrical heating power of 25.6 W and the heating time of 12.5 min by the gradient descent method of AdaGrad. Compared to the baseline continuous heating case, the energy efficiency ratio (10.70) of the optimal scheme is enhanced by 24.7% with the average gas production rate (2.55 SmL/s) enhanced by 18.2%. It's hoped that the findings of this work can provide some insights into extracting natural gas from gas hydrate deposits.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
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    Journal of Petroleum Science and Engineering
    Article . 2022 . Peer-reviewed
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Petroleum Science and Engineering
      Article . 2022 . Peer-reviewed
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Shuyang Liu; Hangyu Li; Bin Wang; Baojiang Sun;

    Abstract Natural gas hydrate (NGH) will be one of the major future energy sources due to its properties of clean energy and large reserves. Depressurization is proposed as an effective method to extract natural gas from hydrate, however, the gas production from hydrate dissociation may be interrupted by ice generation and hydrate re-formation due to insufficient heat supply in the single depressurization process. To solve this issue, this work conducted simulation on accelerating gas production from the depressurization-induced methane hydrate by electrical heating. The continuous heating and intermittent heating modes were employed and then the electrical heating scheme was optimized for the comprehensive effect of high energy efficiency and high gas production rate. The results show that electrical heating is conducive to gas production from hydrate dissociation at a rapid rate. In the continuous heating, a high initial hydration saturation, low initial water saturation, low specific heat capacity, and high thermal conductivity result in the high gas generation rate and efficient electrical energy utilization (a large energy efficiency ratio). The intermittent heating has a higher efficient utilization of electrical energy than continuous heating. The optimal scheme is determined as the first-half heating type with the optimized electrical heating power of 25.6 W and the heating time of 12.5 min by the gradient descent method of AdaGrad. Compared to the baseline continuous heating case, the energy efficiency ratio (10.70) of the optimal scheme is enhanced by 24.7% with the average gas production rate (2.55 SmL/s) enhanced by 18.2%. It's hoped that the findings of this work can provide some insights into extracting natural gas from gas hydrate deposits.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Petroleum...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Petroleum Science and Engineering
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Petroleum Science and Engineering
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Guangming Fu; Bin Wang; Shuyang Liu; Jianchun Xu; +3 Authors

    Abstract The aim of CO2 enhanced gas recovery (CO2-EGR) is to extract more natural gas from depleted gas reservoirs and simultaneously sequestrate large amount of CO2. To achieve these dual objectives, the optimization of CO2 injection strategy in CO2-EGR is proposed to achieve maximum benefit. Thus, the focus of this work is to study CO2-EGR by numerical simulation and optimization. For this purpose, a 3D reservoir model with ‘five-spot’ well pattern (an injection well and four production wells) is established for simulations using the multiphase simulator TOUGH2, and the main focus is on optimization of CO2 injection rate and well placements by coupling the genetic algorithm (GA) with TOUGH2. Simulations are performed to determine the optimal injection rate for both two types of injection wells placements, one vertical injection well with number of perforations at various depth and orthogonal horizontal wells on top of the reservoir. The results show that multipoint perforations in the vertical injection well and the horizontal injection wells with appropriate length show improvement in natural gas recovery and CO2 storage compared to the injection location at the reservoir bottom. More importantly, the optimized injection rate determined by GA-TOUGH2 can substantially improve the natural gas recovery factor for both vertical and horizontal well injection. After computing a number of optimized cases, it’s shown that the case employing the horizontal injection wells with optimized injection rate of 0.0778 kg/s achieves the maximum recovery of 67.21% and maximum CO2 storage efficiency of 69.54%, equal to 23.88 × 106 kg of natural gas exploited from the depleted reservoir and 74.52 × 106 kg of CO2 stored in pore volume of 1.81 × 106 m3 of the reservoir. This case also has minimum injection pressure jump of 0.08 MPa thereby reducing the risk of formation fracture and CO2 leakage. However, by conducting a simple cost/benefit analysis, it is determined that this optimally performing case is not the best economically because of higher drilling cost of horizontal well compared to a vertical well. It is found that a vertical well with two suitably placed perforations with optimized injection rate of 0.1025 kg/s is economically superior since the previously used production wells can be reused for CO2 injection, which can therefore reduce both the equipment and the drilling costs. It is hoped that the findings of this work should provide some insights into the optimization of CO2-EGR with maximum economic benefit for implementation in industrial practice.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Cleaner P...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Cleaner Production
    Article . 2021 . Peer-reviewed
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Cleaner Production
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  • image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Authors: Guangming Fu; Bin Wang; Shuyang Liu; Jianchun Xu; +3 Authors

