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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Frédéric Chevallier; Frank Hase; Peter Bergamaschi; Christian Frankenberg; +46 Authors

    Abstract The GHG-CCI project is one of several projects of the European Space Agency's (ESA) Climate Change Initiative (CCI). The goal of the CCI is to generate and deliver data sets of various satellite-derived Essential Climate Variables (ECVs) in line with GCOS (Global Climate Observing System) requirements. The “ECV Greenhouse Gases” (ECV GHG) is the global distribution of important climate relevant gases – atmospheric CO 2 and CH 4 – with a quality sufficient to obtain information on regional CO 2 and CH 4 sources and sinks. Two satellite instruments deliver the main input data for GHG-CCI: SCIAMACHY/ENVISAT and TANSO-FTS/GOSAT. The first order priority goal of GHG-CCI is the further development of retrieval algorithms for near-surface-sensitive column-averaged dry air mole fractions of CO 2 and CH 4 , denoted XCO 2 and XCH 4 , to meet the demanding user requirements. GHG-CCI focuses on four core data products: XCO 2 from SCIAMACHY and TANSO and XCH 4 from the same two sensors. For each of the four core data products at least two candidate retrieval algorithms have been independently further developed and the corresponding data products have been quality-assessed and inter-compared. This activity is referred to as “Round Robin” (RR) activity within the CCI. The main goal of the RR was to identify for each of the four core products which algorithms should be used to generate the Climate Research Data Package (CRDP). The CRDP will essentially be the first version of the ECV GHG. This manuscript gives an overview of the GHG-CCI RR and related activities. This comprises the establishment of the user requirements, the improvement of the candidate retrieval algorithms and comparisons with ground-based observations and models. The manuscript summarizes the final RR algorithm selection decision and its justification. Comparison with ground-based Total Carbon Column Observing Network (TCCON) data indicates that the “breakthrough” single measurement precision requirement has been met for SCIAMACHY and TANSO XCO 2 ( 4 ( 4 is 3–15 ppb for SCIAMACHY and 2–8 ppb for TANSO depending on algorithm and time period. Meeting the 0.5 ppm systematic error requirement for XCO 2 remains a challenge: approximately 1 ppm has been achieved at the validation sites but also larger differences have been found in regions remote from TCCON. More research is needed to identify the causes for the observed differences. In this context GHG-CCI suggests taking advantage of the ensemble of existing data products, for example, via the EnseMble Median Algorithm (EMMA).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Hyper Article en Lig...arrow_drop_down
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Remote Sensing of Environment
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    Article . 2015
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Article . 2015
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    HAL AMU
    Article . 2015
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    HAL-CEA
    Article . 2015
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    HAL-INSU
    Article . 2015
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Remote Sensing of Environment
    Article . 2015 . Peer-reviewed
    License: Elsevier TDM
    Data sources: Crossref
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    OPUS Augsburg
    Article . 2015
    Data sources: OPUS Augsburg
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Hyper Article en Lig...arrow_drop_down
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Remote Sensing of Environment
      Article
      License: CC BY NC ND
      Data sources: UnpayWall
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      HAL UPEC
      Article . 2015
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      HAL-UPMC
      Article . 2015
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Article . 2015
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Article . 2015
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Article . 2015
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Article . 2015
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      Remote Sensing of Environment
      Article . 2015 . Peer-reviewed
      License: Elsevier TDM
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      OPUS Augsburg
      Article . 2015
      Data sources: OPUS Augsburg
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: R. J. Parker; R. J. Parker; H. Boesch; H. Boesch; +8 Authors

