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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Philip Schulz; Judith L. MacManus-Driscoll; Wen Li; Wen Li; +14 Authors

    Thin (approximately 10 nm) oxide buffer layers grown over lead-halide perovskite device stacks are critical for protecting the perovskite against mechanical and environmental damage. However, the limited perovskite stability restricts the processing methods and temperatures (<=110 C) that can be used to deposit the oxide overlayers, with the latter limiting the electronic properties of the oxides achievable. In this work, we demonstrate an alternative to existing methods that can grow pinhole-free TiOx (x = 2.00+/-0.05) films with the requisite thickness in <1 min without vacuum. This technique is atmospheric pressure chemical vapor deposition (AP-CVD). The rapid but soft deposition enables growth temperatures of >=180 ��C to be used to coat the perovskite. This is >=70 ��C higher than achievable by current methods and results in more conductive TiOx films, boosting solar cell efficiencies by >2%. Likewise, when AP-CVD SnOx (x ~ 2) is grown on perovskites, there is also minimal damage to the perovskite beneath. The SnOx layer is pinhole-free and conformal, which reduces shunting in devices, and increases steady-state efficiencies from 16.5% (no SnOx) to 19.4% (60 nm SnOx), with fill factors reaching 84%. This work shows AP-CVD to be a versatile technique for growing oxides on thermally-sensitive materials. R.D.R and R.A.J contributed equally. 23 pages. 6 figures

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Hyper Article en Lig...arrow_drop_down
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Nano Energy
    Article
    Data sources: UnpayWall
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Apollo
    Article . 2020
    Data sources: Datacite
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Hal
    Article . 2020
    Data sources: Hal
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Apollo
    Article . 2020
    Data sources: Apollo
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Nano Energy
    Article . 2020 . Peer-reviewed
    License: Elsevier TDM
    Data sources: Crossref
    https://dx.doi.org/10.48550/ar...
    Article . 2019
    License: arXiv Non-Exclusive Distribution
    Data sources: Datacite
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Hyper Article en Lig...arrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Nano Energy
      Article
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Apollo
      Article . 2020
      Data sources: Datacite
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Hal
      Article . 2020
      Data sources: Hal
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Apollo
      Article . 2020
      Data sources: Apollo
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
      Nano Energy
      Article . 2020 . Peer-reviewed
      License: Elsevier TDM
      Data sources: Crossref
      https://dx.doi.org/10.48550/ar...
      Article . 2019
      License: arXiv Non-Exclusive Distribution
      Data sources: Datacite
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Robert L.Z. Hoye; David Mu�oz-Rojas; Diana C. Iza; Kevin P. Musselman; +1 Authors

    AbstractA thin ZnO (<200nm) film grown by Atmospheric Atomic Layer Deposition (AALD) in a matter of minutes was studied as a hole-blocking layer in poly(3-hexylthiophene-2,5-diyl):[6,6]-phenyl-C61-buyric acid methyl ester (P3HT:PCBM) based inverted solar cells. These AALD ZnO layers were compact, had a high electron mobility of 3.4+0.1cm2/Vs, had up to 100% transmittance to visible light, and a good wettability for the blend. Despite the very rapid, open atmosphere growth method, the cell performance was comparable with some of the best inverted bulk heterojunction P3HT:PCBM cells in the literature. The performance was also maintained after 200 days of storage in air in the dark.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Solar Energy Materia...arrow_drop_down
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Solar Energy Materials and Solar Cells
    Article . 2013 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Solar Energy Materials and Solar Cells
    Article
    License: CC BY
    Data sources: UnpayWall
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Solar Energy Materia...arrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Solar Energy Materials and Solar Cells
      Article . 2013 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Solar Energy Materials and Solar Cells
      Article
      License: CC BY
      Data sources: UnpayWall
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Federico Baiutti; Francesco Chiabrera; Matias Acosta; David Diercks; +9 Authors