    Abstract The aim of CO2 enhanced gas recovery (CO2-EGR) is to extract more natural gas from depleted gas reservoirs and simultaneously sequestrate large amount of CO2. To achieve these dual objectives, the optimization of CO2 injection strategy in CO2-EGR is proposed to achieve maximum benefit. Thus, the focus of this work is to study CO2-EGR by numerical simulation and optimization. For this purpose, a 3D reservoir model with ‘five-spot’ well pattern (an injection well and four production wells) is established for simulations using the multiphase simulator TOUGH2, and the main focus is on optimization of CO2 injection rate and well placements by coupling the genetic algorithm (GA) with TOUGH2. Simulations are performed to determine the optimal injection rate for both two types of injection wells placements, one vertical injection well with number of perforations at various depth and orthogonal horizontal wells on top of the reservoir. The results show that multipoint perforations in the vertical injection well and the horizontal injection wells with appropriate length show improvement in natural gas recovery and CO2 storage compared to the injection location at the reservoir bottom. More importantly, the optimized injection rate determined by GA-TOUGH2 can substantially improve the natural gas recovery factor for both vertical and horizontal well injection. After computing a number of optimized cases, it’s shown that the case employing the horizontal injection wells with optimized injection rate of 0.0778 kg/s achieves the maximum recovery of 67.21% and maximum CO2 storage efficiency of 69.54%, equal to 23.88 × 106 kg of natural gas exploited from the depleted reservoir and 74.52 × 106 kg of CO2 stored in pore volume of 1.81 × 106 m3 of the reservoir. This case also has minimum injection pressure jump of 0.08 MPa thereby reducing the risk of formation fracture and CO2 leakage. However, by conducting a simple cost/benefit analysis, it is determined that this optimally performing case is not the best economically because of higher drilling cost of horizontal well compared to a vertical well. It is found that a vertical well with two suitably placed perforations with optimized injection rate of 0.1025 kg/s is economically superior since the previously used production wells can be reused for CO2 injection, which can therefore reduce both the equipment and the drilling costs. It is hoped that the findings of this work should provide some insights into the optimization of CO2-EGR with maximum economic benefit for implementation in industrial practice.

    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Journal of Cleaner P...arrow_drop_down
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Journal of Cleaner Production
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Journal of Cleaner Production
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    Authors: Changzhong Zhao; Shezhan Liu; Lei Yuan; Qian Zhang; +5 Authors

    Abstract The CO2/CH4 adsorption property on shale from Huadian shale gas reservoir in Jilin province of China was investigated at 40 °C with a wide pressure range (CH4: 0-15 MPa; CO2: 0-5 MPa) using a High Pressure Volumetric Analyzer (HPVAII-200), employing the static volumetric method. As the pressure rises, the excess adsorbed amount of CH4 increases gradually, while with the increasing pressure, the excess adsorbed amount of CO2 increases and then reaches the peak at about 4 MPa, followed by a downward trend. Furthermore, when the pressure is less than 5 MPa, the adsorption capacity of CO2 is obviously higher than that of CH4, and compared with CH4, the shale sample will preferentially adsorb CO2, which is beneficial to the application of CO2 enhanced shale gas recovery (CO2-ESGR).

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    Energy Procedia
    Article . 2019 . Peer-reviewed
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    Energy Procedia
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      Energy Procedia
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    Authors: Changzhong Zhao; Shezhan Liu; Lei Yuan; Qian Zhang; +5 Authors

    Abstract The CO2/CH4 adsorption property on shale from Huadian shale gas reservoir in Jilin province of China was investigated at 40 °C with a wide pressure range (CH4: 0-15 MPa; CO2: 0-5 MPa) using a High Pressure Volumetric Analyzer (HPVAII-200), employing the static volumetric method. As the pressure rises, the excess adsorbed amount of CH4 increases gradually, while with the increasing pressure, the excess adsorbed amount of CO2 increases and then reaches the peak at about 4 MPa, followed by a downward trend. Furthermore, when the pressure is less than 5 MPa, the adsorption capacity of CO2 is obviously higher than that of CH4, and compared with CH4, the shale sample will preferentially adsorb CO2, which is beneficial to the application of CO2 enhanced shale gas recovery (CO2-ESGR).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
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      Energy Procedia
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    Authors: Zhaoyan Liu; Wanli Xing; Weiwei Jian; Shuyang Liu; +3 Authors

