• Energy Research
• 2016-2025close
• Chinese Academy of Sciences close

Abstract. Regional land carbon budgets provide insights on the spatial distribution of the land uptake of atmospheric carbon dioxide, and can be used to evaluate carbon cycle models and to define baselines for land-based additional mitigation efforts. The scientific community has been involved in providing observation-based estimates of regional carbon budgets either by downscaling atmospheric CO2 observations into surface fluxes with atmospheric inversions, by using inventories of carbon stock changes in terrestrial ecosystems, by upscaling local field observations such as flux towers with gridded climate and remote sensing fields or by integrating data-driven or process-oriented terrestrial carbon cycle models. The first coordinated attempt to collect regional carbon budgets for nine regions covering the entire globe in the RECCAP-1 project has delivered estimates for the decade 2000–2009, but these budgets were not comparable between regions, due to different definitions and component fluxes reported or omitted. The recent recognition of lateral fluxes of carbon by human activities and rivers, that connect CO2 uptake in one area with its release in another also requires better definition and protocols to reach harmonized regional budgets that can be summed up to the globe and compared with the atmospheric CO2 growth rate and inversion results. In this study, for the international initiative RECCAP-2 coordinated by the Global Carbon Project, which aims as an update of regional carbon budgets over the last two decades based on observations, for 10 regions covering the globe, with a better harmonization that the precursor project, we provide recommendations for using atmospheric inversions results to match bottom-up carbon accounting and models, and we define the different component fluxes of the net land atmosphere carbon exchange that should be reported by each research group in charge of each region. Special attention is given to lateral fluxes, inland water fluxes and land use fluxes.

Forest soil acidification caused by acid deposition is a serious threat to the forest ecosystem. To investigate the liming effects of biomass ash (BA) and alkaline slag (AS) on the acidic topsoil and subsoil, a three-year field experiment under artificial Masson pine was conducted at Langxi, Anhui province in Southern China. The surface application of BA and AS significantly increased the soil pH, and thus decreased exchangeable acidity and active Al in the topsoil. Soil exchangeable Ca2+ and Mg2+ in topsoil were significantly increased by the surface application of BA and AS, while an increase in soil exchangeable K+ was only observed in BA treatments. The soil acidity and active Al in subsoil were decreased by the surface application of AS. Compared with the control, soluble monomeric and exchangeable Al in the subsoil was decreased by 38.0% and 29.4% after 3 years of AS surface application. There was a minimal effect on soluble monomeric and exchangeable Al after the application of BA. The soil exchangeable Ca2+ and Mg2+ in the subsoil increased respectively by 54% and 141% after surface application of 10 t ha-1 AS. The decrease of soil active Al and increase of base cations in subsoil were mainly attributed to the high migration capacity of base cations in AS. In conclusion, the effect of surface application of AS was superior to BA in ameliorating soil acidity and alleviating soil Al toxicity in the subsoil of this Ultisol.

Bioenergy is considered a sustainable substitute to fossil-fuel resources and the development of a prudent combination of renewable and innovative conversion technologies are essential for the valorization and effective conversion of biowaste to value-added commodities. Here, a negative pressure-induced carbonization process was proposed for the valorization of lignin-enriched biowaste precursor to bio-oil and environmental materials (biochar) at various temperatures. The high heating values (HHV) of the as-prepared biochars from the lignin enriched precursor under negative pressure (low-medium vacuum) were within 25.9-31.5 MJ/kg, which matched satisfactorily to the commercial charcoal. Whereas, the bio-oils produced from the lignin enriched precursor under vacuum conditions was a blend of complex aromatic and straight-chain hydro-carbons, including aldehyde, ketone, phenol, and furans, exhibiting ability as potential heating-oil with HHV within 21.2-28.2 MJ/kg. Moreover, the biochars produced under vacuum environments at higher temperature showed greater stability (22.5-35.9%) than those produced under N2 atmosphere.

