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China has achieved impressive rapid economic growth over the past 30 years but accompanied by significant extreme weather events and environmental changes caused by global change and overfast urbanization. Using the absolute hazards index (AHI), we assessed the spatial distribution patterns and related health effects of 4 major extreme natural disasters, including drought, floods (landslides, mudslides), hails, and typhoons from 2000 to 2011 at the provincial level in China. The results showed that (1) central and south China were the most affected by the 4 natural disasters, and north China suffered less; (2) the provinces with higher AHI suffered most from total death, missing people, collapse, and emergently relocated population; (3) the present health emergency response system to disasters in China mainly lacks a multidisciplinary approach. In the concluding section of this article, suggestions on preparedness and rapid response to extreme health events from environmental changes are proposed.

Decreasing nutrient losses from excessive synthetic fertilizer inputs is the direct and valid way to address low nutrient use efficiency and the related environmental consequences. Here, we established a comprehensive database of nitrogen (N), phosphorus (P), and carbon (C) losses from rice paddy fields in China, which we used to evaluate fertilization-induced losses and the impact of environmental factors, and to mitigate losses by adopting alternative fertilization options and setting input thresholds. Our results showed that most N-loss pathways had exponential increases with additional N input. In average, 23.8% of the N applied was lost via NH3 (16.1%), N2O (0.3%), leaching (4.8%), and runoff (2.6%). Total P loss was approximately 2.7% of the input, composed of leaching (1.3%) and runoff (1.4%). C lost as CH4 accounted for 4.9% of the organic C input. A relative importance analysis indicated that climate or soil variation rather than fertilizer rate was the dominant factor driving N and P leaching, and CH4 emissions. Based on the sensitivity of multiple N-loss pathways to N fertilization, we propose upper thresholds for N inputs of 142–191 kg N ha−1 across four rice types, which would avoid dramatic increases in N losses. Compared to conventional chemical fertilization, alternative fertilization options had diverse performances: enhanced-efficiency N fertilizer reduced N loss rate by 7.8 percent points and the global warming potential (GWP, considering N2O and CH4 emissions) by 28.8%; combined manure and chemical N fertilizer reduced N loss rate by 9.0 percent points but increased the GWP by 56.9%; straw return had no effect on total N loss but almost doubled the GWP. Using nutrient sources most appropriate to site-specific conditions is demonstrated as a robust way to decrease nutrient losses. Setting nutrient input thresholds would also contribute to the mitigation of environmental pollution, especially in regions with poor fertilization recommendation systems.

Abstract Electrolyte-separator-free fuel cell (EFFC) is a new emerging energy conversion technology. The EFFC consists of a single-component of nanocomposite material which works as a one-layer fuel cell device contrary to the traditional three-layer anode–electrolyte–cathode structure, in which an electrolyte layer plays a critical role. The nanocomposite of a single homogenous layer consists of a mixture of semiconducting and ionic materials that provides the necessary electrochemical reaction sites and charge transport paths for a fuel cell. These can be accomplished through tailoring ionic and electronic (n, p) conductivities and catalyst activities, which enable redox reactions to occur on nano-particles and finally accomplish a fuel cell function.

The acceptability, energy consumption, and environmental benefits of electric vehicles are highly dependent on travel patterns. With increasing ride-hailing popularity in mega-cities, urban mobility patterns are greatly changing; therefore, an investigation of the extent to which electric vehicles would satisfy the needs of ride-hailing drivers becomes important to support sustainable urban growth. A first step in this direction is reported here. GPS-trajectories of 144,867 drivers over 104 million km in Beijing were used to quantify the potential acceptability, energy consumption, and costs of ride-hailing electric vehicle fleets. Average daily travel distance and travel time for ride-hailing drivers was determined to be 129.4 km and 5.7 h; these values are substantially larger than those for household drivers (40.0 km and 1.5 h). Assuming slow level-1 (1.8 KW) or moderate level-2 (7.2 KW) charging is available at all home parking locations, battery electric vehicles with 200 km all electric range (BEV200) could be used by up to 47% or 78% of ride-hailing drivers and electrify up to 20% or 55% of total distance driven by the ride-hailing fleet. With level-2 charging available at home, work, and public parking, the acceptance ceiling increases to up to 91% of drivers and 80% of distance. Our study suggests that long range BEVs and widespread level-2 charging infrastructure are needed for large-scale electrification of ride-hailing mobility in Beijing. The marginal benefits of increased all electric range, effects on charging infrastructure distribution, and payback times are also presented and discussed. Given the observed heterogeneity of ride-hailing vehicle travel, our study outlines the importance of individual-level analysis to understand the electrification potential and future benefits of electric vehicles in the era of shared smart transportation.