    Abstract. The 2015–2016 strong El Niño event has had a dramatic impact on the amount of Indonesian biomass burning, with the El Niño-driven drought further desiccating the already-drier-than-normal landscapes that are the result of decades of peatland draining, widespread deforestation, anthropogenically driven forest degradation and previous large fire events. It is expected that the 2015–2016 Indonesian fires will have emitted globally significant quantities of greenhouse gases (GHGs) to the atmosphere, as did previous El Niño-driven fires in the region. The form which the carbon released from the combustion of the vegetation and peat soils takes has a strong bearing on its atmospheric chemistry and climatological impacts. Typically, burning in tropical forests and especially in peatlands is expected to involve a much higher proportion of smouldering combustion than the more flaming-characterised fires that occur in fine-fuel-dominated environments such as grasslands, consequently producing significantly more CH4 (and CO) per unit of fuel burned. However, currently there have been no aircraft campaigns sampling Indonesian fire plumes, and very few ground-based field campaigns (none during El Niño), so our understanding of the large-scale chemical composition of these extremely significant fire plumes is surprisingly poor compared to, for example, those of southern Africa or the Amazon.Here, for the first time, we use satellite observations of CH4 and CO2 from the Greenhouse gases Observing SATellite (GOSAT) made in large-scale plumes from the 2015 El Niño-driven Indonesian fires to probe aspects of their chemical composition. We demonstrate significant modifications in the concentration of these species in the regional atmosphere around Indonesia, due to the fire emissions.Using CO and fire radiative power (FRP) data from the Copernicus Atmosphere Service, we identify fire-affected GOSAT soundings and show that peaks in fire activity are followed by subsequent large increases in regional greenhouse gas concentrations. CH4 is particularly enhanced, due to the dominance of smouldering combustion in peatland fires, with CH4 total column values typically exceeding 35 ppb above those of background “clean air” soundings. By examining the CH4 and CO2 excess concentrations in the fire-affected GOSAT observations, we determine the CH4 to CO2 (CH4 ∕ CO2) fire emission ratio for the entire 2-month period of the most extreme burning (September–October 2015), and also for individual shorter periods where the fire activity temporarily peaks. We demonstrate that the overall CH4 to CO2 emission ratio (ER) for fires occurring in Indonesia over this time is 6.2 ppb ppm−1. This is higher than that found over both the Amazon (5.1 ppb ppm−1) and southern Africa (4.4 ppb ppm−1), consistent with the Indonesian fires being characterised by an increased amount of smouldering combustion due to the large amount of organic soil (peat) burning involved. We find the range of our satellite-derived Indonesian ERs (6.18–13.6 ppb ppm−1) to be relatively closely matched to that of a series of close-to-source, ground-based sampling measurements made on Kalimantan at the height of the fire event (7.53–19.67 ppb ppm−1), although typically the satellite-derived quantities are slightly lower on average. This seems likely because our field sampling mostly intersected smaller-scale peat-burning plumes, whereas the large-scale plumes intersected by the GOSAT Thermal And Near infrared Sensor for carbon Observation – Fourier Transform Spectrometer (TANSO-FTS) footprints would very likely come from burning that was occurring in a mixture of fuels that included peat, tropical forest and already-cleared areas of forest characterised by more fire-prone vegetation types than the natural rainforest biome (e.g. post-fire areas of ferns and scrubland, along with agricultural vegetation).The ability to determine large-scale ERs from satellite data allows the combustion behaviour of very large regions of burning to be characterised and understood in a way not possible with ground-based studies, and which can be logistically difficult and very costly to consider using aircraft observations. We therefore believe the method demonstrated here provides a further important tool for characterising biomass burning emissions, and that the GHG ERs derived for the first time for these large-scale Indonesian fire plumes during an El Niño event point to more routinely assessing spatiotemporal variations in biomass burning ERs using future satellite missions. These will have more complete spatial sampling than GOSAT and will enable the contributions of these fires to the regional atmospheric chemistry and climate to be better understood.

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    Atmospheric Chemistry and Physics (ACP)
    Article . 2016 . Peer-reviewed
    License: CC BY
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    Atmospheric Chemistry and Physics (ACP)
    Article
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    https://doi.org/10.5194/acp-20...
    Article . 2016 . Peer-reviewed
    License: CC BY
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    https://www.atmos-chem-phys.ne...
    Article
    License: CC BY
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    Atmospheric Chemistry and Physics (ACP)
    Other literature type . 2018
    Data sources: Copernicus
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    Copernicus Publications
    Other literature type . 2018
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ CGIAR CGSpace (Consu...arrow_drop_down
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      Atmospheric Chemistry and Physics (ACP)
      Article . 2016 . Peer-reviewed
      License: CC BY
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      Atmospheric Chemistry and Physics (ACP)
      Article
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      https://doi.org/10.5194/acp-20...
      Article . 2016 . Peer-reviewed
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      Atmospheric Chemistry and Physics (ACP)
      Other literature type . 2018
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Copernicus Publications
      Other literature type . 2018
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    Authors: Yang, D.; Liu, Y.; Boesch, H.; Yao, L.; +8 Authors

    The 1st Chinese carbon dioxide (CO2) monitoring satellite mission, TanSat, was launched in 2016. The 1st TanSat global map of CO2 dry-air mixing ratio (XCO2) measurements over land was released as version 1 data product with an accuracy of 2.11 ppmv (parts per million by volume). In this paper, we introduce a new (version 2) TanSat global XCO2 product that is approached by the Institute of Atmospheric Physics Carbon dioxide retrieval Algorithm for Satellite remote sensing (IAPCAS), and the European Space Agency (ESA) Climate Change Initiative plus (CCI+) TanSat XCO2 product by University of Leicester Full Physics (UoL-FP) retrieval algorithm. The correction of the measurement spectrum improves the accuracy (@#@0.08 ppmv) and precision (1.41 ppmv) of the new retrieval, which provides opportunity for further application in global carbon flux studies in the future. Inter-comparison between the two retrievals indicates a good agreement, with a standard deviation of 1.28 ppmv and a bias of −0.35 ppmv.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Advances in Atmosphe...arrow_drop_down
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    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Advances in Atmospheric Sciences
    Article . 2020 . Peer-reviewed
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Advances in Atmosphe...arrow_drop_down
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Advances in Atmospheric Sciences
      Article . 2020 . Peer-reviewed
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      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
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    Authors: Buchwitz, M.; Reuter, M.; Schneising, O.; Boesch, H.; +38 Authors