    AbstractInjecting carbon dioxide into oil/gas fields has been regarded as a feasible way to reduce the global warming, at the same time it could enhance oil recovery. The density of CO2+oil is a key parameter for carbon dioxide capture and storage. Dodecane has similar thermal physical properties with petroleum. The aim of the work is to reveal the relationship between the density and the pressure and the temperature for the carbon dioxide (x) and dodecane (1-x). It was measured by the magnetic suspension balance (MSB) with temperature from 313.15K to 353.15K and pressure from 8 to 18MPa at different CO2 mole fractions: x=0, 0.2497, 0.5094, 0.7576 and 0.8610. The experimental results show that the density of CO2+dodecane mixture increases with the increasing pressure and decreases with the increasing temperature. It is found that the density of the mixture increases with the increasing concentration of CO2 firstly and then decreases at high mole fractions. The variation trend is similar with that of CO2+decane/tridecane mixtures. BWRS equation of state was established based on the experimental data, which agrees well with the density of CO2+dodecane.

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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
    Article . 2014
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    http://dx.doi.org/10.1016/j.eg...
    Article . Peer-reviewed
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      Energy Procedia
      Article . 2014 . Peer-reviewed
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      Energy Procedia
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      Energy Procedia
      Article . 2014
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      http://dx.doi.org/10.1016/j.eg...
      Article . Peer-reviewed
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    Authors: Zhaoyan Liu; Wanli Xing; Weiwei Jian; Shuyang Liu; +3 Authors

    AbstractInjecting carbon dioxide into oil/gas fields has been regarded as a feasible way to reduce the global warming, at the same time it could enhance oil recovery. The density of CO2+oil is a key parameter for carbon dioxide capture and storage. Dodecane has similar thermal physical properties with petroleum. The aim of the work is to reveal the relationship between the density and the pressure and the temperature for the carbon dioxide (x) and dodecane (1-x). It was measured by the magnetic suspension balance (MSB) with temperature from 313.15K to 353.15K and pressure from 8 to 18MPa at different CO2 mole fractions: x=0, 0.2497, 0.5094, 0.7576 and 0.8610. The experimental results show that the density of CO2+dodecane mixture increases with the increasing pressure and decreases with the increasing temperature. It is found that the density of the mixture increases with the increasing concentration of CO2 firstly and then decreases at high mole fractions. The variation trend is similar with that of CO2+decane/tridecane mixtures. BWRS equation of state was established based on the experimental data, which agrees well with the density of CO2+dodecane.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
    Article . 2014 . Peer-reviewed
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    Energy Procedia
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    Energy Procedia
    Article . 2014
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    http://dx.doi.org/10.1016/j.eg...
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      Energy Procedia
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      Energy Procedia
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      http://dx.doi.org/10.1016/j.eg...
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    Authors: Hangyu Li; Ze Zhou; Tao Long; Yao Wei; +3 Authors

    The U.S. Environmental Protection Agency’s (EPA) Superfund—the Comprehensive Environmental Response, Compensation, and Liability Act (CERCLA) database—has collected and built an open-source database based on nearly 2000 US soil remediation cases since 1980, providing detailed information and references for researchers worldwide to carry out remediation work. However, the cases were relatively independent to each other, so the whole database lacks systematicness and instructiveness to some extent. In this study, the basic features of all 144 soil remediation projects in four major oil-producing states (California, Texas, Oklahoma and Alaska) were extracted from the CERCLA database and the correlations among the pollutant species, pollutant site characteristics and selection of remediation methods were analyzed using traditional and machine learning techniques. The Decision Tree Classifier was selected as the machine learning model. The results showed that the growth of new contaminated sites has slowed down in recent years; physical remediation was the most commonly used method, and the probability of its application is more than 80%. The presence of benzene, toluene, ethylbenzene and xylene (BTEX) substances and the geographical location of the site were the two most influential factors in the choice of remediation method for a specific site; the maximum weights of these two features reaches 0.304 and 0.288.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energiesarrow_drop_down
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    Energies
    Article . 2022 . Peer-reviewed
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    Energies
    Article . 2022
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      Energies
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      Energies
      Article . 2022
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    Authors: Hangyu Li; Ze Zhou; Tao Long; Yao Wei; +3 Authors