    Abstract The implementation of nano-engineered composite oxides opens up the way towards the development of a novel class of superior energy materials. Vertically aligned nanocomposites are characterized by a coherent, dense array of vertical interfaces, which allows for the extension of local effects to the whole volume of the material. Here, we use such a unique architecture to fabricate highly electrochemically active nanocomposites of lanthanum strontium manganite and doped ceria with unprecedented stability and straight applicability as functional layers in solid state energy devices. Direct evidence of synergistic local effects for enhancing the electrochemical performance, stemming from the highly ordered phase alternation, is given here for the first time using atom-probe tomography combined with oxygen isotopic exchange. Interface-induced cationic substitution, enabling lattice stabilization, is presented as the origin of the observed long-term stability. These findings reveal a novel route for materials nano-engineering based on the coexistence between local disorder and long-range arrangement.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Smithsonian figsharearrow_drop_down
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    https://doi.org/10.21203/rs.3....
    Article . 2021 . Peer-reviewed
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    https://doi.org/10.26434/chemr...
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    https://chemrxiv.org/engage/ap...
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Smithsonian figsharearrow_drop_down
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      https://doi.org/10.21203/rs.3....
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      https://doi.org/10.26434/chemr...
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      https://chemrxiv.org/engage/ap...
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    Authors: T. Fix; H. Rinnert; M.G. Blamire; A. Slaoui; +1 Authors

    Abstract We investigate the potential of Nd doped SrTiO3 films for the photon downshifting of ultraviolet photons to infrared ones. We first studied the structural properties of such newly developed layers grown by pulsed laser deposition (PLD). We also show that these layers allow the conversion of photons from 250–350 nm excitation to around 900 nm. We implemented the optimized Nd:SrTiO3 thin films on a conventional silicon solar cell and we show that the internal quantum efficiency is increased at around 350 nm which validates the concept of downshifting applied to solar cells. Future work will be to determine if downconversion takes place in this system.

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    Hyper Article en Ligne
    Conference object . 2011
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    Solar Energy Materials and Solar Cells
    Article . 2012 . Peer-reviewed
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      Solar Energy Materials and Solar Cells
      Article . 2012 . Peer-reviewed
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    Authors: Gan, J; Hoye, R; Ievskaya, Y; Vines, L; +3 Authors

    Heterojunction Cu2O solar cells are an important class of Earth-abundant photovoltaics that can be synthesized by a variety of techniques, including electrochemical deposition (ECD) and thermal oxidation (TO). The latter gives the most efficient solar cells of up to 8.1% reported in the literature, but is limited by low external quantum efficiencies (EQE) in the long wavelength range (490–600 nm). By contrast, ECD Cu2O gives higher short wavelength EQEs of up to 90%. We elucidate the cause of this difference by characterizing and comparing ECD and TO films using impedance spectroscopy and fitting with a lumped circuit model to determine the trap density, followed by simulations. The data indicates that TO Cu2O has a higher density of interface defects, located approximately 0.5 eV above the valence band maximum (NV), and lower bulk defect density thus explaining the lower short wavelength EQEs and higher long wavelength EQEs. This work shows that a route to further efficiency increases of TO Cu2O is to reduce the density of interface defect states.

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    Solar Energy Materials and Solar Cells
    Article . 2020 . Peer-reviewed
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    Solar Energy Materials and Solar Cells
    Article
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    Apollo
    Article . 2020
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Apollo
    Article . 2020
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      Solar Energy Materials and Solar Cells
      Article . 2020 . Peer-reviewed
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      Solar Energy Materials and Solar Cells
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      Apollo
      Article . 2020
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      Apollo
      Article . 2020
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    Authors: Pan, Hao; Jiang, Yizhe; MacManus-Driscoll, Judith L.;
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    Journal of Materiomics
    Article . 2023 . Peer-reviewed
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    Article . 2023
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    Journal of Materiomics
    Article . 2022 . Peer-reviewed
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    http://dx.doi.org/10.1016/j.jm...
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      Journal of Materiomics
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      Article . 2023
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      Journal of Materiomics
      Article . 2022 . Peer-reviewed
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      http://dx.doi.org/10.1016/j.jm...
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    Authors: Ashoka, Arjun; Nagane, Satyawan; Strkalj, Nives; Sharma, Ashish; +7 Authors

