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With the 2015 Paris Agreement pursuing efforts to limit global temperature increase to below 2°C above pre-industrial levels and the “energy trilemma” goals of energy security, energy equity and environmental sustainability, decarbonisation remains a priority across all of the United Kingdom (United Kingdom) energy system, not just electricity. Electricity and thermal energy storage technologies can offer a host of benefits across the energy value chain through the abilityS to capture, store and then release electricity or thermal energy over a period of time. These benefits include helping capture the full potential of renewable generation and providing services such as frequency response and reserve to Great Britain’s (GB) electricity system. In addition, with the aforementioned climate targets in mind, energy storage can also play a role in facilitating the decarbonisation of other activities and sectors. Here we delve deeper into how energy storage technologies can contribute to both energy sector transformation and more broadly, decarbonisation. Furthermore, we discuss the importance of ensuring a technology-agnostic approach to the development of policy and regulation with relevance to energy storage. This ensures that storage technologies with significant potential to contribute to the ‘energy trilemma’ goals are not precluded from entering the market due to unfavourable policy and regulatory frameworks.

Abstract The consumption of takeaway food is increasing worldwide. Single-use containers used for takeaway food represent a significant source of waste and environmental impacts due to their low recyclability. Consequently, it is important to identify the best available alternatives and improvement opportunities to reduce the environmental impacts of fast-food containers. For these purposes, this study estimates and compares for the first time the life cycle impacts of three most widely-used types of takeaway container: aluminium, polypropylene and extruded polystyrene. These are also compared to reusable polypropylene containers. The findings suggest that single-use polypropylene containers are the worst option for seven out of 12 impacts considered, including global warming potential. They are followed by the aluminium alternative with five highest impacts, including depletion of ozone layer and human toxicity. Overall, extruded polystyrene containers have the lowest impacts due to the lower material and electricity requirements in their manufacture. They are also the best option when compared to reused takeaway polypropylene containers, unless the latter are reused 3–39 times. The number of uses needed for the reusable “Tupperware” polypropylene food savers is even higher, ranging from 16 to 208 times, with terrestrial ecotoxicity being always higher than for extruded polystyrene, regardless of the number of uses. However, extruded polystyrene containers are currently not recycled and cannot be considered a sustainable option. If they were recycled in accordance with the European Union 2025 policy on waste packaging, most of their impacts would be reduced by >18%, while also reducing littering and negative effects on marine organisms. Most of the impacts of the other two types of container would also be reduced (>20%) through increased recycling. Implementing the European Union 2025 policy on recycling of waste packaging would reduce all the impacts by 2%–60%, including a 33% reduction in global warming potential. Based on 2025 million takeaway containers used annually in the European Union, the latter would save 61,700 t CO2 eq./yr, equivalent to the emissions of 55,000 light-duty vehicles. The outcomes of this study will be of interest to packaging manufacturers, food outlets, policy makers and consumers.

Driven by the need to develop a wide variety of products with low environmental impact, biorefineries need to emerge as highly integrated facilities. This becomes effective when overall mass and energy integration through a centralised utility system design is undertaken. An approach combining process integration, energy and greenhouse gas (GHG) emission analyses is shown in this paper for Jatropha biorefinery design, primarily producing biodiesel using oil-based heterogeneously catalysed transesterification or green diesel using hydrotreatment. These processes are coupled with gasification of husk to produce syngas. Syngas is converted into end products, heat, power and methanol in the biodiesel case or hydrogen in the green diesel case. Anaerobic digestion of Jatropha by-products such as fruit shell, cake and/or glycerol has been considered to produce biogas for power generation. Combustion of fruit shell and cake is considered to provide heat. Heat recovery within biodiesel or green diesel production and the design of the utility (heat and power) system are also shown. The biorefinery systems wherein cake supplies heat for oil extraction and seed drying while fruit shells and glycerol provide power generation via anaerobic digestion into biogas achieve energy efficiency of 53 % in the biodiesel system and 57 % in the green diesel system. These values are based on high heating values (HHV) of Jatropha feedstocks, HHV of the corresponding products and excess power generated. Results showed that both systems exhibit an energy yield per unit of land of 83 GJ ha−1. The global warming potential from GHG emissions of the net energy produced (i.e. after covering energy requirements by the biorefinery systems) was 29 g CO2-eq MJ−1, before accounting credits from displacement of fossil-based energy by bioenergy exported from the biorefineries. Using a systematic integration approach for utilisation of whole Jatropha fruit, it is shown that global warming potential and fossil primary energy use can be reduced significantly if the integrated process schemes combined with optimised cultivation and process parameters are adopted in Jatropha-based biorefineries.

Abstract In the context of climate change, global industrialised nations are grappling with transforming energy networks to support a low carbon future. Using an energy justice framework this work aims to understand holistic outcomes of one low-carbon energy network intervention: demand-side response enacted on domestic heat pumps. By exploring participants’ lived experience of a pilot project, from recruitment to installation and use, this work reveals how injustices were reduced, introduced and amplified. Choice, consent, cost, comfort, disruption, and control are highlighted as key aspects of interest when considering the distributive, procedural, and recognition implications of this domestic innovation. For a net reduction of energy injustices to be realised, we highlight the need for project designers to work in partnership with end users to optimise the benefits for the household and the electricity system. Whilst this is a UK study, the themes and findings are internationally applicable for interventions that aim to harness the flexibility of heating, the largest global energy end-use.

