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Towards a climate-dependent paradigm of ammonia emission and deposition

descriptionPublicationkeyboard_double_arrow_right Article , Journal , Other literature type 05 Jul 2013 United Kingdom, Belgium, Spain, Netherlands, France, United Kingdom, Netherlands Publisher:The Royal SocietyJournal:Philosophical Transactions of the Royal Society B: Biological Sciences, volume 368, page 20,130,166 (issn: 0962-8436, eissn: 1471-2970, Copyright policy )Publicly fundedFunded by:EC | ECLAIRE
Authors: Raia Silvia Massad; R.F. Mitchell; Celia Milford; Tom Misselbrook; John T. Walker; Eiko Nemitz; Albert Bleeker; +33 Authors

doi: 10.1098/rstb.2013.0166

pmid: 23713128

pmc: PMC3682750

handle: 2013/ULB-DIPOT:oai:dipot.ulb.ac.be:2013/154398

Towards a climate-dependent paradigm of ammonia emission and deposition

Abstract

Existing descriptions of bi-directional ammonia (NH 3 ) land–atmosphere exchange incorporate temperature and moisture controls, and are beginning to be used in regional chemical transport models. However, such models have typically applied simpler emission factors to upscale the main NH 3 emission terms. While this approach has successfully simulated the main spatial patterns on local to global scales, it fails to address the environment- and climate-dependence of emissions. To handle these issues, we outline the basis for a new modelling paradigm where both NH 3 emissions and deposition are calculated online according to diurnal, seasonal and spatial differences in meteorology. We show how measurements reveal a strong, but complex pattern of climatic dependence, which is increasingly being characterized using ground-based NH 3 monitoring and satellite observations, while advances in process-based modelling are illustrated for agricultural and natural sources, including a global application for seabird colonies. A future architecture for NH 3 emission–deposition modelling is proposed that integrates the spatio-temporal interactions, and provides the necessary foundation to assess the consequences of climate change. Based on available measurements, a first empirical estimate suggests that 5°C warming would increase emissions by 42 per cent (28–67%). Together with increased anthropogenic activity, global NH 3 emissions may increase from 65 (45–85) Tg N in 2008 to reach 132 (89–179) Tg by 2100.

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United Kingdom, Belgium, Spain, Netherlands, France, United Kingdom, Netherlands
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Keywords

[SDE] Environmental Sciences, 550, Climate, ammonia, deposition, managed grassland, [PHYS.PHYS.PHYS-AO-PH] Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph], nitrogen, [ SDE ] Environmental Sciences, [SDU.STU.CL] Sciences of the Universe [physics]/Earth Sciences/Climatology, Urban Development, emission, atmospheric modelling, Built Environment, volatilization, dutch heathland, Química, Nitrogen Cycle, Environmental and Life Sciences, [ SDE.MCG ] Environmental Sciences/Global Changes, Atmospheric modeling, [ PHYS.PHYS.PHYS-AO-PH ] Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph], [SDU.STU.CL]Sciences of the Universe [physics]/Earth Sciences/Climatology, [SDE]Environmental Sciences, [ SDU.STU.CL ] Sciences of the Universe [physics]/Earth Sciences/Climatology, Sciences exactes et naturelles, [SDE.MCG]Environmental Sciences/Global Changes, Earth & Environment, Climate Change, [PHYS.PHYS.PHYS-AO-PH] Physics/Physics/Atmospheric and Oceanic Physics, 333, Air and Sustainability, EELS - Earth, Atmospheric Sciences, soil, Emission, Birds, CAS - Climate, Ammonia, Air Pollution, Animals, compensation point, Deposition, [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph], canopy, gas-particle interactions, model, Atmosphere, Models, Theoretical, United States, [SDE.MCG] Environmental Sciences/Global Changes, [SDU.STU.CL] Sciences of the Universe/Earth Sciences/Climatology, plant-atmosphere exchange, Climate Emission Environment

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    citations
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    		 343
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    		 Top 0.1%
    influence
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    impulse
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
343
Top 0.1%
Top 1%
Top 1%
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