    Photoinduced spin-charge interconversion in semiconductors with spin-orbit coupling could provide a route to optically addressable spintronics without the use of external magnetic fields. However, in structurally disordered polycrystalline semiconductors, which are being widely explored for device applications, the presence and role of spin-associated charge currents remains unclear. Here, using femtosecond circular-polarization-resolved pump-probe microscopy on polycrystalline halide perovskite thin films, we observe the photoinduced ultrafast formation of spin domains on the micrometre scale formed through lateral spin currents. Micrometre-scale variations in the intensity of optical second-harmonic generation and vertical piezoresponse suggest that the spin-domain formation is driven by the presence of strong local inversion symmetry breaking via structural disorder. We propose that this leads to spatially varying Rashba-like spin textures that drive spin-momentum-locked currents, leading to local spin accumulation. Ultrafast spin-domain formation in polycrystalline halide perovskite films provides an optically addressable platform for nanoscale spin-device physics.

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    Apollo
    Article . 2023
    License: CC BY
    Data sources: Datacite
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    Apollo
    Article . 2023
    License: CC BY
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    Science Advances
    Article . 2023 . Peer-reviewed
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Nature Materials
    Article . 2023 . Peer-reviewed
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    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Nature Materials
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    Nature Materials
    Article . 2023 . Peer-reviewed
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      Apollo
      Article . 2023
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      Apollo
      Article . 2023
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      Science Advances
      Article . 2023 . Peer-reviewed
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      Nature Materials
      Article . 2023 . Peer-reviewed
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      Nature Materials
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      Nature Materials
      Article . 2023 . Peer-reviewed
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    Authors: Ampattu R. Jayakrishnan; Ji S. Kim; Markus Hellenbrand; Luís S. Marques; +2 Authors

    Ferroelectric memory devices such as ferroelectric memristors, ferroelectric tunnel junctions, and field-effect transistors are considered among the most promising candidates for neuromorphic computing devices.

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    Materials Horizons
    Article . 2024 . Peer-reviewed
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    PubMed Central
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    Apollo
    Article . 2024
    License: CC BY
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    Materials Horizons
    Article . 2024 . Peer-reviewed
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      Materials Horizons
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      Apollo
      Article . 2024
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      Materials Horizons
      Article . 2024 . Peer-reviewed
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Hoye, Robert L. Z.; Hidalgo, Juanita; Jagt, Robert A.; Correa‐Baena, Juan‐Pablo; +2 Authors

    AbstractHalide perovskite semiconductors have risen to prominence in photovoltaics and light‐emitting diodes (LEDs), but traditional oxide perovskites, which overcome the stability limitations of their halide counterparts, have also recently witnessed a rise in potential as solar absorbers. One of the many important factors underpinning these developments is an understanding of the role of dimensionality on the optoelectronic properties and, consequently, on the performance of the materials in photovoltaics and LEDs. This review article examines the role of structural and electronic dimensionality, as well as form factor, in oxide and halide perovskites, and in lead‐free alternatives to halide perovskites. Insights into how dimensionality influences the band gap, stability, charge‐carrier transport, recombination processes and defect tolerance of the materials, and the impact these parameters have on device performance are brought forward. Particular emphasis is placed on carrier/exciton‐phonon coupling, which plays a significant role in the materials considered, owing to their soft lattices and composition of heavy elements, and becomes more prominent as dimensionality is reduced. It is finished with a discussion of the implications on the classes of materials future efforts should focus on, as well as the key questions that need to be addressed.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Advanced Energy Mate...arrow_drop_down
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Advanced Energy Materials
    Article . 2021 . Peer-reviewed
    License: CC BY
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    Advanced Energy Materials
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    Apollo
    Article . 2022
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    Apollo
    Article . 2021
    Data sources: Datacite
    Advanced Energy Materials
    Article . 2021 . Peer-reviewed
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      Advanced Energy Materials
      Article . 2021 . Peer-reviewed
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      Advanced Energy Materials
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      Apollo
      Article . 2022
      Data sources: Apollo
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Apollo
      Article . 2021
      Data sources: Datacite
      Advanced Energy Materials
      Article . 2021 . Peer-reviewed
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    Authors: Jayakrishnan, Ampattu Ravikumar; Silva, José Pedro Basto; Gwozdz, Katarzyna; Gomes, M. J. M.; +2 Authors

