According to the European Commission, green infrastructure (GI) is conceived as a strategically planned network of natural and semi-natural areas. This definition highlights three important issues: environment protection, ecosystems multifunctionality and ecological connectivity. Building upon a methodology that identifies a Sardinian regional GI in relation to four values (conservation value, natural value, recreational value and landscape value), this study aims at assessing the suitability of areas situated within and outside protected areas’ boundaries to be included in the above-mentioned Sardinian regional GI. In relation to conservation value, outcomes reveal a higher suitability of patches situated within protected areas to be included in the regional GI, whereas in relation to the other three values, the behavioral patterns are less evident. These results suggest specific policy recommendations such as mitigation of land-taking processes, increase of Natura 2000 Network’s size, accurate identification of landscape goods, and improved accessibility to sites characterized by outstanding natural beauty.