Abstract The Liquefied natural gas (LNG) cryogenic submerged pump, the core power equipment for the transportation of liquefied natural gas, is prone to cavitation. However, based on the traditional analysis of the pressure drop, the irreversible loss after cavitation can barely be displayed quantitatively. To solve this problem, an entropy production diagnostic model (EPDM) by the contribution of viscous entropy production (VEP), turbulent entropy production (TEP) and wall entropy production (WEP) for the cavitation flow was established to calculate the energy loss. The cryogenic cavitation model and proposed EPDM were proved to be reliable after comparing results with Hord’s experiment in an ogive and cavitation experiment in a centrifugal pump. Then, by studying the total entropy production, it was found that the EPDM could well predict the occurrence of the critical cavitation and the deterioration of cavitation. When compared with TEP and WEP, the effect of VEP is negligible. As the cavitation area expands from the suction surface of inducer (id) to the first-stage impeller (impA), the cavitation process can be divided into three stages and the total energy loss increases significantly from the first stage to the third one. Through the global distribution of energy loss, it was found that the faster growth of the loss in the second-stage impeller (impB) and the second-stage guide vane (gvB), not in id and impA, contributes more to the energy loss after cavitation. Finally, from the variation of ratio of TEP to WEP, it reveals that cavitation has a greater effect on the WEP rate for the impB, but the turbulent viscous dissipation is still dominant, while the eddy dissipation and resistance loss in gvB with the evolution of cavitation are both crucial.

Abstract This paper presents a novel and environmentally friendly production of direct reduced iron (DRI) technology using biomass as an additive agent in iron ore pellets and simulated biomass-derived syngas as the reducing agent. The effects of biomass addition on iron ore pellets reduction and consequent reduction kinetics in simulated biomass-derived syngas atmosphere were investigated. The results demonstrated that the biomass addition improved the pellet porosity and specific surface area, thus increasing both the reducibility and reduction rate and decreasing the apparent activation energy for pellet reduction. Mathematical modelling of experimental data indicated an interfacial chemical reaction mechanism with FeO → Fe as the rate controlling step. The simulated biomass syngas is an alternative gas-based reductant to natural gas, coal gas, more than 99.5% reduction degree of the oxidized pellets was reduced at 1323 K within 20 min. The apparent activation energies were 86.05 kJ·mol −1 , 97.53 kJ·mol −1 for the pellets with and without biomass addition. The proposed iron ore reduction process therefore would be a potential to reduce iron directly using biomass with high efficiency and real environmental benefits.

Abstract A high-flux solar simulator is essential for evaluating solar thermal components under controlled and adjustable flux input conditions. This study presents a newly built high-flux solar simulator composed of 19 individual units. Each unit includes a xenon short-arc lamp (each consuming up to 6 kW electricity power) coupled with a truncated ellipsoidal reflector, a cooling blower, and a power module. The power module yields a current in the range of 50–160 A. The number of lamps in use is flexible, which allows for a wide range of radiation flux (10%–100%) on the focal plane. The radiation power, peak value, flux distribution on the circular target plane, and conversion efficiency are evaluated based on a flux mapping method. The results indicate that the proposed solar simulator is capable of achieving thermal power of 23.3 kW, peak flux in excess of 1.78 MW/m2, a stagnation temperature exceeding 2360 °C, and average irradiance of 773.4 kW/m2 on the focal plane (diameter of 260 mm). The electro-thermal conversion efficiency of the simulator is 35.7%. A ray-tracing method was employed, and the simulation results were found to be in good agreement with those in the experiments. An experimental test of a volumetric ceramic receiver was conducted, and the results indicate the availability and applicability of the high-flux solar simulator when carrying out studies about solar receivers.

Abstract The absorption refrigeration system driven by low grade heat sources, especially the waste heat sources, becomes more and more attractive in recent decades. However, most traditional absorption systems cannot achieve a high utilization rate of the waste heat with limited heat capacity. These systems are usually designed to obtain heat in the generator, which means that the waste heat sources cannot be utilized to the temperature lower than the generator temperature. This paper proposed a new structure heated by heat conduction oil in the generator and electric heating rings around the stripping section. This structure can simulate the temperature-distributed heat sources when the electric heating rings work. It can also simulate a traditional generator when the electric heating rings do not work. Influences of different heat distributions are analyzed in detail in this paper. The results show that the heat sources utilization rate will increase with the increase of the heat in the stripping section, while the coefficient of performance will be negatively affected by the increasing heat in the stripping section. By optimizing the heating structure, the coefficient of performance can be similar to that of a traditional system when the heat is just added in the middle and lower part of stripping section. The optimum utilization rate of heat sources in this test model can reach 1.8 times to that of a traditional system. Under this heating model, the lowest temperature required in the heating section is 82 °C when the heat conduction oil inlet temperature is 169 °C. It is much lower than the temperature inside the generator, which is 137.3 °C.