    Self-powered photodetectors are advantageous over conventional photodetectors because they can have outstanding performance in the absence of an external power source, which is important for a range of applications, including in the Internet of Things. Current research has demonstrated different types of self-powered photodetectors utilizing the photovoltaic effect, pyroelectric effect, piezoelectric effect, and synergic effects, such as the piezo-phototronic and pyro-phototronic effects. Such effects have been demonstrated in standard semiconductors, in hybrid inorganic-organic halide perovskites and in all inorganic perovskites. Very recently, a novel type of self-powered photodetector exploring the coupling between the photovoltaic, the pyroelectric and the ferroelectric effects (i.e., ferro-pyro-phototronic effect) has attracted great interest, owing to the excellent photo current response achieved with this triple coupling. The ferro-pyro-phototronic effect can therefore be an important route towards improving the performance of self-powered photodetectors. Since ferroelectricity has the potential to bring revolutionary changes in many contemporary technologies, including non-volatile memory, solar cells, field effect transistors, energy storage, and energy harvesters, it is worthwhile exploring in more detail how the ferroelectric effect enhances the triple coupling. Thus, this focus review covers the research conducted so far on the ferro-pyro-phototronic effect, discussing recent progress on the development of self-powered photodetectors based on this effect, and also highlighting current challenges and potential solutions for using these devices in real-world applications. This work was supported by: (i) the Portuguese Foundation for Science and Technology (FCT) in the framework of the Strategic Funding Contracts UIDB/04650/2020, (ii) exploratory project 2022.01740. PDTC and (iii) the project M-ERA-NET3/0003/2021 - NanOx4EStor grant agreement No 958174 (https://doi.org/10.54499/M-ERA-NET3/0003/2021). J. P. B. S. also thanks FCT for the contract under the Institutional Call to Scientific Employment Stimulus – 2021 Call (CEECINST/00018/2021). JLM-D. and R.L.Z.H. thank EPSRC CAM-IES grant EP/P007767/. R.L.Z.H. also acknowledges support from the Royal Academy of Engineering under the Research Fellowships scheme (No.: RF\201718\1701). J.L.M-D. acknowledges support from the Royal Academy of Engineering Chair in Emerging Technologies scheme (No.: CIET1819_24) and the ERC Advanced Grant, ERC-ADG #882929 EROS. K. G. acknowledges support from the National Science Centre in Poland Grant No. 2023/07/X/ST7/00073.

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    Nano Energy
    Article . 2023 . Peer-reviewed
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    Universidade do Minho: RepositoriUM
    Other literature type . 2023
    License: CC BY NC ND
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      Nano Energy
      Article . 2023 . Peer-reviewed
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      Universidade do Minho: RepositoriUM
      Other literature type . 2023
      License: CC BY NC ND
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Philip Schulz; Judith L. MacManus-Driscoll; Wen Li; Wen Li; +14 Authors

    Thin (approximately 10 nm) oxide buffer layers grown over lead-halide perovskite device stacks are critical for protecting the perovskite against mechanical and environmental damage. However, the limited perovskite stability restricts the processing methods and temperatures (<=110 C) that can be used to deposit the oxide overlayers, with the latter limiting the electronic properties of the oxides achievable. In this work, we demonstrate an alternative to existing methods that can grow pinhole-free TiOx (x = 2.00+/-0.05) films with the requisite thickness in <1 min without vacuum. This technique is atmospheric pressure chemical vapor deposition (AP-CVD). The rapid but soft deposition enables growth temperatures of >=180 ��C to be used to coat the perovskite. This is >=70 ��C higher than achievable by current methods and results in more conductive TiOx films, boosting solar cell efficiencies by >2%. Likewise, when AP-CVD SnOx (x ~ 2) is grown on perovskites, there is also minimal damage to the perovskite beneath. The SnOx layer is pinhole-free and conformal, which reduces shunting in devices, and increases steady-state efficiencies from 16.5% (no SnOx) to 19.4% (60 nm SnOx), with fill factors reaching 84%. This work shows AP-CVD to be a versatile technique for growing oxides on thermally-sensitive materials. R.D.R and R.A.J contributed equally. 23 pages. 6 figures