    Abstract. The GHG-CCI project (http://www.esa-ghg-cci.org/) is one of several projects of the European Space Agency’s (ESA) Climate Change Initiative (CCI). The goal of the CCI is to generate and deliver data sets of various satellite-derived Essential Climate Variables (ECVs) in line with GCOS (Global Climate Observing System) requirements. The “ECV Greenhouse Gases” (ECV GHG) is the global distribution of important climate relevant gases – namely atmospheric CO2 and CH4 - with a quality sufficient to obtain information on regional CO2 and CH4 sources and sinks. The main goal of GHG-CCI is to generate long-term highly accurate and precise time series of global near-surface-sensitive satellite observations of CO2 and CH4, i.e., XCO2 and XCH4, starting with the launch of ESA’s ENVISAT satellite. These products are currently retrieved from SCIAMACHY/ENVISAT (2002-2012) and TANSO-FTS/GOSAT (2009-today) nadir mode observations in the near-infrared/shortwave-infrared spectral region. In addition, other sensors (e.g., IASI and MIPAS) and viewing modes (e.g., SCIAMACHY solar occultation) are also considered and in the future also data from other satellites. The GHG-CCI data products and related documentation are freely available via the GHG-CCI website and yearly updates are foreseen. Here we present an overview about the latest data set (Climate Research Data Package No. 2 (CRDP#2)) and summarize key findings from using satellite CO2 and CH4 retrievals to improve our understanding of the natural and anthropogenic sources and sinks of these important atmospheric greenhouse gases. We also shortly mention ongoing activities related to validation and initial user assessment of CRDP#2 and future plans.

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    Copernicus Publications
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      Copernicus Publications
      Other literature type . 2019
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    Authors: Xiao Lu; Daniel J. Jacob; Yuzhong Zhang; Lu Shen; +11 Authors

    The United States is the world’s largest oil/gas methane emitter according to current national reports. Reducing these emissions is a top priority in the US government’s climate action plan. Here, we use a 2010 to 2019 high-resolution inversion of surface and satellite observations of atmospheric methane to quantify emission trends for individual oil/gas production regions in North America and relate them to production and infrastructure. We estimate a mean US oil/gas methane emission of 14.8 (12.4 to 16.5) Tg a−1for 2010 to 2019, 70% higher than reported by the US Environmental Protection Agency. While emissions in Canada and Mexico decreased over the period, US emissions increased from 2010 to 2014, decreased until 2017, and rose again afterward. Increases were driven by the largest production regions (Permian, Anadarko, Marcellus), while emissions in the smaller production regions generally decreased. Much of the year-to-year emission variability can be explained by oil/gas production rates, active well counts, and new wells drilled, with the 2014 to 2017 decrease driven by reduction in new wells and the 2017 to 2019 surge driven by upswing of production. We find a steady decrease in the oil/gas methane intensity (emission per unit methane gas production) for almost all major US production regions. The mean US methane intensity decreased from 3.7% in 2010 to 2.5% in 2019. If the methane intensity for the oil/gas supply chain continues to decrease at this pace, we may expect a 32% decrease in US oil/gas emissions by 2030 despite projected increases in production.

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    Proceedings of the National Academy of Sciences
    Article . 2023 . Peer-reviewed
    License: CC BY
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    https://dx.doi.org/10.60692/fj...
    Other literature type . 2023
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    https://dx.doi.org/10.60692/yb...
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    Authors: Buchwitz, Michael; Reuter, Maximilian; Schneising, O; Hewson, W; +22 Authors

    Carbon dioxide (CO2) and methane (CH4) are the two most important greenhouse gases emitted by mankind. Better knowledge of the surface sources and sinks of these Essential Climate Variables (ECVs) and related carbon uptake and release processes is needed for important climate change related applications such as improved climate modelling and prediction. Some satellites provide near-surface-sensitive atmospheric CO2 and CH4 observations that can be used to obtain information on CO2 and CH4 surface fluxes. The goal of the GHG-CCI project of the European Space Agency's (ESA) Climate Change Initiative (CCI) is to use satellite data to generate atmospheric CO2 and CH4 data products meeting demanding GCOS (Global Climate Observing System) greenhouse gas (GHG) ECV requirements. To achieve this, retrieval algorithms are regularly being improved followed by annual data reprocessing and analysis cycles to generate better products in terms of extended time series and continuously improved data quality. Here we present an overview about the latest GHG-CCI data set called Climate Research Data Package No. 3 (CRDP3) focusing on the GHG-CCI core data products, which are column-averaged dry-air mole fractions of CO2 and CH4, i.e., XCO2 and XCH4, as retrieved from SCIAMACHY/ENVISAT and TANSO/GOSAT satellite radiances covering the time period end of 2002 to end of 2014. We present global maps and time series including initial validation results obtained by comparisons with Total Carbon Column Observing Network (TCCON) ground-based observations. We show that the GCOS requirements for systematic error (< 1 ppm for XCO2, < 10 ppb for XCH4) and long-term stability (< 0.2 ppm/year for XCO2, < 2 ppb/year for XCH4) are met for nearly all products (an exception is SCIAMACHY methane especially since 2010). For XCO2 we present comparisons with global models using the output of two CO2 assimilation systems (MACC version 14r2 and CarbonTracker version CT2013B). We show that overall there is reasonable consistency and agreement between all data sets (within ~ 1–2 ppm) but we also found significant differences depending on region and time period.