There are various transport phenomena (gas-phase species, heat, and momentum) occurring at different length scales in anode-supported solid oxide fuel cells (SOFCs), which are strongly affected by catalytic surface reactions at active triple-phase boundaries (TPBs) between the void space (for gas), Ni (catalysts for electrons), and YSZ (an electrolyte material for ions). To understand the multiscale chemical-reacting transport processes in the cell, a three-dimensional numerical calculation approach (the computational fluid dynamics (CFD) method) is further developed and applied for a composite domain including a porous anode, fuel gas flow channel, and solid interconnect. By calculating the rate of microscopic surface-reactions involving the surface-phase species, the gas-phase species/heat generation and consumption related to the internal reforming reactions have been identified and implemented. The applied microscopic model for the internal reforming reactions describes the adsorption and desorption reactions of six gas-phase species and surface reactions of 12 surface-adsorbed species. The predicted results are presented and analyzed in terms of the gas-phase species and temperature distributions and compared with those predicted by employing the global reaction scheme for the internal reforming reactions.

The effect of substrate changes on the performance and microbial community of two-chamber microbial fuel cells (MFCs) was investigated in this study. The MFCs enriched with a single substrate (e.g., acetate, glucose, or butyrate) had different acclimatization capability to substrate changes. The MFC enriched with glucose showed rapid and higher power generation, when glucose was switched with acetate or butyrate. However, the MFC enriched with acetate needed a longer adaptation time for utilizing glucose. Microbial community was also changed when the substrate was changed. Clostridium and Bacilli of phylum Firmicutes were detected in acetate-enriched MFCs after switching to glucose. By contrast, Firmicutes completely disappeared and Geobacter-like species were specifically enriched in glucose-enriched MFCs after feeding acetate to the reactor. This study further suggests that the type of substrate fed to MFC is a very important parameter for reactor performance and microbial community, and significantly affects power generation in MFCs.

AbstractThe rotational spectra of two isotopologues of the 1:1 complex formed between acetone and ethanol have been recorded and analyzed by using Fourier‐transform microwave spectroscopy. One rotamer was detected, in which ethanol adopts the gauche form. The two subunits are linked by a conventional O−H⋅⋅⋅O and a weak C−H⋅⋅⋅O hydrogen bond, forming a six‐membered ring. Each rotational transition is split into five component lines due to the internal rotations of two nonequivalent acetone methyl groups. The V3 barriers to internal rotation of the two CH3 tops of acetone were determined to be 252(4) and 220(1) cm−1, which are noticeably lower than the value for the monomer (266 cm−1).

The benefits of introducing heating, CO2 supply, ventilation and LED lighting in a Chinese solar greenhouse are investigated. To that end, a two time-scale receding horizon optimal control system is assumed to accompany the introduction. The model of the Chinese solar greenhouse dynamics used by the optimal control system incorporates the effect of a north wall, present in any Chinese solar greenhouse. This wall stores heat during the day and releases heat at night to improve temperature. The optimal control system also takes control of a thermal blanket, that can be partly opened and closed to reduce heat loss to the environment. Apart from performing real-time optimal control, the optimal control system enables computation of improvements in terms of profit. Finally the feasibility of real-time implementation of the two time-scale receding horizon optimal control system on a personal computer is verified.