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Global analysis of continental boundary layer new particle formation based on long-term measurements

Authors: T. Nieminen; T. Nieminen; V.-M. Kerminen; T. Petäjä; P. P. Aalto; M. Arshinov; E. Asmi; +41 Authors

Global analysis of continental boundary layer new particle formation based on long-term measurements

Abstract

Abstract. Atmospheric new particle formation (NPF) is an important phenomenon in terms of global particle number concentrations. Here we investigated the frequency of NPF, formation rates of 10 nm particles, and growth rates in the size range of 10–25 nm using at least 1 year of aerosol number size-distribution observations at 36 different locations around the world. The majority of these measurement sites are in the Northern Hemisphere. We found that the NPF frequency has a strong seasonal variability. At the measurement sites analyzed in this study, NPF occurs most frequently in March–May (on about 30 % of the days) and least frequently in December–February (about 10 % of the days). The median formation rate of 10 nm particles varies by about 3 orders of magnitude (0.01–10 cm−3 s−1) and the growth rate by about an order of magnitude (1–10 nm h−1). The smallest values of both formation and growth rates were observed at polar sites and the largest ones in urban environments or anthropogenically influenced rural sites. The correlation between the NPF event frequency and the particle formation and growth rate was at best moderate among the different measurement sites, as well as among the sites belonging to a certain environmental regime. For a better understanding of atmospheric NPF and its regional importance, we would need more observational data from different urban areas in practically all parts of the world, from additional remote and rural locations in North America, Asia, and most of the Southern Hemisphere (especially Australia), from polar areas, and from at least a few locations over the oceans.

Countries
Finland, Finland, France
Keywords

CONDENSATION NUCLEI PRODUCTION, FORMATION EVENTS, AEROSOL-SIZE DISTRIBUTION, QC1-999, [SDU] Sciences of the Universe [physics], ATMOSPHERIC NUCLEATION, SULFURIC-ACID, PARTICULATE MATTER, QD1-999, [SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, FREE TROPOSPHERE, [SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, [SDU.OCEAN] Sciences of the Universe [physics]/Ocean, Atmosphere, Physics, Physical sciences, Chemistry, Chemical sciences, [SDU]Sciences of the Universe [physics], BLACK CARBON, HIGH-ALTITUDE SITE, AIRBORNE MEASUREMENTS

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    Top 1%
    influence
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    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
124
Top 1%
Top 10%
Top 1%