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    Article . 2017
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    Remote Sensing of Environment
    Article . 2017 . Peer-reviewed
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      Remote Sensing of Environment
      Article . 2017 . Peer-reviewed
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    Authors: Ross, A. N.; Wooster, M. J.; Boesch, Hartmut; Parker, Robert;

    Using methane and carbon dioxide atmospheric mixing ratios retrieved using SWIR spectra from the Greenhouse Gases Observing SATellite (GOSAT), we report the first wildfire plume CH4 to CO2 emission ratios (ERCH4/CO2) determined from space. We demonstrate the approach's potential using forward modeling and identify a series of real GOSAT spectra containing wildfire plumes. These show significantly changed total‐column CO2 and CH4 mixing ratios, and from these we calculate ERCH4/CO2 for boreal forest, tropical forest, and savanna fires as 0.00603, 0.00527, and 0.00395 mol mol−1, respectively. These ERs are statistically significantly different from each other and from the “normal” atmospheric CH4 to CO2 ratio and generally agree with past ground and airborne studies.

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    Geophysical Research Letters
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    Geophysical Research Letters
    Article . 2013 . Peer-reviewed
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      Geophysical Research Letters
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    Authors: Mahesh Kumar Sha; Saswati Das; Matthias M. Frey; Darko Dubravica; +53 Authors

    The COllaborative Carbon Column Observing Network has become a reliable source of high-quality ground-based remote sensing network data that provide column-averaged dry-air mole fractions of carbon dioxide (XCO2), methane (XCH4), and carbon monoxide (XCO). The fiducial reference measurements of these gases from the COCCON complement the TCCON and NDACC-IRWG data. This study shows the application of COCCON data for the validation of existing greenhouse gas satellite products. This study includes the validation of XCH4 and XCO products from the European Copernicus Sentinel-5 Precursor (S5P) mission, XCO2 products from the American Orbiting Carbon Observatory-2 (OCO-2) mission, and XCO2 and XCH4 products from the Japanese Greenhouse gases Observing SATellite (GOSAT). A total of 27 datasets contributed to this study; some of these were collected in the framework of campaign activities and covered only a short time period. In addition, several permanent stations provided long-term observations. The random uncertainties in the validation results, specifically for S5P with a lot of coincidences pairs, are found to be similar to the comparison with the TCCON. The comparison results of OCO-2 land nadir and land glint observation modes to the COCCON on a global scale, despite limited coincidences, are very promising. The stations can, therefore, expand on the coverage of the already existing ground-based reference remote sensing sites from the TCCON and the NDACC network. The COCCON data can be used for future satellite and model validation studies and carbon cycle studies.

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    Remote Sensing
    Article . 2025 . Peer-reviewed
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    Article . 2025
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    Article . 2025
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      https://dx.doi.org/10.5445/ir/...
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      Article . 2025
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Article . 2025 . Peer-reviewed
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Yuzhong Zhang; Shuangxi Fang; Jianmeng Chen; Yi Lin; +10 Authors

    China is set to actively reduce its methane emissions in the coming decade. A comprehensive evaluation of the current situation can provide a reference point for tracking the country’s future progress. Here, using satellite and surface observations, we quantify China’s methane emissions during 2010–2017. Including newly available data from a surface network across China greatly improves our ability to constrain emissions at subnational and sectoral levels. Our results show that recent changes in China’s methane emissions are linked to energy, agricultural, and environmental policies. We find contrasting methane emission trends in different regions attributed to coal mining, reflecting region-dependent responses to China’s energy policy of closing small coal mines (decreases in Southwest) and consolidating large coal mines (increases in North). Coordinated production of coalbed methane and coal in southern Shanxi effectively decreases methane emissions, despite increased coal production there. We also detect unexpected increases from rice cultivation over East and Central China, which is contributed by enhanced rates of crop-residue application, a factor not accounted for in current inventories. Our work identifies policy drivers of recent changes in China’s methane emissions, providing input to formulating methane policy toward its climate goal.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Proceedings of the N...arrow_drop_down
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    Proceedings of the National Academy of Sciences
    Article . 2022 . Peer-reviewed
    License: CC BY
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    https://doi.org/10.5194/egusph...
    Article . 2023 . Peer-reviewed
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    https://dx.doi.org/10.60692/am...
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    https://dx.doi.org/10.60692/gx...
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/

    Abstract. China, being one of the major emitters of greenhouse gases, has taken strong actions to tackle climate change, e.g., to achieve carbon neutrality by 2060. It also becomes important to better understand the changes in the atmospheric mixing ratio and emissions of CH4, the second most important human-influenced greenhouse gas, in China. Here we analyze the sources contributing to the atmospheric CH4 mixing ratio and their trends in China over 2007–2018 using the GEOS-Chem model simulations driven by two commonly used global anthropogenic emission inventories: the Emissions Database for Global Atmospheric Research (EDGAR v4.3.2) and the Community Emissions Data System (CEDS). The model results are interpreted with an ensemble of surface, aircraft, and satellite observations of CH4 mixing ratios over China and the Pacific region. The EDGAR and CEDS estimates show considerable differences reflecting large uncertainties in estimates of Chinese CH4 emissions. Chinese CH4 emission estimates based on EDGAR and natural sources increase from 46.7 Tg per annum (Tg a−1) in 1980 to 69.8 Tg a−1 in 2012 with an increase rate of 0.7 Tg a−2, and estimates with CEDS increase from 32.9 Tg a−1 in 1980 and 76.7 Tg a−1 in 2014 (a much stronger trend of 1.3 Tg a−2 over the period). Both surface, aircraft, and satellite measurements indicate CH4 increase rates of 7.0–8.4 ppbv a−1 over China in the recent decade. We find that the model simulation using the CEDS inventory and interannually varying OH levels can best reproduce these observed CH4 mixing ratios and trends over China. Model results over China are sensitive to the global OH level, with a 10 % increase in the global tropospheric volume-weighted mean OH concentration presenting a similar effect to that of a 47 Tg a−1 decrease in global CH4 emissions. We further apply a tagged tracer simulation to quantify the source contributions from different emission sectors and regions. We find that domestic CH4 emissions account for 11.4 % of the mean surface mixing ratio and drive 68.3 % of the surface trend (mainly via the energy sector) in China over 2007–2018. We emphasize that intensive CH4 measurements covering eastern China will help better assess the driving factors of CH4 mixing ratios and support the emission mitigation in China.

