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Ultra-low NOx emissions from catalytic hydrogen combustion

Authors: Ulrich Vogt; Ulrich Vogt; Benjamin Fumey; T. Buetler;

Ultra-low NOx emissions from catalytic hydrogen combustion

Abstract

The objective of this work is to determine the nitrogen oxide emission in the flue gas of a catalytic hydrogencombustion process, operating without premixed hydrogen and air supply. The study was investigated on a noveldesigned gas under glass stove top burner, suitable for domestic kitchen applications. The basic catalytic burnerassembly consists of two platinum coated silicon carbide (SiC) foam disks with a diameter of 150 mm, a thicknessof 10 mm and a porosity of 60 and 80 pores per inch (ppi) respectively. The two catalytic SiC disks are stackedwith 10 mm space between for a uniform air feeding and distribution. Hydrogen is supplied from below theassembly and air is blown in between the two Pt coated catalytic SiC disks, leading to a homogeneous airdistribution and thus a uniform catalytic reaction of hydrogen and air. Tests are performed at hydrogen flowrates of 5, 10 and 15 Nl/min, equivalent to 0.9, 1.8, 2.7 kW power, the hydrogen to oxygen ratios (φ) were fixedto 0.66, 0.5 and 0.33 respectively. Ultra-low nitrogen oxide emissions of 0.09 ppmv to 9.49 ppmv, equivalent to0.007 to 0.37 mg/kWh are achieved with this novel developed catalytic combustion design. These values aresignificantly lower than the present EU regulation of 56 mg/kWh for combustion processes of gaseous fuels forheating applications. This result shows the very high potential of converting hydrogen to heat without harmfulexhaust gases for a broad domestic application in decarbonised gas grids or stationary power to gas applications.

+ ID der Publikation: hslu_101489 + Art des Beitrages: Wissenschaftliche Medien + Sprache: Englisch + Letzte Aktualisierung: 2024-07-03 14:48:57

Country
Switzerland
Keywords

catalytic combustion, ultra-low NOx, domestic application, hydrogen, non premixing

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
58
Top 10%
Top 10%
Top 10%
Green