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In this work, the impact of exogenous aerobic bacteria mixture (EABM) on municipal solid waste (MSW) is well evaluated in the following aspects: biogas production, leachate analysis, organic waste degradation, EABM population, and the composition of microbial communities. The study was designed and performed as follows: the control bioreactor (R1) was filled up with MSW and the culture medium of EABM and the experimental bioreactor (R2) was filled up with MSW and EABM. The data suggests that the composition of microbial communities (bacterial and methanogenic) in R1 and R2 were similar at day 0, while the addition of EABM in R2 led to a differential abundance of Bacillus cereus, Bacillus subtilis, Staphylococcus saprophyticus, Staphlyoccus xylosus, and Pantoea agglomerans in two bioreactors. The population of exogenous aerobic bacteria in R2 greatly increased during hydrolysis and acidogenesis stages, and subsequently increased the degradation of volatile solid (VS), protein, lipid, and lignin by 59.25%, 25.68%, 60.47%, and 197.62%, respectively, compared to R1. The duration of hydrolysis and acidogenesis in R2 was 33.33% shorter than that in R1. At the end of the study, the accumulative methane yield in R2 (494.4 L) was almost three times more than that in R1 (187.4 L). In addition, the abundance of acetoclasic methanogens increased at acetogenesis and methanogenesis stages in both bioreactors, which indicates that acetoclasic methanogens (especially Methanoseata) could contribute to methane production. This study demonstrates that EABM can accelerate organic waste degradation to promote MSW biodegradation and methane production. Moreover, the operational parameters helped EABM to generate 20.85% more in accumulative methane yield. With a better understanding of how EABM affects MSW and the composition of bacterial community, this study offers a potential practical approach to MSW disposal and cleaner energy generation worldwide.

Promoting biodiesel industrialization is not only an important measure in addressing the energy crisis and global warming but is also a driver for industrial restructuring and rural development. To...

AbstractCellulose and lignin nanoparticles are high‐value‐added products obtained from lignocellulosic biomasses through several steps of cellulose purification and lignin extraction. These steps drastically reduce the potential feedstock revenue when carried out as stand‐alone methodologies. To increase biomass yields, we describe here a strategy to design a biorefinery focused on producing cellulose and lignin nanoparticles as main products, but also aim to recover and benefit from other biomass components using only water‐based processes. Sequential pressurized liquid extractions and diluted acid and alkaline treatments were carried out to fractionate elephant grass biomass, yielding (for every 100 g of biomass): 30 g of cellulose pulp (converted to 9 g of cellulose nanocrystals and 9 g of cellulose nanofibers); 10 g of lignin (used to produce 8.5 g of stable colloidal lignin nanoparticles by probe‐sonication in water); 7.5 g of extractives (e.g. sterols and phenolics) and 23 g of xylose (converted to 4.1 g of furfural). Alternatively, to allow for the flexible use of the cellulose fraction in the proposed biorefinery, 22 g of glucose could be produced by enzymatic hydrolysis. The results demonstrate that water‐based processes are suitable for a holistic use of biomass, providing a comprehensive set of high‐value‐added co‐products that are renewable and cost‐effective chemical, cosmetic, food, polymer and pharmaceutical solutions.

Abstract Gasification has been increasingly seen as a method to convert solid fuel into combustible syngas. However, these applications require syngas with strict requirements and raw syngas often does not meet these requirements. Therefore, a form of syngas upgrading needs to be applied. One of the most common form of syngas upgrading is removal of CO2, which is often present in large concentrations in raw syngas. The currently existing CO2 removal technologies were either designed not with syngas in mind or for large scale industries, which makes them somewhat inefficient for application with gasification syngas. This calls for more research into efficient removal of CO2, from syngas. In this review, the application of deep eutectic solvent (DES) as one of the potential new absorbent for CO2 removal from gas streams and more specifically from syngas are discussed. DES has garnered attention due to its high CO2 absorption performance, process friendliness, and environmental friendliness. At present, most studies on DES are still limited to basic absorption behavior of the absorbent. This review aims to provide not just a clear picture of the current research situation for DES as CO2 removal absorbent, but also detail the possible research directions that might be taken for the development of DES as CO2 absorbent from syngas. To that end, this paper shall discuss the specific situation of gasification development, syngas utilization, and the current DES research situation including: its advantages compared to conventional absorbents, its current research situation, challenges, and possible future research directions.