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    https://doi.org/10.5194/acp-20...
    Article . 2021 . Peer-reviewed
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    https://acp.copernicus.org/art...
    Article
    License: CC BY
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    Atmospheric Chemistry and Physics (ACP)
    Article . 2022 . Peer-reviewed
    License: CC BY
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    Atmospheric Chemistry and Physics (ACP)
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    https://dx.doi.org/10.60692/72...
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ https://doi.org/10.5...arrow_drop_down
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      https://doi.org/10.5194/acp-20...
      Article . 2021 . Peer-reviewed
      License: CC BY
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      https://acp.copernicus.org/art...
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Atmospheric Chemistry and Physics (ACP)
      Article . 2022 . Peer-reviewed
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      https://dx.doi.org/10.60692/72...
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Frédéric Chevallier; Frank Hase; Peter Bergamaschi; Christian Frankenberg; +46 Authors

    Abstract The GHG-CCI project is one of several projects of the European Space Agency's (ESA) Climate Change Initiative (CCI). The goal of the CCI is to generate and deliver data sets of various satellite-derived Essential Climate Variables (ECVs) in line with GCOS (Global Climate Observing System) requirements. The “ECV Greenhouse Gases” (ECV GHG) is the global distribution of important climate relevant gases – atmospheric CO 2 and CH 4 – with a quality sufficient to obtain information on regional CO 2 and CH 4 sources and sinks. Two satellite instruments deliver the main input data for GHG-CCI: SCIAMACHY/ENVISAT and TANSO-FTS/GOSAT. The first order priority goal of GHG-CCI is the further development of retrieval algorithms for near-surface-sensitive column-averaged dry air mole fractions of CO 2 and CH 4 , denoted XCO 2 and XCH 4 , to meet the demanding user requirements. GHG-CCI focuses on four core data products: XCO 2 from SCIAMACHY and TANSO and XCH 4 from the same two sensors. For each of the four core data products at least two candidate retrieval algorithms have been independently further developed and the corresponding data products have been quality-assessed and inter-compared. This activity is referred to as “Round Robin” (RR) activity within the CCI. The main goal of the RR was to identify for each of the four core products which algorithms should be used to generate the Climate Research Data Package (CRDP). The CRDP will essentially be the first version of the ECV GHG. This manuscript gives an overview of the GHG-CCI RR and related activities. This comprises the establishment of the user requirements, the improvement of the candidate retrieval algorithms and comparisons with ground-based observations and models. The manuscript summarizes the final RR algorithm selection decision and its justification. Comparison with ground-based Total Carbon Column Observing Network (TCCON) data indicates that the “breakthrough” single measurement precision requirement has been met for SCIAMACHY and TANSO XCO 2 ( 4 ( 4 is 3–15 ppb for SCIAMACHY and 2–8 ppb for TANSO depending on algorithm and time period. Meeting the 0.5 ppm systematic error requirement for XCO 2 remains a challenge: approximately 1 ppm has been achieved at the validation sites but also larger differences have been found in regions remote from TCCON. More research is needed to identify the causes for the observed differences. In this context GHG-CCI suggests taking advantage of the ensemble of existing data products, for example, via the EnseMble Median Algorithm (EMMA).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Hyper Article en Lig...arrow_drop_down
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Authors: R. J. Parker; R. J. Parker; H. Boesch; H. Boesch; +8 Authors