AbstractErbium doped silicon-rich silica offers broad band and very efficient excitation of erbium photoluminescence (PL) due to a sensitization effect attributed to silicon nanocrystals (Si-nc), which grow during thermal treatment. PL decay lifetime measurements of sensitised Er3+ ions are usually reported to be stretched or multi exponential, very different to those that are directly excited, which usually show a single exponential decay component.In this paper, we report on SiO2 thin films doped with Si-nc's and erbium. Time resolved PL measurements reveal two distinct 1.54μm Er decay components; a fast microsecond component, and a relatively long lifetime component (10ms). We also study the structural properties of these samples through TEM measurements, and reveal the formation of Er clusters. We propose that these Er clusters are responsible for the fast μs decay component, and we develop rate equation models that reproduce the experimental transient observations, and can explain some of the reported transient behaviour in previously published literature.

Environmental concern for our planet has changed significantly over time due to climate change, caused by an increasing population and the subsequent demand for electricity, and thus increased power generation. Considering that natural gas is regarded as a promising fuel for such a purpose, the need to integrate carbon capture technologies in such plants is becoming a necessity, if gas power plants are to be aligned with the reduction of CO2 in the atmosphere, through understanding the capturing efficacy of different absorbents under different operating conditions. Therefore, this study provided for the first time the comparison of available absorbents in relation to amine solvents (MEA, DEA, and DEA) CO2 removal efficiency, cost, and recirculation rate to achieve Climate change action through caron capture without causing absorbent disintegration. The study analyzed Flue under different amine-based solvent solutions (monoethanolamine (MEA), diethanolamine (DEA), and methyldiethanolamine (MDEA)), in order to compare their potential for CO2 reduction under different operating conditions and costs. This was simulated using ProMax 5.0 software modeled as a simple absorber tower to absorb CO2 from flue gas. Furthermore, MEA, DEA, and MDEA adsorbents were used with a temperature of 38 °C and their concentration varied from 10 to 15%. Circulation rates of 200–300 m3/h were used for each concentration and solvent. The findings deduced that MEA is a promising solvent compared to DEA and MDEA in terms of the highest CO2 captured; however, it is limited at the top outlet for clean flue gas, which contained 3.6295% of CO2 and less than half a percent of DEA and MDEA, but this can be addressed either by increasing the concentration to 15% or increasing the MEA circulation rate to 300 m3/h.

Thermal modelling tools have widely been used in the construction industry at the design stage, either for new build or retrofitting existing buildings, providing data for informed decision-making. The accuracy of thermal models has been subject of much research in recent decades due to the potential large difference between predicted and ‘in-use’ performance – the so called ‘performance gap’. A number of studies suggested that better representation of building physics and operation details in thermal models can improve the accuracy of predictions. However, full-scale model calibration has always been challenging as it is difficult to measure all the necessary boundary conditions in an open environment. Thus, the Energy House facility at the University of Salford – a full-sized end terrace house constructed within an environmental chamber – presents a unique opportunity to conduct full-scale model calibration.\ud \ud The aim of this research is to calibrate Energy House thermal models using various full-scale measurements. The measurements used in this research include the co-heating tests for a whole house retrofit case study, and thermal resistance from window coverings and heating controls with thermostatic radiator valves (TRVs). Thermal models were created using an IESVE (Integrated Environment Solutions Virtual Environment). IESVE is a well-established dynamic thermal simulation tool widely used in analysing the dynamic response of a building based on the hourly input of weather data. The evidence from this study suggests that thermal models using measured U-values and infiltration rates do perform better than the models using calculated thermal properties and assumed infiltration rates. The research suggests that better representations of building physics help thermal models reduce the performance gap. However, discrepancies still exist due to various other underlying uncertainties which need to be considered individually with each case. In relative terms, i.e., variations in percentage, the predictions from thermal models tend to be more reliable than predicting the absolute numbers.

Before lower purity, lower cost silicon (Si) materials, such as compensated Si, can play a role in the terawatt-level (TW) capacity of photovoltaics, a better understanding of the fundamental properties of impurities in compensated Si is essential. In this work, high-resolution photoluminescence (PL) has been used to study the charge carrier radiative recombination through Donor-Acceptor pairs (DAPs) in phosphorus (P) and gallium (Ga) co-doped Si material grown for solar cell applications. The high spectral resolution of our PL system, 0.06 meV, enables us to overcome hitherto prior issues of overlapping spectral lines, giving access to extremely fine structures associated with DA pair (DAP) recombination. Our results confirm the presence of three broad bands and a discrete line structure related to DAP luminescence. The comparison of the discrete line structure due to DAPs recombination in the PL spectra with the theoretically predicted one allows the accurate determination of the Ga ionization energy. Temperature-dependent PL is then used to understand the thermally-induced changes in the DAP luminescence. In particular, we observe that the radiative recombination channel remains active for distant DAPs up to ∼40 K, unlike that for close-range DAPs for which the radiative channel is quenched after only slight increases in the temperature range 10–25 K. Furthermore, the analysis of the temperature dependent changes in the PL intensity of the broad DAP bands up to ∼200 K is used to derive the ionization energy of P donors in compensated Si material. In light of this important information, the significance of using high resolution PL to analyse spectral features in compensated Si is demonstrated.