    The U.S. Environmental Protection Agency’s (EPA) Superfund—the Comprehensive Environmental Response, Compensation, and Liability Act (CERCLA) database—has collected and built an open-source database based on nearly 2000 US soil remediation cases since 1980, providing detailed information and references for researchers worldwide to carry out remediation work. However, the cases were relatively independent to each other, so the whole database lacks systematicness and instructiveness to some extent. In this study, the basic features of all 144 soil remediation projects in four major oil-producing states (California, Texas, Oklahoma and Alaska) were extracted from the CERCLA database and the correlations among the pollutant species, pollutant site characteristics and selection of remediation methods were analyzed using traditional and machine learning techniques. The Decision Tree Classifier was selected as the machine learning model. The results showed that the growth of new contaminated sites has slowed down in recent years; physical remediation was the most commonly used method, and the probability of its application is more than 80%. The presence of benzene, toluene, ethylbenzene and xylene (BTEX) substances and the geographical location of the site were the two most influential factors in the choice of remediation method for a specific site; the maximum weights of these two features reaches 0.304 and 0.288.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energiesarrow_drop_down
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    Energies
    Article . 2022 . Peer-reviewed
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    Energies
    Article . 2022
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      Energies
      Article . 2022 . Peer-reviewed
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      Energies
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    Authors: Shuyang Liu; Yuan Chi; Yongchen Song; Wanli Xing; +1 Authors

    Abstract The adsorption/desorption of CH4/CO2/N2 mixture was investigated at 294 K, 311 K, 333 K, and 353 K with a wide pressure range (0∼70 Bar) on anthracite from China using a High Pressure Volumetric Analyzer (HPVAII-200). When the temperature is relatively low (293 K and 311 K), as the pressure rises, the excess adsorbed amount increases and peaks before experiencing a decrease. However, when the temperature is relatively high (353 K), the excess adsorbed amount increases and plateaus among the entire pressure range in this study. The pressure corresponding to the maximum adsorbed amount is lower in the process of desorption compared with adsorption, because there exists a hysteresis between adsorption and desorption. With the increasing temperature, the excess adsorbed amount is on the decline, which is the same as pure gas. While the pressure corresponding to the maximum adsorbed amount ascends as the temperature rises, even beyond the pressure range in this study. Moreover, the excess adsorbed amount have a good linear relationship with the temperature. Furthermore, the CO2 shows the best adsorption capacity and the adsorption capacity of CH4 is greater slightly than N2. In addition, with the increasing temperature, the competitive adsorption among CO2, CH4 and N2 is weaker.

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    Energy Procedia
    Article . 2017 . Peer-reviewed
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      Energy Procedia
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    Authors: Shuyang Liu; Yuan Chi; Yongchen Song; Wanli Xing; +1 Authors

    Abstract The adsorption/desorption of CH4/CO2/N2 mixture was investigated at 294 K, 311 K, 333 K, and 353 K with a wide pressure range (0∼70 Bar) on anthracite from China using a High Pressure Volumetric Analyzer (HPVAII-200). When the temperature is relatively low (293 K and 311 K), as the pressure rises, the excess adsorbed amount increases and peaks before experiencing a decrease. However, when the temperature is relatively high (353 K), the excess adsorbed amount increases and plateaus among the entire pressure range in this study. The pressure corresponding to the maximum adsorbed amount is lower in the process of desorption compared with adsorption, because there exists a hysteresis between adsorption and desorption. With the increasing temperature, the excess adsorbed amount is on the decline, which is the same as pure gas. While the pressure corresponding to the maximum adsorbed amount ascends as the temperature rises, even beyond the pressure range in this study. Moreover, the excess adsorbed amount have a good linear relationship with the temperature. Furthermore, the CO2 shows the best adsorption capacity and the adsorption capacity of CH4 is greater slightly than N2. In addition, with the increasing temperature, the competitive adsorption among CO2, CH4 and N2 is weaker.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
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    Energy Procedia
    Article . 2017 . Peer-reviewed
    License: CC BY NC ND
    Data sources: Crossref
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    Energy Procedia
    Article
    License: CC BY NC ND
    Data sources: UnpayWall
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Energy Procediaarrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Energy Procedia
      Article . 2017 . Peer-reviewed
      License: CC BY NC ND
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Energy Procedia
      Article
      License: CC BY NC ND
      Data sources: UnpayWall
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      addClaim

      This Research product is the result of merged Research products in OpenAIRE.

      You have already added works in your ORCID record related to the merged Research product.
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