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International Journal of Greenhouse Gas Control
Article . 2021 . Peer-reviewed
License: Elsevier TDM
Data sources: Crossref
http://dx.doi.org/10.1016/j.ij...
Article
License: Elsevier TDM
Data sources: Sygma
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Analysis of the physicochemical detectability and impacts of offshore CO2 leakage through multi-scale modelling of in-situ experimental data using the PLUME model

Authors: Jerry Blackford; Umer Saleem; Jianghui Li; Anita Flohr; Ben Roche; Allison Schaap; Marius Dewar; +4 Authors

Analysis of the physicochemical detectability and impacts of offshore CO2 leakage through multi-scale modelling of in-situ experimental data using the PLUME model

Abstract

Abstract Carbon storage is required to keep rising global temperatures below 2°C, meanwhile, storage reservoirs monitoring is required for assurance of early detection of potential leakages. Projects such as QICS and STEMM-CCS have used small in-situ experiments to develop detection techniques, tools, and strategies. Given the expense of experiments it is crucial to develop accurate simulation models that replicate observed behaviours and can be extrapolated to many different scenarios. However, anomalies occur between modelled and experimental data, and a key question has been how can the models be improved? This has been approached through the development of a complex modelling system to include the effects of coastal hydrodynamics on very localised experiments, with a new multi-phase leakage model – PLUME, integrated into a high-resolution hydrodynamic model, and linked to a carbonate system for CO2 analysis. The resolution of the nested domains range from 2.5 km at the boundaries to approximately 0.5 - 1.0 m at the release sites. The efficacy of the PLUME model is demonstrated with application to the STEMM-CCS and QICS experimental sites in 120 and 9-12 m water depths respectively. Results show that the newly developed model can predict observed pCO2 and pH changes within acceptable errors. Local effects are shown to be affected greatly by both the resolution and the water currents, with momentary spikes in pCO2 and reductions in pH caused by tidal oscillation. The spatial impacts of the releases are shown to move with the tide, covering a far greater area over a tidal cycle.

Country
United Kingdom
Keywords

550, 551

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
9
Top 10%
Average
Top 10%
Green