    Abstract. The 2015–2016 strong El Niño event has had a dramatic impact on the amount of Indonesian biomass burning, with the El Niño-driven drought further desiccating the already-drier-than-normal landscapes that are the result of decades of peatland draining, widespread deforestation, anthropogenically driven forest degradation and previous large fire events. It is expected that the 2015–2016 Indonesian fires will have emitted globally significant quantities of greenhouse gases (GHGs) to the atmosphere, as did previous El Niño-driven fires in the region. The form which the carbon released from the combustion of the vegetation and peat soils takes has a strong bearing on its atmospheric chemistry and climatological impacts. Typically, burning in tropical forests and especially in peatlands is expected to involve a much higher proportion of smouldering combustion than the more flaming-characterised fires that occur in fine-fuel-dominated environments such as grasslands, consequently producing significantly more CH4 (and CO) per unit of fuel burned. However, currently there have been no aircraft campaigns sampling Indonesian fire plumes, and very few ground-based field campaigns (none during El Niño), so our understanding of the large-scale chemical composition of these extremely significant fire plumes is surprisingly poor compared to, for example, those of southern Africa or the Amazon.Here, for the first time, we use satellite observations of CH4 and CO2 from the Greenhouse gases Observing SATellite (GOSAT) made in large-scale plumes from the 2015 El Niño-driven Indonesian fires to probe aspects of their chemical composition. We demonstrate significant modifications in the concentration of these species in the regional atmosphere around Indonesia, due to the fire emissions.Using CO and fire radiative power (FRP) data from the Copernicus Atmosphere Service, we identify fire-affected GOSAT soundings and show that peaks in fire activity are followed by subsequent large increases in regional greenhouse gas concentrations. CH4 is particularly enhanced, due to the dominance of smouldering combustion in peatland fires, with CH4 total column values typically exceeding 35 ppb above those of background “clean air” soundings. By examining the CH4 and CO2 excess concentrations in the fire-affected GOSAT observations, we determine the CH4 to CO2 (CH4 ∕ CO2) fire emission ratio for the entire 2-month period of the most extreme burning (September–October 2015), and also for individual shorter periods where the fire activity temporarily peaks. We demonstrate that the overall CH4 to CO2 emission ratio (ER) for fires occurring in Indonesia over this time is 6.2 ppb ppm−1. This is higher than that found over both the Amazon (5.1 ppb ppm−1) and southern Africa (4.4 ppb ppm−1), consistent with the Indonesian fires being characterised by an increased amount of smouldering combustion due to the large amount of organic soil (peat) burning involved. We find the range of our satellite-derived Indonesian ERs (6.18–13.6 ppb ppm−1) to be relatively closely matched to that of a series of close-to-source, ground-based sampling measurements made on Kalimantan at the height of the fire event (7.53–19.67 ppb ppm−1), although typically the satellite-derived quantities are slightly lower on average. This seems likely because our field sampling mostly intersected smaller-scale peat-burning plumes, whereas the large-scale plumes intersected by the GOSAT Thermal And Near infrared Sensor for carbon Observation – Fourier Transform Spectrometer (TANSO-FTS) footprints would very likely come from burning that was occurring in a mixture of fuels that included peat, tropical forest and already-cleared areas of forest characterised by more fire-prone vegetation types than the natural rainforest biome (e.g. post-fire areas of ferns and scrubland, along with agricultural vegetation).The ability to determine large-scale ERs from satellite data allows the combustion behaviour of very large regions of burning to be characterised and understood in a way not possible with ground-based studies, and which can be logistically difficult and very costly to consider using aircraft observations. We therefore believe the method demonstrated here provides a further important tool for characterising biomass burning emissions, and that the GHG ERs derived for the first time for these large-scale Indonesian fire plumes during an El Niño event point to more routinely assessing spatiotemporal variations in biomass burning ERs using future satellite missions. These will have more complete spatial sampling than GOSAT and will enable the contributions of these fires to the regional atmospheric chemistry and climate to be better understood.

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    Atmospheric Chemistry and Physics (ACP)
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      Copernicus Publications
      Other literature type . 2018
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    Authors: Yang, D.; Liu, Y.; Boesch, H.; Yao, L.; +8 Authors

    The 1st Chinese carbon dioxide (CO2) monitoring satellite mission, TanSat, was launched in 2016. The 1st TanSat global map of CO2 dry-air mixing ratio (XCO2) measurements over land was released as version 1 data product with an accuracy of 2.11 ppmv (parts per million by volume). In this paper, we introduce a new (version 2) TanSat global XCO2 product that is approached by the Institute of Atmospheric Physics Carbon dioxide retrieval Algorithm for Satellite remote sensing (IAPCAS), and the European Space Agency (ESA) Climate Change Initiative plus (CCI+) TanSat XCO2 product by University of Leicester Full Physics (UoL-FP) retrieval algorithm. The correction of the measurement spectrum improves the accuracy (@#@0.08 ppmv) and precision (1.41 ppmv) of the new retrieval, which provides opportunity for further application in global carbon flux studies in the future. Inter-comparison between the two retrievals indicates a good agreement, with a standard deviation of 1.28 ppmv and a bias of −0.35 ppmv.

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    Advances in Atmospheric Sciences
    Article . 2020 . Peer-reviewed
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      Advances in Atmospheric Sciences
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    Authors: Buchwitz, M.; Reuter, M.; Schneising, O.; Boesch, H.; +38 Authors

    Abstract. The GHG-CCI project (http://www.esa-ghg-cci.org/) is one of several projects of the European Space Agency’s (ESA) Climate Change Initiative (CCI). The goal of the CCI is to generate and deliver data sets of various satellite-derived Essential Climate Variables (ECVs) in line with GCOS (Global Climate Observing System) requirements. The “ECV Greenhouse Gases” (ECV GHG) is the global distribution of important climate relevant gases – namely atmospheric CO2 and CH4 - with a quality sufficient to obtain information on regional CO2 and CH4 sources and sinks. The main goal of GHG-CCI is to generate long-term highly accurate and precise time series of global near-surface-sensitive satellite observations of CO2 and CH4, i.e., XCO2 and XCH4, starting with the launch of ESA’s ENVISAT satellite. These products are currently retrieved from SCIAMACHY/ENVISAT (2002-2012) and TANSO-FTS/GOSAT (2009-today) nadir mode observations in the near-infrared/shortwave-infrared spectral region. In addition, other sensors (e.g., IASI and MIPAS) and viewing modes (e.g., SCIAMACHY solar occultation) are also considered and in the future also data from other satellites. The GHG-CCI data products and related documentation are freely available via the GHG-CCI website and yearly updates are foreseen. Here we present an overview about the latest data set (Climate Research Data Package No. 2 (CRDP#2)) and summarize key findings from using satellite CO2 and CH4 retrievals to improve our understanding of the natural and anthropogenic sources and sinks of these important atmospheric greenhouse gases. We also shortly mention ongoing activities related to validation and initial user assessment of CRDP#2 and future plans.