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    Apollo
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    Nano Energy
    Article . 2020 . Peer-reviewed
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      Nano Energy
      Article . 2020 . Peer-reviewed
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    Authors: Robert L.Z. Hoye; David Mu�oz-Rojas; Diana C. Iza; Kevin P. Musselman; +1 Authors

    AbstractA thin ZnO (<200nm) film grown by Atmospheric Atomic Layer Deposition (AALD) in a matter of minutes was studied as a hole-blocking layer in poly(3-hexylthiophene-2,5-diyl):[6,6]-phenyl-C61-buyric acid methyl ester (P3HT:PCBM) based inverted solar cells. These AALD ZnO layers were compact, had a high electron mobility of 3.4+0.1cm2/Vs, had up to 100% transmittance to visible light, and a good wettability for the blend. Despite the very rapid, open atmosphere growth method, the cell performance was comparable with some of the best inverted bulk heterojunction P3HT:PCBM cells in the literature. The performance was also maintained after 200 days of storage in air in the dark.

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    Solar Energy Materials and Solar Cells
    Article . 2013 . Peer-reviewed
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    Solar Energy Materials and Solar Cells
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      Solar Energy Materials and Solar Cells
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    Authors: Federico Baiutti; Francesco Chiabrera; Matias Acosta; David Diercks; +9 Authors

    Abstract The implementation of nano-engineered composite oxides opens up the way towards the development of a novel class of superior energy materials. Vertically aligned nanocomposites are characterized by a coherent, dense array of vertical interfaces, which allows for the extension of local effects to the whole volume of the material. Here, we use such a unique architecture to fabricate highly electrochemically active nanocomposites of lanthanum strontium manganite and doped ceria with unprecedented stability and straight applicability as functional layers in solid state energy devices. Direct evidence of synergistic local effects for enhancing the electrochemical performance, stemming from the highly ordered phase alternation, is given here for the first time using atom-probe tomography combined with oxygen isotopic exchange. Interface-induced cationic substitution, enabling lattice stabilization, is presented as the origin of the observed long-term stability. These findings reveal a novel route for materials nano-engineering based on the coexistence between local disorder and long-range arrangement.

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    https://doi.org/10.21203/rs.3....
    Article . 2021 . Peer-reviewed
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    https://doi.org/10.26434/chemr...
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    https://chemrxiv.org/engage/ap...
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    Authors: T. Fix; H. Rinnert; M.G. Blamire; A. Slaoui; +1 Authors

    Abstract We investigate the potential of Nd doped SrTiO3 films for the photon downshifting of ultraviolet photons to infrared ones. We first studied the structural properties of such newly developed layers grown by pulsed laser deposition (PLD). We also show that these layers allow the conversion of photons from 250–350 nm excitation to around 900 nm. We implemented the optimized Nd:SrTiO3 thin films on a conventional silicon solar cell and we show that the internal quantum efficiency is increased at around 350 nm which validates the concept of downshifting applied to solar cells. Future work will be to determine if downconversion takes place in this system.

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    Conference object . 2011
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    Solar Energy Materials and Solar Cells
    Article . 2012 . Peer-reviewed
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      Solar Energy Materials and Solar Cells
      Article . 2012 . Peer-reviewed
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    Authors: Gan, J; Hoye, R; Ievskaya, Y; Vines, L; +3 Authors

    Heterojunction Cu2O solar cells are an important class of Earth-abundant photovoltaics that can be synthesized by a variety of techniques, including electrochemical deposition (ECD) and thermal oxidation (TO). The latter gives the most efficient solar cells of up to 8.1% reported in the literature, but is limited by low external quantum efficiencies (EQE) in the long wavelength range (490–600 nm). By contrast, ECD Cu2O gives higher short wavelength EQEs of up to 90%. We elucidate the cause of this difference by characterizing and comparing ECD and TO films using impedance spectroscopy and fitting with a lumped circuit model to determine the trap density, followed by simulations. The data indicates that TO Cu2O has a higher density of interface defects, located approximately 0.5 eV above the valence band maximum (NV), and lower bulk defect density thus explaining the lower short wavelength EQEs and higher long wavelength EQEs. This work shows that a route to further efficiency increases of TO Cu2O is to reduce the density of interface defect states.

