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Mechanisms and kinetics of CO 2 hydrogenation to value-added products: A detailed review on current status and future trends

descriptionPublicationkeyboard_double_arrow_right Article , Journal 01 Dec 2017Publisher:Elsevier BVJournal:Renewable and Sustainable Energy Reviews, volume 80, pages 1,292-1,311 (issn: 1364-0321,

Authors: Samrand Saeidi; Jiří Jaromír Klemeš; Maryam Khoshtinat Nikoo; Fatemeh Sefidkon; Farhad Fazlollahi; Sara Najari; Larry L. Baxter;

doi: 10.1016/j.rser.2017.05.204

Mechanisms and kinetics of CO 2 hydrogenation to value-added products: A detailed review on current status and future trends

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Abstract

Abstract Global warming, fossil fuel depletion and energy security are driving scientists to investigate the mechanism of hydrocarbons production from CO 2 hydrogenation. The need for more comprehensive understanding on mechanism of CO 2 hydrogenation to hydrocarbons remains controversial because of the complex reaction mechanism and a large number of involved species. The micro mechanism of CO 2 hydrogenation to hydrocarbons has been considered as a possible remedy to fulfill the requirements. This review comprehensively discusses two processes: reverse water gas shift (RWGS) and CO 2 hydrogenation to hydrocarbons. The review includes reaction mechanisms and catalyst effects on yields and rates. In addition, the review outlines each of the Fischer-Tropsch (FT) micro mechanisms. The review infers some mechanisms from existing work and proposes a new mechanism that improves several predictions. These mechanisms form the design basis for optimal reactor design.

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	citations This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).	206
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	influence This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).	Top 10%
	impulse This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.	Top 1%