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Application of the Mott-Schottky model to select potentials for EIS studies on electrodes for electrochemical charge storage

descriptionPublicationkeyboard_double_arrow_right Article , Journal 01 Nov 2018 France, Portugal, Portugal Publisher:Elsevier BVJournal:Electrochimica Acta, volume 289, pages 47-55 (issn: 0013-4686,

Authors:

T.M. Silva; T.M. Silva;

Alberto Adán-Más; Alberto Adán-Más;

M. F. Montemor;

Liliane Guerlou-Demourgues; Liliane Guerlou-Demourgues;

doi: 10.1016/j.electacta.2018.08.077

Application of the Mott-Schottky model to select potentials for EIS studies on electrodes for electrochemical charge storage

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Abstract

Abstract Electrochemical Impedance Spectroscopy (EIS) is a powerful technique to understand the electrode-electrolyte interaction and to evaluate degradation, resistive behaviour and electrochemical activity of energy storage materials used in batteries, pseudocapacitors and supercapacitors among others. However, it can sometimes be misused or under-interpreted. To effectively acquire EIS results, the voltages imposed to the working electrode at which EIS spectra are obtained, shall be critically selected. This work follows a previous study on the EIS response of Nickel-Cobalt hydroxide, and highlights how the Mott-Schottky model can be used as a complementary tool to explain EIS results obtained at different potentials. The Mott-Schottky model is used to understand further the fundamental processes occurring at the electrode-electrolyte interface of nickel-cobalt hydroxide in alkali media and to explain the changes in conductivity of the material that ultimately determine the electrode electrochemical activity. The applicability of the model to assist in the potential selection for EIS studies on other important charge storage materials such as MnOx and MoOx is discussed too.

Countries

France, Portugal, Portugal

Related Organizations

Grenoble Alpes University
France
Instituto Superior de Espinho
Portugal
University of Bordeaux
France
French National Centre for Scientific Research
France
Centre national de la recherche scientifique
France

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Keywords

[CHIM.MATE] Chemical Sciences/Material chemistry, Armazenamento de carga electroquímica, Nickel-cobalt hydroxide, [CHIM.MATE]Chemical Sciences/Material chemistry, Hidróxido de níquel-cobalto, 540, Espectroscopia de impedância eletroquímica, Charge storage, Electrochemical impedance spectroscopy

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Impact of surface patterning on oxygen vacancy formation and subsequent photoelectrochemical performance of TiO2 nanostructures
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doi: 10.1016/j.apsusc.2025.162900
doi: 10.1016/j.apsusc.2025.162900
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Enhancing photocatalytic efficiency with hematite photoanodes: principles, properties, and strategies for surface, bulk, and interface charge transfer improvement
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doi: 10.1039/d3qm01100c
doi: 10.1039/d3qm01100c
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Schottky Interface Enabled Electrospun Rhodium Oxide Doped Gold for Both pH Sensing and Glucose Measurements in Neutral Buffer and Human Serum
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doi: 10.1021/acs.langmuir.4c02999
pmid: 39287604
pmc: PMC11447893
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Impact byBIP!

	citations This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).	71
	popularity This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.	Top 1%
	influence This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).	Top 10%
	impulse This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.	Top 10%

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7. Clean energy

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Fields of Science (3) View all

engineering and technology

electrical engineering, electronic engineering, information engineering

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engineering and technology

electrical engineering, electronic engineering, information engineering

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FCT| Centro de Química Estrutural

Related to Research communities

SDSN Greece

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Synthesis and characterization of Co(OH)2/TiO2 nanotube composites as supercapacitor materials

The effect of cobalt on the chemical and electrochemical behaviour of the nickel hydroxide electrode

Redox active materials for metal compound based hybrid electrochemical energy storage: a perspective view

Achieving high specific charge capacitances in Fe3O4/reduced graphene oxide nanocomposites

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Accelerating water oxidation on BiVO₄ photoanodes via surface modification with Co dopants

Innovative syntheses of immobilized CuxO semiconductors grown on 3D prints and their photoelectrochemical activity for sulfamethoxazole degradation

Humidity-Tolerant Room-Temperature Selective Dual Sensing and Discrimination of NH₃ and NO Using a WS₂/MWCNT Composite

Influence of Ga-halogen bond formation at the interface of nanoporous GaN photoelectrodes for enhanced photoelectrochemical water splitting efficiency

MoO_x-based high-density nanoarrays on a substrate via smart anodizing as novel 3D electrodes for nano-energy applications

Development and characterization of rGO supported CdS MoS2 photoelectrochemical catalyst for splitting water by visible light

Viscosity effect of polyols on the growth of nanostructured titania photoanode for photoelectrochemical water splitting

Impact of surface patterning on oxygen vacancy formation and subsequent photoelectrochemical performance of TiO2 nanostructures

Enhancing photocatalytic efficiency with hematite photoanodes: principles, properties, and strategies for surface, bulk, and interface charge transfer improvement

Schottky Interface Enabled Electrospun Rhodium Oxide Doped Gold for Both pH Sensing and Glucose Measurements in Neutral Buffer and Human Serum