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Ultra-low NOx emissions from catalytic hydrogen combustion

The objective of this work is to determine the nitrogen oxide emission in the flue gas of a catalytic hydrogencombustion process, operating without premixed hydrogen and air supply. The study was investigated on a noveldesigned gas under glass stove top burner, suitable for domestic kitchen applications. The basic catalytic burnerassembly consists of two platinum coated silicon carbide (SiC) foam disks with a diameter of 150 mm, a thicknessof 10 mm and a porosity of 60 and 80 pores per inch (ppi) respectively. The two catalytic SiC disks are stackedwith 10 mm space between for a uniform air feeding and distribution. Hydrogen is supplied from below theassembly and air is blown in between the two Pt coated catalytic SiC disks, leading to a homogeneous airdistribution and thus a uniform catalytic reaction of hydrogen and air. Tests are performed at hydrogen flowrates of 5, 10 and 15 Nl/min, equivalent to 0.9, 1.8, 2.7 kW power, the hydrogen to oxygen ratios (φ) were fixedto 0.66, 0.5 and 0.33 respectively. Ultra-low nitrogen oxide emissions of 0.09 ppmv to 9.49 ppmv, equivalent to0.007 to 0.37 mg/kWh are achieved with this novel developed catalytic combustion design. These values aresignificantly lower than the present EU regulation of 56 mg/kWh for combustion processes of gaseous fuels forheating applications. This result shows the very high potential of converting hydrogen to heat without harmfulexhaust gases for a broad domestic application in decarbonised gas grids or stationary power to gas applications.
+ ID der Publikation: hslu_101489 + Art des Beitrages: Wissenschaftliche Medien + Sprache: Englisch + Letzte Aktualisierung: 2024-07-03 14:48:57
- University of Freiburg Germany
- Zentral und Hochschulbibliothek Luzern Switzerland
- Lucerne University of Applied Sciences and Arts Switzerland
- Swiss Federal Laboratories for Materials Science and Technology Switzerland
- Lucerne University of Applied Sciences and Arts Switzerland
catalytic combustion, ultra-low NOx, domestic application, hydrogen, non premixing
catalytic combustion, ultra-low NOx, domestic application, hydrogen, non premixing
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