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    Solar Energy Materials and Solar Cells
    Article . 2020 . Peer-reviewed
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    Solar Energy Materials and Solar Cells
    Article
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    Apollo
    Article . 2020
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    Apollo
    Article . 2020
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      Solar Energy Materials and Solar Cells
      Article . 2020 . Peer-reviewed
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      Solar Energy Materials and Solar Cells
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      Apollo
      Article . 2020
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      Article . 2020
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    Authors: Pan, Hao; Jiang, Yizhe; MacManus-Driscoll, Judith L.;
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    Journal of Materiomics
    Article . 2023 . Peer-reviewed
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    Article . 2023
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    Journal of Materiomics
    Article . 2022 . Peer-reviewed
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    http://dx.doi.org/10.1016/j.jm...
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      Journal of Materiomics
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      Journal of Materiomics
      Article . 2022 . Peer-reviewed
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      http://dx.doi.org/10.1016/j.jm...
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    Authors: Ashoka, Arjun; Nagane, Satyawan; Strkalj, Nives; Sharma, Ashish; +7 Authors

    Photoinduced spin-charge interconversion in semiconductors with spin-orbit coupling could provide a route to optically addressable spintronics without the use of external magnetic fields. However, in structurally disordered polycrystalline semiconductors, which are being widely explored for device applications, the presence and role of spin-associated charge currents remains unclear. Here, using femtosecond circular-polarization-resolved pump-probe microscopy on polycrystalline halide perovskite thin films, we observe the photoinduced ultrafast formation of spin domains on the micrometre scale formed through lateral spin currents. Micrometre-scale variations in the intensity of optical second-harmonic generation and vertical piezoresponse suggest that the spin-domain formation is driven by the presence of strong local inversion symmetry breaking via structural disorder. We propose that this leads to spatially varying Rashba-like spin textures that drive spin-momentum-locked currents, leading to local spin accumulation. Ultrafast spin-domain formation in polycrystalline halide perovskite films provides an optically addressable platform for nanoscale spin-device physics.

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    Apollo
    Article . 2023
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    Apollo
    Article . 2023
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    Science Advances
    Article . 2023 . Peer-reviewed
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    Nature Materials
    Article . 2023 . Peer-reviewed
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    Nature Materials
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    Nature Materials
    Article . 2023 . Peer-reviewed
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      Apollo
      Article . 2023
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      Apollo
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      Science Advances
      Article . 2023 . Peer-reviewed
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      Nature Materials
      Article . 2023 . Peer-reviewed
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      Nature Materials
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      Nature Materials
      Article . 2023 . Peer-reviewed
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    Authors: Ampattu R. Jayakrishnan; Ji S. Kim; Markus Hellenbrand; Luís S. Marques; +2 Authors

    Ferroelectric memory devices such as ferroelectric memristors, ferroelectric tunnel junctions, and field-effect transistors are considered among the most promising candidates for neuromorphic computing devices.

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    Materials Horizons
    Article . 2024 . Peer-reviewed
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    Apollo
    Article . 2024
    License: CC BY
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    Materials Horizons
    Article . 2024 . Peer-reviewed
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      Materials Horizons
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      PubMed Central
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      Apollo
      Article . 2024
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      Materials Horizons
      Article . 2024 . Peer-reviewed
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    Authors: Hoye, Robert L. Z.; Hidalgo, Juanita; Jagt, Robert A.; Correa‐Baena, Juan‐Pablo; +2 Authors

