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Sulfate geoengineering: a review of the factors controlling the needed injection of sulfur dioxide

Authors: Daniele Visioni; Valentina Aquila; Valentina Aquila; Giovanni Pitari;

Sulfate geoengineering: a review of the factors controlling the needed injection of sulfur dioxide

Abstract

Abstract. Sulfate geoengineering has been proposed as an affordable and climate-effective means for temporarily offset the warming produced by the increase of well mixed greenhouse gases (WMGHG). This climate engineering technique has been planned for a timeframe of a few decades needed to implement global inter-governmental measures needed to achieve stabilization of the atmospheric content of WMGHGs (CO2 in particular). The direct radiative effects of sulfur injection in the tropical lower stratosphere can be summarized as increasing shortwave scattering with consequent tropospheric cooling and increasing long- wave absorption with stratospheric warming. Indirect radiative effects are related to induced changes in the ozone distribution, stratospheric water vapor abundance, formation and size of upper tropospheric cirrus ice particles and lifetime of longlived species, namely CH4 in connection with OH changes through several photochemical mechanisms. A direct comparison of the net effects of WMGHG increase with direct and indirect effects of sulfate geoengineering may help fine-tune the best amount of sulfate to be injected in an eventual realization of the experiment. However, we need to take into account large uncertainties in the estimate of some of these aerosol effects, such as cirrus ice particle size modifications.

Country
Italy
Keywords

Chemistry, Physics, QC1-999, QD1-999

  • BIP!
    Impact byBIP!
    citations
    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    38
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    Top 10%
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
    Top 10%
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
38
Top 10%
Top 10%
Top 10%
Green
gold