Coal will continue to be the main energy source in China for the immediate future, although the environmental pollution and ecological impacts of each stage in the full life cycle of coal mining, transportation, and combustion generate large quantities of external costs. The Late Permian coals in southwestern (SW) China usually contain high amounts of fluorine (F), arsenic (As), and ash, which together with high-F clays cause abnormally high levels of endemic fluorosis, As poisoning, and lung cancer in areas where coal is mined and burned. In this paper, we estimate the external costs of the life cycle of coal. The results show that the externalities of coal in SW China are estimated at USD 73.5 billion or 284.3 USD/t, which would have accounted for 6.5 % of the provincial GDP in this area in 2018. The external cost of human health accounts for 87.2% of the total external costs, of which endemic skeletal fluorosis diseases and related lung cancers have the most important impact. Our study provides a more precise estimate of externalities compared with its counterparts in other provinces in China. Therefore, several policy recommendations would be proposed to internalize the external cost.

Abstract In the past, most studies considered solar as a drawback to road pavement, especially the asphalt pavement. Not only its radiation causes the asphalt aging, simultaneously with high temperature, asphalt pavement contributes to the urban heat island (UHI) effect. In recent, as the world becomes more supportive towards implementing sustainable energy as the alternatives to the scarcity of non-renewable resources, utilizing the abundant solar radiation as the main source of energy has gradually attracted attention from both industries and academia with its potentials, including solar application on roads. Nevertheless, more researches have focused on the potential energy collection with less consideration to simultaneously overcome the side effects of abundant solar radiation on its lifecycle. This study found the necessity to review a comprehensive correlation between solar radiation and asphalt pavement from both positive and negative effects. The negative effects included asphalt aging and its effects on surroundings i.e. UHI effect. Meanwhile, the positive effects included exhaust purification and solar energy conversion into other forms of energy that can be used by humans using pavement solar heat collection for winter snowmelt, thermoelectric technology and photoelectric technology to convert solar energy into electrical energy. The cases in various application scenarios were analysed and summarized and the existing problems in the current research were proposed in this paper. Also, the reflection on the transformation of road design concept from “avoiding harm” to “seeking profit” was included. Finally, a new concept of “solar-road harmonious symbiosis” for future road application was proposed based on a comprehensive review of previous published works. It is also the new suggestion to scholars on the treatment of solar diseases on roads to prolong its symbiosis functions.

How environmental regulations affect the transfer of pollution-intensive industries is the core issue of balanced regional development and pollution reduction in China. This paper analyses the theoretical mechanism of the impact of environmental regulation on industrial transfer based on the distinction between formal environmental regulation and informal environmental regulation. To this aim, the paper selects panel data of 30 provinces in China from 2008 to 2018 and uses the fixed effect econometric model to test the impact of environmental regulation on the transfer of pollution-intensive industries, then uses a threshold regression model to study the threshold characteristics and spatial heterogeneity of environmental regulation on pollution-intensive industrial transfer. The results show a significant inverted U-shaped relationship between formal environmental regulation and the transfer of pollution-intensive industries. The increase of formal environmental regulation intensity affects restraining and then promoting the transfer out of pollution-intensive industries. The promoting effect also shows the characteristics of first increasing and then decreasing, verifying that there are threshold characteristics and spatial heterogeneity. Overall, informal environmental regulation promotes the transfer of pollution-intensive industries and shows the informal regulation’s economic effect. The paper then puts forward the corresponding policy suggestions, including utilizing clean energy-saving technologies in the industrial sector, which is incredibly significant to realize the coordinated development of environmental protection and economy.

Volatile organic compounds (VOCs) can lead to environmental pollution and threaten human health due to their toxic and carcinogenic nature. The emission of VOCs increases dramatically with the accelerated industrialization and economic growth. Adsorption is identified as one of the most promising recovery technologies owing to its cost-effectiveness, flexible operation, and low energy consumption. In particular, adsorption-based technologies have a high potential to recycle both adsorbents and adsorbates, typically to capture valuable aromatic VOCs from industrial exhaust. Porous materials such as carbon-based materials, zeolite-based materials, and organic polymers and their composites have been extensively developed for VOCs adsorption focusing in adsorption capacity, hydrophobic property, thermal stability and regenerability. Among them, porous carbons as VOCs adsorbents have attracted increasingly attention, because they can be regulated by tuning the pore structure for VOCs accessibility during the adsorption process. Moreover, porous carbons can adsorb target VOCs by controlling the pore structure and surface functional groups. Significantly, the pore size distribution of porous carbons mostly controls the VOCs sorption process. Micropores provide the main adsorption sites, while mesopores enhance the diffusion of VOCs. In this review, the adsorption mechanism of VOCs onto porous carbons was generally concluded. Porous carbons can be designed as a specific structure for adsorption of aromatic VOCs by controlling the pore structure, hydrophobic sites, π-electronic structure, and surface functional groups. Since there are limited review literatures on porous carbons derived from renewable resources for VOCs adsorption, this paper will provide an overview on the synthesis of porous carbons from biomass and other organic wastes for VOCs adsorption or integrated oxidation processes (e.g., photocatalysis, non-thermal plasma catalysis, chemical catalysis) under ambient conditions with the objective of guiding ...