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    Copernicus Publications
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      Copernicus Publications
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    Authors: Xiao Lu; Daniel J. Jacob; Yuzhong Zhang; Lu Shen; +11 Authors

    The United States is the world’s largest oil/gas methane emitter according to current national reports. Reducing these emissions is a top priority in the US government’s climate action plan. Here, we use a 2010 to 2019 high-resolution inversion of surface and satellite observations of atmospheric methane to quantify emission trends for individual oil/gas production regions in North America and relate them to production and infrastructure. We estimate a mean US oil/gas methane emission of 14.8 (12.4 to 16.5) Tg a−1for 2010 to 2019, 70% higher than reported by the US Environmental Protection Agency. While emissions in Canada and Mexico decreased over the period, US emissions increased from 2010 to 2014, decreased until 2017, and rose again afterward. Increases were driven by the largest production regions (Permian, Anadarko, Marcellus), while emissions in the smaller production regions generally decreased. Much of the year-to-year emission variability can be explained by oil/gas production rates, active well counts, and new wells drilled, with the 2014 to 2017 decrease driven by reduction in new wells and the 2017 to 2019 surge driven by upswing of production. We find a steady decrease in the oil/gas methane intensity (emission per unit methane gas production) for almost all major US production regions. The mean US methane intensity decreased from 3.7% in 2010 to 2.5% in 2019. If the methane intensity for the oil/gas supply chain continues to decrease at this pace, we may expect a 32% decrease in US oil/gas emissions by 2030 despite projected increases in production.

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    Proceedings of the National Academy of Sciences
    Article . 2023 . Peer-reviewed
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    https://dx.doi.org/10.60692/fj...
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    https://dx.doi.org/10.60692/yb...
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    Authors: Buchwitz, Michael; Reuter, Maximilian; Schneising, O; Hewson, W; +22 Authors

    Carbon dioxide (CO2) and methane (CH4) are the two most important greenhouse gases emitted by mankind. Better knowledge of the surface sources and sinks of these Essential Climate Variables (ECVs) and related carbon uptake and release processes is needed for important climate change related applications such as improved climate modelling and prediction. Some satellites provide near-surface-sensitive atmospheric CO2 and CH4 observations that can be used to obtain information on CO2 and CH4 surface fluxes. The goal of the GHG-CCI project of the European Space Agency's (ESA) Climate Change Initiative (CCI) is to use satellite data to generate atmospheric CO2 and CH4 data products meeting demanding GCOS (Global Climate Observing System) greenhouse gas (GHG) ECV requirements. To achieve this, retrieval algorithms are regularly being improved followed by annual data reprocessing and analysis cycles to generate better products in terms of extended time series and continuously improved data quality. Here we present an overview about the latest GHG-CCI data set called Climate Research Data Package No. 3 (CRDP3) focusing on the GHG-CCI core data products, which are column-averaged dry-air mole fractions of CO2 and CH4, i.e., XCO2 and XCH4, as retrieved from SCIAMACHY/ENVISAT and TANSO/GOSAT satellite radiances covering the time period end of 2002 to end of 2014. We present global maps and time series including initial validation results obtained by comparisons with Total Carbon Column Observing Network (TCCON) ground-based observations. We show that the GCOS requirements for systematic error (< 1 ppm for XCO2, < 10 ppb for XCH4) and long-term stability (< 0.2 ppm/year for XCO2, < 2 ppb/year for XCH4) are met for nearly all products (an exception is SCIAMACHY methane especially since 2010). For XCO2 we present comparisons with global models using the output of two CO2 assimilation systems (MACC version 14r2 and CarbonTracker version CT2013B). We show that overall there is reasonable consistency and agreement between all data sets (within ~ 1–2 ppm) but we also found significant differences depending on region and time period.

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    Remote Sensing of Environment
    Article . 2017 . Peer-reviewed
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    Authors: Ross, A. N.; Wooster, M. J.; Boesch, Hartmut; Parker, Robert;

    Using methane and carbon dioxide atmospheric mixing ratios retrieved using SWIR spectra from the Greenhouse Gases Observing SATellite (GOSAT), we report the first wildfire plume CH4 to CO2 emission ratios (ERCH4/CO2) determined from space. We demonstrate the approach's potential using forward modeling and identify a series of real GOSAT spectra containing wildfire plumes. These show significantly changed total‐column CO2 and CH4 mixing ratios, and from these we calculate ERCH4/CO2 for boreal forest, tropical forest, and savanna fires as 0.00603, 0.00527, and 0.00395 mol mol−1, respectively. These ERs are statistically significantly different from each other and from the “normal” atmospheric CH4 to CO2 ratio and generally agree with past ground and airborne studies.