    AbstractHalide perovskite semiconductors have risen to prominence in photovoltaics and light‐emitting diodes (LEDs), but traditional oxide perovskites, which overcome the stability limitations of their halide counterparts, have also recently witnessed a rise in potential as solar absorbers. One of the many important factors underpinning these developments is an understanding of the role of dimensionality on the optoelectronic properties and, consequently, on the performance of the materials in photovoltaics and LEDs. This review article examines the role of structural and electronic dimensionality, as well as form factor, in oxide and halide perovskites, and in lead‐free alternatives to halide perovskites. Insights into how dimensionality influences the band gap, stability, charge‐carrier transport, recombination processes and defect tolerance of the materials, and the impact these parameters have on device performance are brought forward. Particular emphasis is placed on carrier/exciton‐phonon coupling, which plays a significant role in the materials considered, owing to their soft lattices and composition of heavy elements, and becomes more prominent as dimensionality is reduced. It is finished with a discussion of the implications on the classes of materials future efforts should focus on, as well as the key questions that need to be addressed.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Advanced Energy Mate...arrow_drop_down
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Advanced Energy Materials
    Article . 2021 . Peer-reviewed
    License: CC BY
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    Advanced Energy Materials
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    License: CC BY
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    Apollo
    Article . 2022
    Data sources: Apollo
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Apollo
    Article . 2021
    Data sources: Datacite
    Advanced Energy Materials
    Article . 2021 . Peer-reviewed
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      Advanced Energy Materials
      Article . 2021 . Peer-reviewed
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      Apollo
      Article . 2022
      Data sources: Apollo
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Apollo
      Article . 2021
      Data sources: Datacite
      Advanced Energy Materials
      Article . 2021 . Peer-reviewed
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    Authors: Jayakrishnan, Ampattu Ravikumar; Silva, José Pedro Basto; Gwozdz, Katarzyna; Gomes, M. J. M.; +2 Authors

    Self-powered photodetectors are advantageous over conventional photodetectors because they can have outstanding performance in the absence of an external power source, which is important for a range of applications, including in the Internet of Things. Current research has demonstrated different types of self-powered photodetectors utilizing the photovoltaic effect, pyroelectric effect, piezoelectric effect, and synergic effects, such as the piezo-phototronic and pyro-phototronic effects. Such effects have been demonstrated in standard semiconductors, in hybrid inorganic-organic halide perovskites and in all inorganic perovskites. Very recently, a novel type of self-powered photodetector exploring the coupling between the photovoltaic, the pyroelectric and the ferroelectric effects (i.e., ferro-pyro-phototronic effect) has attracted great interest, owing to the excellent photo current response achieved with this triple coupling. The ferro-pyro-phototronic effect can therefore be an important route towards improving the performance of self-powered photodetectors. Since ferroelectricity has the potential to bring revolutionary changes in many contemporary technologies, including non-volatile memory, solar cells, field effect transistors, energy storage, and energy harvesters, it is worthwhile exploring in more detail how the ferroelectric effect enhances the triple coupling. Thus, this focus review covers the research conducted so far on the ferro-pyro-phototronic effect, discussing recent progress on the development of self-powered photodetectors based on this effect, and also highlighting current challenges and potential solutions for using these devices in real-world applications. This work was supported by: (i) the Portuguese Foundation for Science and Technology (FCT) in the framework of the Strategic Funding Contracts UIDB/04650/2020, (ii) exploratory project 2022.01740. PDTC and (iii) the project M-ERA-NET3/0003/2021 - NanOx4EStor grant agreement No 958174 (https://doi.org/10.54499/M-ERA-NET3/0003/2021). J. P. B. S. also thanks FCT for the contract under the Institutional Call to Scientific Employment Stimulus – 2021 Call (CEECINST/00018/2021). JLM-D. and R.L.Z.H. thank EPSRC CAM-IES grant EP/P007767/. R.L.Z.H. also acknowledges support from the Royal Academy of Engineering under the Research Fellowships scheme (No.: RF\201718\1701). J.L.M-D. acknowledges support from the Royal Academy of Engineering Chair in Emerging Technologies scheme (No.: CIET1819_24) and the ERC Advanced Grant, ERC-ADG #882929 EROS. K. G. acknowledges support from the National Science Centre in Poland Grant No. 2023/07/X/ST7/00073.

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    Nano Energy
    Article . 2023 . Peer-reviewed
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    Universidade do Minho: RepositoriUM
    Other literature type . 2023
    License: CC BY NC ND
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      Nano Energy
      Article . 2023 . Peer-reviewed
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      Universidade do Minho: RepositoriUM
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