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    Geophysical Research Letters
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    Geophysical Research Letters
    Article . 2013 . Peer-reviewed
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      Geophysical Research Letters
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    Authors: Mahesh Kumar Sha; Saswati Das; Matthias M. Frey; Darko Dubravica; +53 Authors

    The COllaborative Carbon Column Observing Network has become a reliable source of high-quality ground-based remote sensing network data that provide column-averaged dry-air mole fractions of carbon dioxide (XCO2), methane (XCH4), and carbon monoxide (XCO). The fiducial reference measurements of these gases from the COCCON complement the TCCON and NDACC-IRWG data. This study shows the application of COCCON data for the validation of existing greenhouse gas satellite products. This study includes the validation of XCH4 and XCO products from the European Copernicus Sentinel-5 Precursor (S5P) mission, XCO2 products from the American Orbiting Carbon Observatory-2 (OCO-2) mission, and XCO2 and XCH4 products from the Japanese Greenhouse gases Observing SATellite (GOSAT). A total of 27 datasets contributed to this study; some of these were collected in the framework of campaign activities and covered only a short time period. In addition, several permanent stations provided long-term observations. The random uncertainties in the validation results, specifically for S5P with a lot of coincidences pairs, are found to be similar to the comparison with the TCCON. The comparison results of OCO-2 land nadir and land glint observation modes to the COCCON on a global scale, despite limited coincidences, are very promising. The stations can, therefore, expand on the coverage of the already existing ground-based reference remote sensing sites from the TCCON and the NDACC network. The COCCON data can be used for future satellite and model validation studies and carbon cycle studies.

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    Authors: Yuzhong Zhang; Shuangxi Fang; Jianmeng Chen; Yi Lin; +10 Authors

    China is set to actively reduce its methane emissions in the coming decade. A comprehensive evaluation of the current situation can provide a reference point for tracking the country’s future progress. Here, using satellite and surface observations, we quantify China’s methane emissions during 2010–2017. Including newly available data from a surface network across China greatly improves our ability to constrain emissions at subnational and sectoral levels. Our results show that recent changes in China’s methane emissions are linked to energy, agricultural, and environmental policies. We find contrasting methane emission trends in different regions attributed to coal mining, reflecting region-dependent responses to China’s energy policy of closing small coal mines (decreases in Southwest) and consolidating large coal mines (increases in North). Coordinated production of coalbed methane and coal in southern Shanxi effectively decreases methane emissions, despite increased coal production there. We also detect unexpected increases from rice cultivation over East and Central China, which is contributed by enhanced rates of crop-residue application, a factor not accounted for in current inventories. Our work identifies policy drivers of recent changes in China’s methane emissions, providing input to formulating methane policy toward its climate goal.

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    Proceedings of the National Academy of Sciences
    Article . 2022 . Peer-reviewed
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    https://doi.org/10.5194/egusph...
    Article . 2023 . Peer-reviewed
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    https://dx.doi.org/10.60692/gx...
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    Abstract. China, being one of the major emitters of greenhouse gases, has taken strong actions to tackle climate change, e.g., to achieve carbon neutrality by 2060. It also becomes important to better understand the changes in the atmospheric mixing ratio and emissions of CH4, the second most important human-influenced greenhouse gas, in China. Here we analyze the sources contributing to the atmospheric CH4 mixing ratio and their trends in China over 2007–2018 using the GEOS-Chem model simulations driven by two commonly used global anthropogenic emission inventories: the Emissions Database for Global Atmospheric Research (EDGAR v4.3.2) and the Community Emissions Data System (CEDS). The model results are interpreted with an ensemble of surface, aircraft, and satellite observations of CH4 mixing ratios over China and the Pacific region. The EDGAR and CEDS estimates show considerable differences reflecting large uncertainties in estimates of Chinese CH4 emissions. Chinese CH4 emission estimates based on EDGAR and natural sources increase from 46.7 Tg per annum (Tg a−1) in 1980 to 69.8 Tg a−1 in 2012 with an increase rate of 0.7 Tg a−2, and estimates with CEDS increase from 32.9 Tg a−1 in 1980 and 76.7 Tg a−1 in 2014 (a much stronger trend of 1.3 Tg a−2 over the period). Both surface, aircraft, and satellite measurements indicate CH4 increase rates of 7.0–8.4 ppbv a−1 over China in the recent decade. We find that the model simulation using the CEDS inventory and interannually varying OH levels can best reproduce these observed CH4 mixing ratios and trends over China. Model results over China are sensitive to the global OH level, with a 10 % increase in the global tropospheric volume-weighted mean OH concentration presenting a similar effect to that of a 47 Tg a−1 decrease in global CH4 emissions. We further apply a tagged tracer simulation to quantify the source contributions from different emission sectors and regions. We find that domestic CH4 emissions account for 11.4 % of the mean surface mixing ratio and drive 68.3 % of the surface trend (mainly via the energy sector) in China over 2007–2018. We emphasize that intensive CH4 measurements covering eastern China will help better assess the driving factors of CH4 mixing ratios and support the emission mitigation in China.

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    https://doi.org/10.5194/acp-20...
    Article . 2021 . Peer-reviewed
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    Atmospheric Chemistry and Physics (ACP)
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    https://dx.doi.org/10.60692/72...
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      https://doi.org/10.5194/acp-20...
      Article . 2021 . Peer-reviewed
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      Atmospheric Chemistry and Physics (ACP)
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      https://dx.doi.org/10.60692/72...
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      https://dx.doi.org/10.60692/js...
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      https://dx.doi.org/10.60692/cf...
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      https://dx.doi.org/10.60692/wv...
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